Supersolidity in electron-hole bilayers with a large density - - PowerPoint PPT Presentation

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Supersolidity in electron-hole bilayers with a large density - - PowerPoint PPT Presentation

Supersolidity in electron-hole bilayers with a large density imbalance Francesca Maria Marchetti ICSCE-5, 8 February 2011 In collaboration with Meera Parish & Peter Littlewood Cavendish Laboratory, University of Cambridge, UK [1] arxiv >


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Francesca Maria Marchetti

Supersolidity in electron-hole bilayers with a large density imbalance

ICSCE-5, 8 February 2011

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In collaboration with

Supersolidity in imbalanced electron-hole bilayers Meera Parish & Peter Littlewood Cavendish Laboratory, University of Cambridge, UK [1] arxiv > cond.mat > 1009.1420 Previous related work on imbalanced Fermi gases: [2] Nature Physics 3, 124 (2007) [3] Phys. Rev. Lett. 98 98, 160402 (2007)

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Background: Two component Fermi gases

Supersolidity in imbalanced electron-hole bilayers BEC BCS ✧ Tunable interactions ✧ BEC-BCS crossover

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Background: Two component Fermi gases

Supersolidity in imbalanced electron-hole bilayers BEC BCS ✧ Tunable interactions ✧ BEC-BCS crossover

[Zwierlein et al. Nature (2005)]

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Background: Imbalanced Fermi gases

Supersolidity in imbalanced electron-hole bilayers BEC BCS Can superfluidity persist in presence of a population imbalance? ✧ Tunable interactions ✧ BEC-BCS crossover ✧ Density imbalance frustrates pairing

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Background: T=0 phase diagram

Supersolidity in imbalanced electron-hole bilayers

[Parish, Marchetti et al. Nature Physics (2007)] [Sheehy et al. PRL (2006)]

BEC BCS

[Shin et al. PRL (2006)]

N N SF Fully paired SF phase Macroscpic spatial phase separation between SF and N (inhomogeneous) Polarised SF or 1FS breached pairing (space homogeneous) Bose-Fermi mixture

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Background: T=0 phase diagram

Supersolidity in imbalanced electron-hole bilayers

[Parish, Marchetti et al. Nature Physics (2007)] [Sheehy et al. PRL (2006)]

FFLO

BEC BCS FFLO phase Fully paired SF phase Macroscpic spatial phase separation between SF and N (inhomogeneous)

[Shin et al. PRL (2006)]

N N SF Polarised SF or 1FS breached pairing (space homogeneous) Bose-Fermi mixture SUPERSOLID PHASE

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Background: FFLO unlikely in 3D Fermi gases

Supersolidity in imbalanced electron-hole bilayers ✧ Experiments (Rice & MIT): FFLO elusive  Displacement of Fermi surface: …allows the system to polarise …allows Fermi surface nesting  Phase separation dominates over FFLO
  However …it costs kinetic energy …nesting is partial


[Liao et al. Nature (2010)]

FFLO FFLO phase

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Motivation: Relevance to other systems

Supersolidity in imbalanced electron-hole bilayers  Magnetised superconductors  QCD and neutron stars

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Motivation: Relevance to other systems

Supersolidity in imbalanced electron-hole bilayers  Magnetised superconductors  QCD and neutron stars  Electron-hole systems (N.B. here the density is varied) BEC BCS

e- h+ e- e- e- e- e- h+ h+ h+ h+ e- h+ e- h+ h+

BEC of bound excitons exciton insulator

e- h+

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e-

Motivation: Relevance to other systems

Supersolidity in imbalanced electron-hole bilayers  Magnetised superconductors  QCD and neutron stars  Electron-hole systems (N.B. here the density is varied) BEC BCS

e- h+ e- e- e- e- e- h+ h+ h+ h+ e- h+ e- h+ h+

BEC of bound excitons exciton insulator

e- h+ e- e-

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Electron-hole bilayers: FFLO more ‘likely’

Supersolidity in imbalanced electron-hole bilayers

  • 2. No phase separation on macro-scales

e- e- e- e- e- e- h+ h+ 1 h+ h+ h+

  • 1. Enhanced Fermi surface nesting

3D 2D 1D valence band conduction band position QW1 QW2 electron-hole bilayers: better route to achieve FFLO!

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Electron-hole bilayers: FFLO more ‘likely’

Supersolidity in imbalanced electron-hole bilayers e- e- e- e- e- e- h+ h+ 1 h+ h+ h+ Novel ‘bosonic’ limit of FFLO valence band conduction band position QW1 QW2

  • 2. No phase separation on macro-scales

electron-hole bilayers: better route to achieve FFLO!

  • 1. Enhanced Fermi surface nesting

3D 2D 1D

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Electron-hole bilayers: Experimental realisations

Supersolidity in imbalanced electron-hole bilayers  Optically pumped coupled quantum wells

[Butov et al. Nature (2002)] [Snoke et al. Nature (2002)] […and many more…]

⇒ Equilibrium phase diagram  Individually contacted doped layers

[Croxall et al. PRL (2008)] [Seamons et al. PRL (2009)]

e- e- e- e- e- e- h+ h+ 1 h+ h+ h+ valence band conduction band position QW1 QW2

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Electron-hole bilayers: Hamiltonian

Supersolidity in imbalanced electron-hole bilayers 1 1 1 1 1 1 1 2 2 2 2 2 ⇒ No spin (spin polarised) bare intra-layer Coulomb interaction bare inter-layer

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Limit of large imbalance: Variational ground state

Supersolidity in imbalanced electron-hole bilayers 1 1 1 1 1 1 1 2  single particle in the 2nd layer + Fermi see in the 1st layer (SF) (FFLO) relative k CoM Q  Good description of both low and high density limit

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Limit of large imbalance: Variational ground state

Supersolidity in imbalanced electron-hole bilayers 1 1 1 1 1 1 1 2  Good description of both low and high density limit (N) Interpolate by screening the interactions (within RPA) = dress with density fluctuations, including particle-hole excitations (SF)  single particle in the 2nd layer + Fermi see in the 1st layer relative k CoM Q

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Phase diagram

Supersolidity in imbalanced electron-hole bilayers

  • 2. Eigenvalue equation

 Read also as mean-field (linearised) gap equation

  • 1. Minimise
  • 3. Unbinding transition

 SF & FFLO  Parameters: exciton Bohr radius
 ⇒ interlayer distance ⇒ dimensionless density ⇒ mass ratio

[Yamashita et al. J Phys Soc Japan (2010)] [Pieri et al. PRB (2007)] [Subasi et al. PRB (2010)]

⇒ Current theories ⇒ … some neglect screening ⇒ … some neglect finite Q FFLO (next talk)

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Phase diagram

Supersolidity in imbalanced electron-hole bilayers

  • 2. Eigenvalue equation

 Read also as mean-field (linearised) gap equation

  • 1. Minimise
  • 3. Unbinding transition

[Yamashita et al. J Phys Soc Japan (2010)] [Pieri et al. PRB (2007)] [Subasi et al. PRB (2010)]

 Parameters: exciton Bohr radius
 ⇒ Current theories ⇒ … some neglect screening ⇒ … some neglect finite Q FFLO (next talk)  SF & FFLO ⇒ interlayer distance ⇒ dimensionless density ⇒ mass ratio

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Phase diagram of fully imbalanced EH bilayer

Supersolidity in imbalanced electron-hole bilayers

[arxiv/cond.mat/1009.1420]

high density low density ⇒ interlayer distance ⇒ dimensionless density ⇒ mass ratio  GaAs:

h+ e- h+ e-

FFLO region enhanced if minority particle lighter

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Effect of screening on the LOFF phase

Supersolidity in imbalanced electron-hole bilayers  Unscreened case ⇒ Numerically ⇒ Analytically

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Effect of screening on the LOFF phase

Supersolidity in imbalanced electron-hole bilayers  Unscreened case ⇒ Numerically ⇒ Analytically

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Which kind of FFLO phase?

Supersolidity in imbalanced electron-hole bilayers

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Dilute gas of minority particles: Interactions

Supersolidity in imbalanced electron-hole bilayers  Normal phase: ⇒ repulsive and dipolar : the dilute gas is a Fermi liquid 1
 2
 effective interaction between two unbound minority particles (RPA)  Excitonic phase: 1
 2
 ⇒ also repulsive and dipolar : no phase separation (biexciton formation suppressed for single spin species & ) well separated excitons (dipoles)

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Phenomenology of ‘bosonic’ FFLO

Supersolidity in imbalanced electron-hole bilayers 1
 2
  Landau theory for = exciton density chemical potential minimum energy at

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Phenomenology of ‘bosonic’ FFLO

Supersolidity in imbalanced electron-hole bilayers 1
 2
  Landau theory for = exciton density (weak crystalisation theory)  Complex order parameter chemical potential minimum energy at  Minimal energy solution ⇒ supersolid: exciton condesate with 2D spatial modulation (diagonal and off-diagonal order)

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Observing FFLO

Supersolidity in imbalanced electron-hole bilayers Exciton binding energy in GaAs = upper bound for the FFLO critical temperature

  • 1. Light scattering off the spatial modulations
  • 2. Photon angular emission

(electron hole recombining): finite momentum pairing ( ) GaAs 1
 2


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Conclusions

Supersolidity in imbalanced electron-hole bilayers  Electron-hole bilayers: promising for observing exotic pairing phenomena  Evidence of FFLO phase at large imbalance: finite-Q exciton in presence of a fermi sea  Dilute gas of finite-Q excitons: condensation with 2D spatial modulation (a supersolid)  Prospects for experimental observation ⇒ bosonic limit of FFLO

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Additional slides

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Motivation: Relevance to other systems

Supersolidity in imbalanced electron-hole bilayers  Magnetised superconductors SC Zeeman term

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Include p-h excitation (in within RPA)

Supersolidity in imbalanced electron-hole bilayers  Interpolate between high and low density via RPA 1 1 1 1 1 1 1 2  Full imbalance limit:  Screening between 12 through 11 = + + … = + 1
 1
 1
 1
 1
 = + + … = + 1
 1
 1
 polarisation operator (Linhard function)

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Phase diagram

Supersolidity in imbalanced electron-hole bilayers

  • 2. Eigenvalue equation

 Read also as mean-field (linearised) gap equation (BEC-BCS crossover)

  • 1. Minimise
  • 3. Unbinding transition: compare with

 SF & FFLO ⇒ minority particle chemical potential

[Yamashita et al. J Phys Soc Japan (2010)] [Pieri et al. PRB(2007)] [Subasi et al. PRB (2010)]

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Comparison with the polaron approach

Supersolidity in imbalanced electron-hole bilayers  Our approach + screened Coulomb interactions (infinite particle-hole excitations) bound state unbound state  In cold atoms (majority Fermi sea non-interacting and interspecies interaction short range): POLARON ANSATZ add a single particle-hole excitation  Not profitable to just excite one particle-hole pair when interactions are long-range and the majority Fermi sea is interacting

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Phase diagram of fully imbalanced EH bilayer

Supersolidity in imbalanced electron-hole bilayers

[arxiv/cond.mat/1009.1420]

high density low density  Low density: Q=0 exciton (SF) (two-body limit)  High density: screening causes unbinding (N)  Intermediate density: Significant region of FFLO  FFLO region enhanced if minority particle lighter

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Changing the mass ratio

Supersolidity in imbalanced electron-hole bilayers  FFLO region enhanced if minority particle lighter

[arxiv/cond.mat/1009.1420]

 A Q=0 exciton requires a minority particle to sit above the Fermi sea ⇒ Kinetic cost increases for lighter m2 favouring FFLO

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Behaviour of Qmin

Supersolidity in imbalanced electron-hole bilayers  Second order phase transitions at the FFLO-N transition

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Effect of screening on the LOFF phase

Supersolidity in imbalanced electron-hole bilayers

[Yamashita et al. J Phys Soc Japan (2010)]

 At the unbinding transitions ( ) the integral is divergent for , so the exciton with is always bound ( )  Unscreened case ⇒ Numerically ⇒ Analytically:

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Dilute gas of minority particles: Interactions

Supersolidity in imbalanced electron-hole bilayers  Normal phase: effective interaction between two unbound minority particles (RPA) + 1
 1
 = ⇒ repulsive and dipolar : the dilute gas is a Fermi liquid  Well separated excitons (dipoles) 1
 2
 1
 2
 ⇒ also repulsive and dipolar : no phase separation (biexciton formation suppressed for single spin species & )

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Transparency title

Supersolidity in imbalanced electron-hole bilayers