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■♥tr♦❞✉❝t✐♦♥ ❇✐❣✈✐s ♦✈❡r✈✐❡✇ ❇✐❣✈✐s ❞❡♠♦ ❱✐s✉❛❧✐s✐♥❣ ❜✐❣ ❞❛t❛ ✐♥ ❘ ❆♣r✐❧ ✷✵✶✸ ❇✐r♠✐♥❣❤❛♠ ❘ ❯s❡r ▼❡❡t✐♥❣ ❆❧❛st❛✐r ❙❛♥❞❡rs♦♥ ✇✇✇✳❆❧❛st❛✐r❙❛♥❞❡rs♦♥✳❝♦♠ ✷✸r❞ ❆♣r✐❧ ✷✵✶✸

■♥tr♦❞✉❝t✐♦♥ ❇✐❣✈✐s ♦✈❡r✈✐❡✇ ❇✐❣✈✐s ❞❡♠♦ ❚❤❡ ❝❤❛❧❧❡♥❣❡ ♦❢ ✈✐s✉❛❧✐s✐♥❣ ❜✐❣ ❞❛t❛ ❖♥❧② ❛ ❢❡✇ ♠✐❧❧✐♦♥ ♣✐①❡❧s ♦♥ ❛ s❝r❡❡♥✱ ❜✉t ♠❛♥② ♠♦r❡ ❞❛t❛ ♣♦✐♥ts ❚❤❡r❡❢♦r❡ ♥❡❡❞ t♦ ❣❡♥❡r❛t❡ ❛ s✉✐t❛❜❧❡ s✉♠♠❛r② t♦ ♣❧♦t ✐♥st❡❛❞ ❉✐r❡❝t❧② ✈✐s✉❛❧✐s✐♥❣ r❛✇ ❜✐❣ ❞❛t❛ ✐s ♣r♦❜❛❜❧② ♣♦✐♥t❧❡ss ✱ ❛t ❧❡❛st ❢♦r st❛t✐❝ ❣r❛♣❤✐❝s ✭r❡❛❧✲t✐♠❡ ♠❛♥✐♣✉❧❛t✐♦♥ ♦❢ ❜✐❣ ❞❛t❛✱ ❡✳❣✳ ✢② t❤r♦✉❣❤s ✐s ❛♥♦t❤❡r ♠❛tt❡r✳ ✳ ✳ ✮ → ❆ t②♣✐❝❛❧ ✶❉✴✷❉ ♣❧♦t ♦❢ ❜✐❣ ❞❛t❛ ✇✐❧❧ ❤❛✈❡ ❧♦ts ♦❢ ♦✈❡r❧❛♣♣✐♥❣ ✫ t❤❡r❡❢♦r❡ ♦❜s❝✉r❡❞ ♣♦✐♥ts✿ t❤❡s❡ ❞✐✛❡r❡♥t ✈❛❧✉❡s ✇✐❧❧ ❜❡ ✈✐s✉❛❧❧② ✐♥❞✐st✐♥❣✉✐s❤❛❜❧❡

■♥tr♦❞✉❝t✐♦♥ ❇✐❣✈✐s ♦✈❡r✈✐❡✇ ❇✐❣✈✐s ❞❡♠♦ ❍✐❞❞❡♥ ♣❧♦t ♣♦✐♥ts ❙✐♥❣❧❡ ✈s✳ ♠✉❧t✐♣❧❡ ♦✈❡r❧❛♣♣✐♥❣ ♣♦✐♥ts ♣❞❢✭❢✐❧❡ ❂ ✧◆✶✳♣❞❢✧✱ ❝♦♠♣r❡ss ❂ ❋❆▲❙❊✮❀ ♣❧♦t✭✶✱ ✶✱ ♣❝❤ ❂ ✶✾✮ ❜♠♣✭❢✐❧❡ ❂ ✧◆✶✳❜♠♣✧✱ ❛♥t✐❛❧✐❛s ❂ ✧♥♦♥❡✧✮❀ ♣❧♦t✭✶✱ ✶✱ ♣❝❤ ❂ ✶✾✮ ① ❁✲ r❡♣✭✶✱ ✶❡✸✮ ★ ✶✵✵✵ ✐❞❡♥t✐❝❛❧ ♣♦✐♥ts ♣❞❢✭❢✐❧❡ ❂ ✧◆✶✵✵✵✳♣❞❢✧✱ ❝♦♠♣r❡ss ❂ ❋❆▲❙❊✮❀ ♣❧♦t✭①✱ ①✱ ♣❝❤ ❂ ✶✾✮ ❜♠♣✭❢✐❧❡ ❂ ✧◆✶✵✵✵✳❜♠♣✧✱ ❛♥t✐❛❧✐❛s ❂ ✧♥♦♥❡✧✮❀ ♣❧♦t✭①✱ ①✱ ♣❝❤ ❂ ✶✾✮ ❣r❛♣❤✐❝s✳♦❢❢✭✮ 1.4 1.4 1.2 1.2 1.0 1.0 1 ● x ● 0.8 0.8 0.6 0.6 0.6 0.8 1.0 1.2 1.4 0.6 0.8 1.0 1.2 1.4 1 x ❚❤❡ ✷ ♣❧♦ts ❧♦♦❦ ✐❞❡♥t✐❝❛❧ ✭❛♣❛rt ❢r♦♠ s✉❜t❧❡ ❛♥t✐✲❛❧✐❛s✐♥❣ ❡✛❡❝ts✮

■♥tr♦❞✉❝t✐♦♥ ❇✐❣✈✐s ♦✈❡r✈✐❡✇ ❇✐❣✈✐s ❞❡♠♦ ■♠❛❣❡ ✜❧❡ s✐③❡ ❝♦♠♣❛r✐s♦♥ ▲✐st t❤❡ s✐③❡ ♦❢ ❡❛❝❤ ✐♠❛❣❡ ✜❧❡ ✭✐♥ ❜②t❡s✮✿ s❛♣♣❧②✭❧✐st✳❢✐❧❡s✭♣❛tt❡r♥❂✧◆✶✳✯✧✮✱ ❢✉♥❝t✐♦♥✭❢✮ ❢✐❧❡✳✐♥❢♦✭❢✮✩s✐③❡✮ ◆✶✵✵✵✳❜♠♣ ◆✶✵✵✵✳♣❞❢ ◆✶✳❜♠♣ ◆✶✳♣❞❢ ✷✸✶✹✼✽ ✼✺✸✾✵ ✷✸✶✹✼✽ ✶✷✹✺✷ ❚❤❡ ❜✐t♠❛♣ ❣r❛♣❤✐❝s r❛st❡r ✐♠❛❣❡s ❛r❡ ✐❞❡♥t✐❝❛❧ ✐♥ s✐③❡✱ ❜✉t t❤❡ ✭✉♥❝♦♠♣r❡ss❡❞✮ ✈❡❝t♦r ❣r❛♣❤✐❝s P❉❋s ❞✐✛❡r ✐♥ s✐③❡ ❜② ❛ ❢❛❝t♦r ∼ ✻ ❘❛st❡r ❣r❛♣❤✐❝s r❡s♦❧✈❡ ♦✈❡r❧❛♣s✿ ✶✵✵✵ ♦✈❡r❧❛♣♣✐♥❣ ♣♦✐♥ts ≡ ✶ ♣♦✐♥t✱ ❜✉t ✈❡❝t♦r ❣r❛♣❤✐❝s r❡t❛✐♥ ❡❛❝❤ ♣♦✐♥t ❛s ❛ s❡♣❛r❛t❡ ❡♥t✐t② ❙✐♠✐❧❛r ♣r✐♥❝✐♣❧❡ r❡q✉✐r❡❞ ❢♦r ❇✐❣ ❉❛t❛✱ ❜✉t ♥❡❡❞ ♠♦r❡ ❝♦♥tr♦❧✳ ✳ ✳

■♥tr♦❞✉❝t✐♦♥ ❇✐❣✈✐s ♦✈❡r✈✐❡✇ ❇✐❣✈✐s ❞❡♠♦ ❚❤❡ ❜✐❣✈✐s ❝♦♥❝❡♣t ❉♦✇♥❧♦❛❞ t❤❡ ♣❛♣❡r ✭✈✐t❛✳❤❛❞✳❝♦✳♥③✴♣❛♣❡rs✴❜✐❣✈✐s✳❤t♠❧✮✱ ❜② ❍❛❞❧❡② ❲✐❝❦❤❛♠✿ ❇✐♥✲s✉♠♠❛r✐s❡✲s♠♦♦t❤✿ ❛ ❢r❛♠❡✇♦r❦ ❢♦r ✈✐s✉❛❧✐s✐♥❣ ❧❛r❣❡ ❞❛t❛ ❇✐❣✈✐s ✐s ❛ s❝❤❡♠❡ ❢♦r ♣r❡✲♣r♦❝❡ss✐♥❣ ❜✐❣ ❞❛t❛s❡ts ♦✉t♣✉t ❝❛♥ t❤❡♥ ❜❡ ❤❛♥❞❧❡❞ ❜② ❝♦♥✈❡♥t✐♦♥❛❧ ✭ ❘ ✮ ♣❧♦t t♦♦❧s ♣r♦❝❡ss✐♥❣ ❞♦♥❡ ✐♥ ✭❢❛st✮ ❝♦♠♣✐❧❡❞ ❈✰✰ ❝♦❞❡✱ ✉s✐♥❣ ❘❝♣♣ ♣❛❝❦❛❣❡ ❜✐❣✈✐s ❣♦❛❧✿ ❜❡ ❛❜❧❡ t♦ ♣❧♦t ✶✵✵ ♠✐❧❧✐♦♥ ♣♦✐♥ts ✐♥ ✉♥❞❡r ✺ s❡❝♦♥❞s ❆❧s♦ ♣r♦✈✐❞❡s ♦✉t❧✐❡r r❡♠♦✈❛❧ ❛♥❞ s♠♦♦t❤✐♥❣✿ ❜✐❣ ❞❛t❛ ♠❡❛♥s ✈❡r② r❛r❡ ❝❛s❡s ❝❛♥ ♦❝❝✉r ⇒ ♦✉t❧✐❡rs ♠❛② ❜❡ ♠♦r❡ ♦❢ ❛ ♣r♦❜❧❡♠ s♠♦♦t❤✐♥❣ ✈❡r② ✐♠♣♦rt❛♥t t♦ ❤✐❣❤❧✐❣❤t tr❡♥❞s ✫ s✉♣♣r❡ss ♥♦✐s❡

■♥tr♦❞✉❝t✐♦♥ ❇✐❣✈✐s ♦✈❡r✈✐❡✇ ❇✐❣✈✐s ❞❡♠♦ ■♥st❛❧❧✐♥❣ ❜✐❣✈✐s Pr♦❥❡❝t ✇❡❜s✐t❡✿ ❣✐t❤✉❜✳❝♦♠✴❤❛❞❧❡②✴❜✐❣✈✐s ✐♥st❛❧❧✳♣❛❝❦❛❣❡s✭✧❞❡✈t♦♦❧s✧✮ ❧✐❜r❛r②✭❞❡✈t♦♦❧s✮ ✐♥st❛❧❧❴❣✐t❤✉❜✭✧❜✐❣✈✐s✧✮ ❘❡❝❡♥t ❜❧♦❣ ❛rt✐❝❧❡ ❛❜♦✉t ❜✐❣✈✐s ✿ ❜❧♦❣✳r❡✈♦❧✉t✐♦♥❛♥❛❧②t✐❝s✳❝♦♠✴✷✵✶✸✴✵✹✴✈✐s✉❛❧✐③❡✲❧❛r❣❡✲❞❛t❛✲s❡ts✲✇✐t❤✲t❤❡✲❜✐❣✈✐s✲♣❛❝❦❛❣❡✳❤t♠❧

■♥tr♦❞✉❝t✐♦♥ ❇✐❣✈✐s ♦✈❡r✈✐❡✇ ❇✐❣✈✐s ❞❡♠♦ ❜✐❣✈✐s ❛♣♣❧✐❡❞ t♦ ❛ s♠❛❧❧ ❞❛t❛s❡t ❧✐❜r❛r②✭❜✐❣✈✐s✮❀ ❧✐❜r❛r②✭❣❣♣❧♦t✷✮ ★ ❧♦❛❞ ♣❛❝❦❛❣❡s ❜✐♥❉❛t❛ ❁✲ ✇✐t❤✭❛✐rq✉❛❧✐t②✱ ❝♦♥❞❡♥s❡✭❜✐♥✭❖③♦♥❡✱ ✷✵✮✱ ❜✐♥✭❚❡♠♣✱ ✺✮✮ ✮ ♣ ❁✲ ❣❣♣❧♦t✭❞❛t❛❂❜✐♥❉❛t❛✱ ❛❡s✭❚❡♠♣✱ ❖③♦♥❡✱ ❢✐❧❧❂✳❝♦✉♥t✮✮ ✰ ❣❡♦♠❴t✐❧❡✭✮ ♣ ✰ ❣❡♦♠❴♣♦✐♥t✭❞❛t❛❂❛✐rq✉❛❧✐t②✱ ❛❡s✭❢✐❧❧❂◆❯▲▲✮✱ ❝♦❧♦✉r❂✧♦r❛♥❣❡✧✮ ● 150 ● .count ● ● 12.5 ● ● ● 10.0 Ozone 100 ● ● ● ● 7.5 ● ● ● ● ● ● ● ● ● ● 5.0 ● ● ● ● ● ● ● ● ● ● ● 2.5 ● 50 ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● ● 0 ● 60 70 80 90 100 Temp

■♥tr♦❞✉❝t✐♦♥ ❇✐❣✈✐s ♦✈❡r✈✐❡✇ ❇✐❣✈✐s ❞❡♠♦ ▼♦✈✐❡ ❧❡♥❣t❤ ✈s✳ ■▼❉❇ r❛t✐♥❣✿ ❜✐❣✲✐s❤ ❞❛t❛✱ ✇✐t❤ ♦✉t❧✐❡rs✦ ∼ ✶✸✵✱✵✵✵ r♦✇ ❞❛t❛ ❢r❛♠❡ ✭ ❜✐❣✈✐s✿✿♠♦✈✐❡s ✱ ❢r♦♠ ✐♠❞❜✳❝♦♠✮ ◆❜✐♥ ❁✲ ✶❡✹ ★ ♥✉♠❜❡r ♦❢ ❜✐♥s ❜✐♥❉❛t❛ ❁✲ ✇✐t❤✭♠♦✈✐❡s✱ ❝♦♥❞❡♥s❡✭❜✐♥✭❧❡♥❣t❤✱ ❢✐♥❞❴✇✐❞t❤✭❧❡♥❣t❤✱ ◆❜✐♥✮✮✱ ❜✐♥✭r❛t✐♥❣✱ ❢✐♥❞❴✇✐❞t❤✭r❛t✐♥❣✱ ◆❜✐♥✮✮✮✮ ❣❣♣❧♦t✭❞❛t❛❂❜✐♥❉❛t❛✱ ❛❡s✭❧❡♥❣t❤✱ r❛t✐♥❣✱ ❢✐❧❧ ❂ ✳❝♦✉♥t✮✮ ✰ ❣❡♦♠❴t✐❧❡✭✮ 10.0 7.5 .count 100 75 rating 50 5.0 25 2.5 0 1000 2000 3000 4000 5000 length