MI T Modular Pebble Bed React or (MPBR) A Summary of Research Act - - PowerPoint PPT Presentation

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MI T Modular Pebble Bed React or (MPBR) A Summary of Research Act - - PowerPoint PPT Presentation

MI T Modular Pebble Bed React or (MPBR) A Summary of Research Act ivit ies and Accomplishment s Andrew C. Kadak Ronald Ballinger 2nd I nt ernat ional Topical Meet ing on High Temperat ure React or Technology Beij ing, China Sept ember 22-24,


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SLIDE 1

MI T Modular Pebble Bed React or (MPBR)

A Summary of Research Act ivit ies and Accomplishment s Andrew C. Kadak Ronald Ballinger

2nd I nt ernat ional Topical Meet ing on High Temperat ure React or Technology Beij ing, China Sept ember 22-24, 2004

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SLIDE 2

St udent s Who Have Worked on t he Proj ect

  • Heat her MacLean
  • J ing Wang
  • J ulian Lebenhaf t
  • Marc Bert e
  • Chunyun Wang
  • Tieliang Zhai
  • Tamara Galen
  • J eremy J ohnson
  • Elt on Dean
  • J ennif er Anderson
  • Paul Owen
  • Nat e Carst ens
  • Daniel Walker
  • Andreea Chisca
  • Ryan Kabir
  • Michael St awicki
  • Richard Wat kins
  • I an Parrish
  • Vict oria Anderson
  • Paige Hopewell
  • I shna Trivedi
  • Mark Laught er
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SLIDE 3
  • Dean Wang
  • J acob Eapen
  • Tanya Burka
  • Lars Gronning
  • Nicholas Hernandez
  • Mat hew Aichele
  • J aehyuk Choi
  • Rhet t Creight on
  • Dandong Feng
  • Cat herine Gof f
  • J ef f Hung
  • William Kennedy
  • Ashley Finan
  • Scot t Mahar
  • Marina Savkina
  • Timot hy Alvey
  • Chang W. Kang
  • Allan Smit h
  • Mark Wright
  • Frank Yao
  • J amie Warburt on

Facult y:

  • David Gordon Wilson (ME)
  • Sidney Yip
  • Michael Driscoll
  • Richard Lanza
  • Mart in Bazant (Mat h)
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SLIDE 4
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SLIDE 5
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SLIDE 6
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SLIDE 7

Our Vision f or 1150 MW Combined Heat and Power Station

Turbine Hall Boundary

Admin Training Control Bldg. Maintenance Parts / Tools

10 9 8 7 6 4 2 5 3 1

0 20 40 60 80 100 120 140 160 20 40 60 80 100

Primary island with reactor and IHX Turbomachinery

Ten-Unit VHTR Plant Layout (Top View)

(distances in meters)

Equip Access Hatch Equip Access Hatch Equip Access Hatch

Oil Refinery Hydrogen Production

Desalinization Plant VHTR Characteristics

  • Temperatures > 900 C
  • Indirect Cycle
  • Core Options Available
  • Waste Minimization
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SLIDE 8

MI T’s Pebble Bed Proj ect

  • Developed

I ndependent ly

  • I ndirect Gas Cycle
  • Real Modularit y
  • High Aut omat ion
  • License by Test
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SLIDE 9

Project Overview

  • Fuel Performance
  • Fission Product Barrier

(silver migration)

  • Core Physics
  • Safety

Loss of Coolant Air Ingress

  • Balance of Plant Design
  • Modularity Design
  • Intermediate Heat

Exchanger Design

  • Core Power Distribution

Monitoring

  • Pebble Flow Experiments
  • Non-Proliferation
  • Safeguards
  • Waste Disposal
  • Reactor Research/

Demonstration Facility

  • License by Test
  • Expert I&C System -

Hands free operation

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SLIDE 10

MI T MPBR Specif icat ions

Thermal Power 250 MW - 120 Mwe Target Thermal Ef f iciency 45 % Core Height

  • 10. 0 m

Core Diameter

  • 3. 5 m

Pressure Vessel Height 16 m Pressure Vessel Radius

  • 5. 6 m

Number of Fuel Pebbles 360, 000 Microspheres/ Fuel Pebble 11, 000 Fuel UO2 Fuel Pebble Diameter 60 mm Fuel Pebble enrichment 8% Uranium Mass/ Fuel Pebble 7 g Coolant Helium Helium mass f low rate 120 kg/ s (100% power) Helium entry/ exit temperatures 520oC/ 900oC Helium pressure 80 bar Mean Power Density

  • 3. 54 MW/ m3

Number of Control Rods 6

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SLIDE 11

Features of Current Design

Three-shaft Arrangement Power conversion unit 2.96 Cycle pressure ratio 900°C/520°C Core Outlet/Inlet T 126.7 kg/s Helium Mass flowrate 48.1% (Not take into account cooling IHX and HPT. if considering, it is believed > 45%) Plant Net Efficiency 120.3 MW Net Electrical Power 132.5 MW Gross Electrical Power 250 MW Thermal Power

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SLIDE 12

Current Design Schematic

Generator

522.5°C 7.89MPa 125.4kg/s

Reactor core

900°C 7.73MPa 800°C 7.75MPa 511.0°C 2.75MPa 96.1°C 2.73MPa 69.7°C 8.0MPa 509.2°C 7.59MPa 350°C 7.90MPa 326°C 105.7kg/s 115 °C 1.3kg/s 69.7°C 1.3kg/s 280 °C 520°C 126.7kg/s HPT 52.8MW

Precooler Inventory control Intercooler Bypass Valve Circulator IHX Recuperator

LPT 52.8MW PT 136.9MW 799.2 C 6.44 MPa 719.°C 5.21MPa MPC2 26.1 MW MPC1 26.1MW LPC 26.1 MW HPC 26.1MW 30 C 2.71MPa 69.7 C 4.67MPa

Cooling RPV

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SLIDE 13

BOP System Analysis and Dynamic Simulation Model Development

Student: Chunyun Wang Advisor: Prof. Ronald G. Ballinger

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SLIDE 14

Objectives

  • Develop an advanced design for a pebble bed

reactor power plant system with high efficiency and minimum capital cost – Net efficiency > 45% – Must be achievable with current technology or minimal extension of technology

  • Develop a dynamic simulation model to determine

the control structure, investigate the control schemes and simulate the transients

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SLIDE 15

Model Development

T/H Steady State & Dynamic Model Development

Steady State Model Dynamic Model T,P distribution Fission power, components’ overall performance Optimum cycle pressure ratio, plant net efficiency Component physical parameters, control scheme Load transient simulation

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SLIDE 16

Design Constraints

  • Compliance with ASME code

– Section III, Class 1 Pressure Boundary (Nuclear side) – Section VIII (where applicable)

  • Build with achievable extension of

Technology

  • Using “ESKOM-Like” reactor as heat source
  • Components must be commercially feasible
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SLIDE 17

Consequences of Indirect Cycle

  • Advantages

– Section VIII used for BOP (Exclusive IHX) – Non-radioactive maintenance – Air/Water ingress to primary less likely – Less of a “loose parts” problem

  • Disadvantages

– Efficiency penalty – System complexity – IHX “operating curve” required – Vessel cooling system – Primary system volume control

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SLIDE 18

IHX & Recuperator Design Data (Printed Circuit HX configuration)—By Concepts- NREC

IHX Recuperator Effectiveness(%) 90 92.5 95 95 95 95 Hot side pres. loss(%) 1.60 1.68 1.77 0.8 1.4 2.0 Cold side pres. Loss(%) 2.00 2.00 2.00 0.13 0.23 0.33 Number of Modules 6 6 6 30 30 30 Module Width (mm) 600 600 600 600 600 600 Module Length(mm) 885 1013 1255 648 694 727 Module Height (mm) 2773 3014 3454 2745 2042 1693

  • Est. Weight (kg)

38,854 50,669 76,233 155,585 126,260 110,821 Cost (million $) 4.53 5.91 8.88 2.59 2.10 1.84

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SLIDE 19

Dynamic Model Development

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SLIDE 20

Dynamic Model Structure

Component Model Component Model

Heat Exchanger Valve Turbo Machines Gas merge & splitting Generator Control Loops Pipe PCU cycle & Inventory vessel Algorithm (Solving P) Algorithm (Solving P) Reactor Core ACSL ACSL

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SLIDE 21

Component Models

  • Reactor core

– Thermal-hydraulic model: two-dimensional – Core neutronics: Point kinetics equations – Fission product poisoning – Temperature coefficient of reactivity (Doppler effect)

  • Heat Exchanger

– Lumped parameter modeling approach (Has been verified with the HX model of Flownet)

  • Turbomachines

– Use normalized non-dimensional characteristic maps of turbine and compressor (By combination of the nondimentional parameters, the Correct mass flowrate Wc, Correct speed Nc, the axial turbine map collapses into one line for different speed line)

  • PI controller algorithm
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SLIDE 22

Control Methods and Control Objective

  • “Primary” system:

– Control rod position: Combined with the negative temperature coefficient of reactivity to control the reactivity and core outlet temperature – Circulator rotational speed: Adjusting the coolant mass flow rate in the “primary” loop allows the mass flow rates

  • f two loops are identical
  • “Secondary” system

– (1) Bypass valve: For rapid load decreases (2) Inventory control: For less rapid load reductions and load increases To maintain the power turbine’s shaft speed constant

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SLIDE 23

Control Scheme

  • 100% power (Normal Steady State)

– Full primary and secondary mass flowrate

  • 100% --> 50% ramp

– Fast response: Bypass control – Slow response: Inventory control – Inventory in the secondary system is decreased

  • gradually. After reaching new steady state, bypass

valve is closed or “feathered”.

  • 50% --> 100% ramp

– Inventory control

  • 50% <--> 0% ramp

– Bypass control (Automatic or manual)

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SLIDE 24

10% Load Step Reduction—Bypass valve mass flowrate

0.5 1 1.5 2 2.5 3 3.5 4 20 40 60 80 100 Time (sec) Mass flowrate(kg/s) Bypass Valve

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SLIDE 25

Summary

  • Analyses of balance of plant have been performed for cycle
  • ptimization
  • Plant cycle design has been defined and the MBPR net

efficiency can reach 45% with achievable technology

  • A dynamic model has been developed for plant dynamic

simulation and HX sub-model has been verified

  • The preliminary control scheme has been designed
  • 10% load rejection, both for centrifugal compressors and axial

compressors, has been simulated, and its results agree, in general, with the results of a model for a similar system developed using FlowNet

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SLIDE 26

MPBR Modularity

Marc V Berte

  • Prof. Andrew Kadak
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SLIDE 27

Modularity Progression

  • Conventional Nuclear Power Systems
  • Assembled on site
  • Component-level transportation
  • Extensive Site Preparation
  • Advanced Systems
  • Mass Produced / “Off the Shelf” Designs
  • Construction / Assembly Still Primarily on Site
  • MPBR
  • Mass Produced Components
  • Remote Assembly / Simple Transportation &

Construction

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SLIDE 28

MPBR Modularity Plan

  • Road- Truck / Standard-Rail Transportable

– 8 x 10 x 60 ft. 100,000 kg Limits

  • Bolt-together Assembly

– Minimum labor / time on site required – Minimum assembly tools – Goal: Zero Welding

  • Minimum Site Preparation

– BOP Facilities designed as “Plug-and-Play” Modules – Single Level Foundation – System Enclosure integrated into modules

  • ASME Code compliant

– Thermal expansion limitations – Code material limitations

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SLIDE 29

Space Frame Technology f or Shipment and Assembly

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SLIDE 30

Current MI T/ I NEEL Design Layout

Reactor Vessel Intermediate Heat Exchangers Turbo-generator Recuperators High Pressure Turbine and Compressor Low Pressure Turbine and Compressor Precooler

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SLIDE 31

Reactor Vessel IHX Vessel High Pressure Turbine Low Pressure Turbine Compressor (4) Power Turbine Recuperator Vessel

Present Layout

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SLIDE 32

Plant With Space Frames

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SLIDE 33
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SLIDE 34

For 1150 MW Electric Power Station

Turbine Hall Boundary

Admin Training Control Bldg. Maintenance Parts / Tools

10 9 8 7 6 4 2 5 3 1

0 20 40 60 80 100 120 140 160 20 40 60 80 100

Primary island with reactor and IHX Turbomachinery

Ten-Unit MPBR Plant Layout (Top View)

(distances in meters)

Equip Access Hatch Equip Access Hatch Equip Access Hatch

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SLIDE 35

AP1000 Footprint Vs. MPBR-1GW

~400 ft. ~200 ft.

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SLIDE 36

Intermediate Heat Exchanger Design

  • Prof. R. Ballinger, P. Stahle

Jim Kesseli - Brayton Energy

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SLIDE 37

Heat Exchanger Design

  • Two Concepts Identified

Compact Plate-Fin (NREC) PCHE Design (Heatric)

  • Base Designs Established
  • Model Developed for System Analysis
  • Limitations Identified
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SLIDE 38

Compact Plate-Fin

Old Design (NREC)

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SLIDE 39

Printed Circuit Design (Heatric)

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SLIDE 40

IHX Primary Conditions

  • Inlet

– Temperature 900oC – Pressure 7.73 Mpa

  • Outlet

– Temperature 509oC – Pressure 7.49 Mpa

  • Flow

~130 Kg/s

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SLIDE 41

IHX Secondary Conditions

  • Inlet

– Temperature 488oC – Pressure 7.99 Mpa

  • Outlet

– Temperature 879oC – Pressure 7.83 Mpa

  • Flow

~130 Kg/s

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SLIDE 42

IHX Modular Assembly Isometric View

  • Six units per assy.
  • Interconnection piping

between units

  • Pipe loops relieve

expansion stress

  • Small units for ease of

fabrication and maintenance.

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SLIDE 43

IHX Design Data (Concepts-NREC)

Effectiveness (%) 90 92.5 95 Hot Side Pres. Loss (%) 1.60 1.68 1.77 Cold Side Pres. Loss (%) 2.00 2.00 2.00 Number of Modules 6 6 6 Module Width (mm) 600 600 600 Module Length (mm) 885 1013 1255 Module Height (mm) 2773 3014 3454

  • Est. Wt. PC Config. (kg)

38,854 50,669 76,233

  • Est. Wt. PF Config. (kg)

10,335 13,478 20,278 Cost (M$) 4.53 5.91 8.88

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SLIDE 44

Heat Exchanger Core Modules

  • Printed Circuit 92%

– Wt 111,700 lb. – Ht Same as PF – Wd Same as PF – Dp Same as PF

  • 18 Req’d for IHX
  • Plate Fin 92% Eff

– Wt 30,000 lb. – Ht 118” – Wd 24” – Dp 40”

  • 18 Req’d for IHX
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SLIDE 45

IHX Unit Pressure Vessel

  • Dia.

90.5”

  • Thk.

2”

  • Ht.

240”

  • Wt.

90,000 lb

– (inc. Plate Fin xch.)

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SLIDE 46

Cooled Internal Volume

  • Temp.

288oC

  • Press.

~8 Mpa

  • ASME Sec III Bndry
  • Piping grouped by

temperature

  • Internal legs for

flexibility

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SLIDE 47

Primary Internals

  • (3) Plate Fin Core

Modules

  • Core Modules

Suspended to accommodate expansion

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SLIDE 48

Plate Fin Grouping

  • Primary Inlet
  • Primary Outlet
  • Secondary Inlet
  • Secondary Outlet
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SLIDE 49

Future Plans

  • Join with industrial partner(s) to develop

highest temperature IHX (900-950 C) possible using current material knowledge for Hydrogen demonstration plant.

  • Identify key design issues for higher

temperatures including transients.

  • Work on materials challenges for higher

temperature operation.

  • Modular approach allows for testing.
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SLIDE 50

Proposed Test Program

f or Advanced High Temperat ure Plat e Fin HX (800 - 1000 C)

Figure 6 Unit Cell Pressure Fatigue Test at Elevated Temperature. This test conducts numerous pressure cycles on three cells at elevated temperature (800 and 1000 C). At each selected pressure, the cycling will continue to failure (ie gas leakage is out
  • f spec). The test will be performed at
three to five pressures of increasing
  • magnitude. The data will be formulated
into an endurance plot. The results will be used to calibrate and validate the analytical models. The MIT high- temperature furnace is capable of heating three or more cells to 1000 C. Figure 7 Unit cell Creep Test and Elevated Temperatures. This test will use a modified version of the rig MIT high temp furnace. The tests are performed at steady pressure and temperature conditions. An empirical Larsen-Miller map of the cell is created by operating the cell to failure at two elevated temperatures, 800 and 1000 C. The pressures imposed on the cell will be selected to induce failure at intervals ranging from one hour to 1000 hours. Failure is indicated by the cells inability to maintain the leak specification. After completing the mapping, three cells will be subjected to the design pressure and temperature and left to operate
  • indefinitely. Inspection will be made at
regular intervals. Figure 8 Thermal Strain Measurement for model Validation. This test rig will heat a sub-core (5 or more cells) to an elevated temperature, but not so high as to compromise the accuracy of piezoresistive strain gauges. Transient temperature and strain measurements will be recorded while flowing very cold gas generated from a liquid nitrogen bath on one side and combustion products from a commercial burner on the other side. Proof of manufacturability, demonstration of mechanical integrity, and validation of analytical life prediction models are critical steps towards the qualification of the proposed high temperature heat exchanger. This program will address a these three steps by fabricating and instrument roughly 30 IHX cells for a series of rigorous endurance tests and characterizing.

MI T/ Brayt on Energy

  • 1. Unit Cell Pressure Fatigue Test
  • 2. Unit cell Creep Test
  • 3. Thermal Strain Measurement

for model Validation.

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SLIDE 51

Hydrogen Mission Modularity Flexibility

Hydrogen Plant A

Secondary IHX - Helium to Molten Salt?

Hydrogen Plant B May use one or more IHX’s from base electric plant for H2

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SLIDE 52

An Integrated Fuel Performance Model for Modular Pebble Bed Reactor

Jing Wang Professor R. G. Ballinger

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SLIDE 53

Fuel Performance Model

  • Detailed modeling of fuel kernel
  • Microsphere
  • Monte Carlo Sampling of Properties
  • Use of Real Reactor Power Histories
  • Fracture Mechanics Based
  • Considers Creep, stress, strains, fission

product gases, irradiation and temperature dependent properties.

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SLIDE 54

Fuel Performance

The Key Safety System

  • Develop Fuel Performance Model
  • Develop an optimized design for reliability
  • Work with manufacturer to optimize
  • Make fuel and test
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SLIDE 55

Integrated Fuel Performance Model

Power Distribution in the Reactor Core Sample a pebble/fuel particle Randomly re-circulate the pebble Get power density, neutron flux

t=t+∆t

T distribution in the pebble and TRISO Accumulate fast neutron fluence FG release (Kr,Xe) PyC swelling Mechanical model Failure model Mechanical Chemical Stresses FP distribution Strength Pd & Ag

Failed In reactor core

Y

10 times 1,000,000 times MC Outer Loop MC inner loop

N N Y

Monte Carlo outer loop: Samples fuel particle statistical characteristics MC inner loop: Implements refueling scheme in reactor core

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SLIDE 56

Simulation of Refueling - cont’d

0.0E+00 2.0E+06 4.0E+06 6.0E+06 8.0E+06 1.0E+07 1.2E+07 1.4E+07 1.6E+07 100 200 300 400 500 600 700 800

Irradiation time (days) Power density (W/m^3)

A typical power history of a pebble in MPBR core

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SLIDE 57

Simulations

Fuel Type Kernel Density (g/cm3) Kernel Diameter (µm) Buffer Thickness (µm) IPyC Thickness (µm) SiC Thickness (µm) OPyC Thickness (µm) NPR

UCO 10.70 195 100 53 35 43

HTTR

UO2 10.96 600 60 30 25 45

NPR — New Production Reactor (USA) HTTR — High Temperature Test Reactor (Japan)

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SLIDE 58

Circumferential Stresses in NPR & HTTR Type Fuel

  • 800
  • 600
  • 400
  • 200

200 400 0.2 0.4 0.6 0.8 1 1.2 1.4 1.6 1.8 2

Fast Neutron Fluence (10^21nvt) Stress (MPa) IPyC_NPR SiC_NPR OPyC_NPR IPyC_HTTR SiC_HTTR OPyC_HTTR

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SLIDE 59

NPR & HTTR Type Fuel Reliability in MPBR Environments

0.1017% 13.30%

SiC Failure Probability

16.22% 17.07%

OPyC Failure Probability

0.1017% 5.660% 1,000,000 HTTR type fuel 13.30% 27.79% 1,000,000 NPR type fuel

Particle Failure Probability IPyC Failure Probability Cases Sampled

All particle failures observed were induced by IPyC cracking

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SLIDE 60

Fuel Design Parameters

  • 6
  • 6

SiC Weibull Modulus 530.7 3300 530.7 3300 SiC Fracture Toughness (MPa.µm1/2)

  • 9
  • 9

SiC Characteristic Strength (MPa.m3/Modulus) 1.7 36 4 35 SiC Thickness (µm) 2.2 40 10 40 OPyC Thickness (µm)

  • 9.5
  • 9.5

OPyC Weibull Modulus

  • 24
  • 24

OPyC Characteristic Strength (MPa.m3/Modulus)

  • 1.9
  • 1.9

OPyC Density (g/cm3) 0.00543 1.05788 0.00543 1.05788 OPyC Initial BAF 4 41 10 40 IPyC Thickness (µm)

  • 9.5
  • 9.5

IPyC Weibull Modulus

  • 24
  • 24

IPyC Characteristic Strength (MPa.m3/Modulus)

  • 1.9
  • 1.9

IPyC Density (g/cm3) 0.00543 1.05788 0.00543 1.05788 IPyC Initial BAF 10.3 94 18 90 Buffer Thickness (µm)

  • 2.25
  • 2.25

Buffer Theoretical Density (g/cm3) 0.05 1.05 0.05 1.05 Buffer Density (g/cm3) 14.1 497 20 500 Kernel Diameter (µm)

  • 10.95
  • 10.95

Kernel Theoretical Density (gm/cm3) 0.01 10.4 0.01 10.4 Kernel Density (gm/cm3) 0.1 96 0.1 96 Uranium Enrichment (%) Uncertainty As-Fabricated Value Uncertainty Design Value Parameter

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SLIDE 61

Fuel Performance Model Development Path

Steady State Transient & Accident

Initial Steady State Model

  • Initial Probabilistic Fracture Mechanics Model
  • Simple Chemistry Model

Advanced Steady State Model

  • Advanced Fracture Mechanics Model
  • Ag Migration & Release Model

Complete Steady State Model

  • Detailed Chemical Model
  • Detailed Layer Degradation Model

Initial Transient & Accident Model Complete Transient & Accident Model

Current Development Status

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SLIDE 62

Conclusions

  • A fuel performance model has been developed

which can simulate fuel behavior in Pebble Bed Reactor cores

  • Monte Carlo simulations can be performed to

account for particle-to-particle variability in fabrication parameters as well as variability in fueling during operation

  • Results have been compared with other models

and with actual fuel performance.

  • Model can be used to optimize fuel particle design
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SLIDE 63

Silver Transport in Silicon Carbide for High-Temperature Gas Reactors

Heather J. MacLean Professor Ronald Ballinger

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SLIDE 64

Barrier Integrity

  • Silver Diffusion observed in tests @ temps
  • Experiments Proceeding with Clear

Objective - Understand phenomenon

  • Focus on Grain SiC Structure Effect
slide-65
SLIDE 65

Silver Ion Implantation

SiC masks on sample frame Light transmission through SiC mask and sample

  • 161 MeV silver beam, peak at 13 µm
  • 93 MeV silver beam, peak at 9 µm
  • implanted ~1017 ions = ~2 atomic % silver
  • measure silver concentration profiles
  • examine SiC damage
slide-66
SLIDE 66

Ion Implantation Silver Depth Profile

0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4 1.6 1.8 2.0 2 4 6 8 10 12 14 16 18 Depth (µm) Atomic Concentration (%) Ag as implanted Ag after 210 hr heat

Sample 2b

2a 2b

No silver movement No silver movement after 210 hr at 1500 after 210 hr at 1500° °C C

Predicted Profile

slide-67
SLIDE 67

Spherical Diffusion Couple Experiments

RESULTS

  • No silver in SiC depth profiles
  • Mass loss after heating
  • Leak rates increased after heating

Diffusion couple (cross-section) CVD SiC coating graphite or SiC shell silver

  • ptical microscopy from top of graphite-SiC

diffusion couple

slide-68
SLIDE 68

Calculated Silver Diffusion (from release)

1.E-19 1.E-18 1.E-17 1.E-16 1.E-15 1.E-14 1.E-13 1.E-12 1.E-11 1.E-10 3.5 4.0 4.5 5.0 5.5 6.0 6.5 7.0 7.5 8.0 8.5

104/T (K) Release Coefficient (m2/s)

Selected Literature Data Amian & Stover calculated fit 1000oC 1200oC 1600oC D calculated from silver release (literature) Nabielek et al. ion implantation limit

low silver concentration ~2 ppm high silver concentration (unit activity) Mass Transfer Coefficients (m2/s)

Release coefficients calculated from silver release (current experiments) 100 ppm boundary condition

R e le a s e c o e ffic ie n ts c a lc u la te d fr o m s ilv e r r e le a s e ( c u r r e n t e x p e r im e n ts )

2 ppm boundary condition

slide-69
SLIDE 69

Silver Mass Loss

0.2 0.4 0.6 0.8 1 1.2 1000 1200 1400 1600 1800 Heating Temperature (oC) Fractional Silver Loss 0.2 0.4 0.6 0.8 1 1.2 1000 1200 1400 1600 1800 Heating Temperature (oC) Fractional Silver Loss 0.2 0.4 0.6 0.8 1 1.2 1000 1200 1400 1600 1800 Heating Temperature (oC) Fractional Silver Loss

SiC-1

graphite shell, standard SiC coating

SiC-2

graphite shell, modified SiC coating

SiC-3

SiC shell, standard SiC coating (normalized to seam area)

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SLIDE 70

Possible Nano-Cracking

  • Nanometer-sized features (cracks) observed in

experimental SiC coating in AFM (atomic force microscopy)

  • Mechanical pathway
  • Origin not yet known
  • Stresses from differential thermal expansion

between individual SiC grains may cause nano- scale cracks

  • May be aggravated by thermal cycling
  • Consistent with fuel performance discussions at

ORNL

slide-71
SLIDE 71

Conclusions

  • Silver does not diffuse through intact, fine-grained SiC

– no change in silver concentration profiles – no silver movement despite increased grain boundary area

  • Vapor migration governs silver release from CVD SiC

coatings – mass release observed, but silver profiles not found – increased leak rates indicate mechanical cracks

  • Transport model will compare proposed mechanisms with

literature data

  • Continued SiC development needs to focus on identifying

and eliminating crack path

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SLIDE 72

Core Physics

  • Basic tool Very Special Old Programs (VSOP)
  • Developing MNCP Modeling Process
  • Tested Against HTR-10 Benchmark
  • Tested Against ASTRA Tests with South

African Fuel and Annular Core

slide-73
SLIDE 73

MIT Nuclear Engineering Departm ent

Modeling Considerations

Packing of Spheres

Spheres dropped into a

cylinder pack randomly

Packing fraction ~ 0.61 Repeated-geometry feature

in MCNP4B requires use of a regular lattice

SC, BCC, FCC or HCP? BCC/BCT works well for

loose sphere packing

Random Close Packed Body Centered Cubic

5

slide-74
SLIDE 74

MIT Nuclear Engineering Departm ent

HTR-10 MCNP4B Model

12 Reactor TRISO fuel particle Core Fuel sphere Core lattice

slide-75
SLIDE 75

MIT Nuclear Engineering Departm ent

MCNP4B/VSOP Model Output

Top of core top

161 242 402 483 644 725 108 134 175 1 2 3 4 5 6 7 8 MW/m 3 Axial Position (cm) Radial Position (cm)

Power Density in PBMR Equilibrium Core

Control Rods 1/4 Inserted (z = 201.25 cm)

7.00E+00-8.00E+00 6.00E+00-7.00E+00 5.00E+00-6.00E+00 4.00E+00-5.00E+00 3.00E+00-4.00E+00 2.00E+00-3.00E+00 1.00E+00-2.00E+00 0.00E+00-1.00E+00

Power density in annular core regions

25

slide-76
SLIDE 76

MIT Nuclear Engineering Departm ent ASTRA Critical Experiments

Side reflector Central h l Core Mixing zone Internal reflector Experimental channels

CR - Control d MR1 - Manual control d SR - Safety d E1-E6 - Experimental chambers h l 1-9 - Experimental channels for d t t PIR,ZPT,ZII,ZRTA - Ionization chambers and neutron t Neutron source channel

SR2 SR3 CR5 SR7 E5 SPU2 PIR PIR E6 ZII2 ZRTA4 E1 SPU3 E2 ZIIЗ ZRTA1 E3 E4 ZII1 SPU1 ZRTA2 ZPT2 ZII1 ZRTA3 CR4 SR6 MR1 SR5 CR3 SR4 SR8 CR2 SR1 CR1

a b c d e f g h j k l m n i

  • 15

14 13 12 11 10 9 8 7 6 5 4 3 2 1

A

B

Kurchatov Institute, Moscow Mockup of PBMR annular core

Inner reflector: graphite spheres (M)

10.5 cm ID 72.5 cm OD Mixed zone: 50/47.5/2.5 (M/F/A) 105.5 cm OD Fuel zone: 95/5 (F/A) 181 cm OD (equiv.) Core height: 268.9 cm

packing fraction = 0.64 2.44 g U/FS, 21% U235, 0.1 g B/AS 5 CRs, 8 SRs, 1 MR CR = 15 s/s tubes with B4C powder 6 in-core experimental tubes

13

slide-77
SLIDE 77

ASTRA Conclusions

  • Criticality Predictions fairly close (keff = .99977)
  • Rod Worth Predictions off 10%
  • Analysis Raises Issues of Coupling of Core
slide-78
SLIDE 78

MIT Nuclear Engineering Department

HTR-10 (Beijing)

10 MW Pebble Bed Reactor:

Graphite reflector Core: Rc = 90 cm, H ≤ 197 cm TRISO fuel with 5 g U/Fuel Sphere 17% U235 F/M sphere ratio = 57:43, modeled

by reducing moderator sphere size

Initial criticality December 2000

1.00081± 0.00086 K-eff 128.5 cm Critical Height 16,890 Actual Loading 16,830 Calculated Loading

MCNP4B Results 9

slide-79
SLIDE 79

Safety

Tieliang Zhai

  • Prof. Hee Cheon No (Korea)

Professor Andrew Kadak

slide-80
SLIDE 80

Safety Issues

  • Loss of Coolant Accident
  • Air Ingress
  • Reactor Cavity Heat Removal
slide-81
SLIDE 81

Safety

  • LOCA Analysis Complete - No Meltdown
  • Air Ingress to study fundamental processes

and benchmark Computational Fluid Dynamics Codes

  • Conservative analysis show no “flame”
  • Address Chimney effect
  • Address Safety of Fuel < 1600 C
  • Use Fluent for detailed modeling of RV
slide-82
SLIDE 82

Massachusetts Institute of Technology Department of Nuclear Engineering

Advanced Reactor Technology Pebble Bed Project

MPBR-5

slide-83
SLIDE 83

Temperat ure Prof ile

Fig-10: The Temperature Profile in the 73rd Day

200 400 600 800 1000 1200 1400 1600 1 2 3 4 5 6 7 8 9 10 11 Distance to the Central Line Temperature (C)

Vessel Core Reflector Cavity Soil Concrete Wall

slide-84
SLIDE 84

The Prediction of the Air Velocity (By Dr. H. C. No)

Fig-14: Trends of maximum temperature for 0, 2, 4, 6 m/s of air velocity in the air gap region

200 400 600 800 1000 1200 1400 1600 1800 30 60 90 120 150 180 210 Time (hr) Temperature (C)

Hot-Point Temperature of the core(0m/s) Hot-Point Temperature of the Vessel (0m/s) Hot-Point Temperature of the Concrete Wall (0m/s) Hot-Point Temperature of the Core (2m/s) Hot-Point Temperature of the Vessel (2m/s) Hot-Point Temperature of the Concrete Wall (2m/s) Hot-Point Temperature of the Core (6m/s) Hot-Point Temperature of the Vessel (6m/s) Hot-Point Temperature of the Concrete Wall (6m/s) Limiting Temperature for the Vessel Limiting Temperature for the Containment

slide-85
SLIDE 85

Air Ingress

Vary Choke Flow

Bottom Reflector Air In Air/COx out

  • Most severe accidents

among PBMR’s conceivable accidents with a low

  • ccurrence

frequency.

  • Challenges: Complex

geometry, Natural Convection, Diffusion, Chemical Reactions

slide-86
SLIDE 86

Air Ingress Velocity f(temperature)

Fig-2: Air Inlet Velocity Vs. the Average Temp. of the Gases

0.01 0.02 0.03 0.04 0.05 0.06 0.07 0.08 0.09 400 800 1200 1600 2000 2400 2800 3200 the Average Temp. of the Gases (C) Air Inlet Velocity (m/s)

slide-87
SLIDE 87

Preliminary Conclusions Air Ingress

For an open cylinder of pebbles:

  • Due to the very high resistance through the pebble

bed, the inlet air velocity will not exceed 0.08 m/s.

  • The negative feedback: the Air inlet velocity is not

always increase when the core is heated up. It reaches its peak value at 300 °C.

  • Preliminary combined chemical and chimney

effect analysis completed - peak temperatures about 1670 C.

slide-88
SLIDE 88

Simplified HEATING7 Open Cylinder Analysis Peak Temperature

Figure 3: The peak temperature

800 900 1000 1100 1200 1300 1400 1500 1600 1700 50 100 150 200 250 300 350 400 time(hr) Temperature (C)

slide-89
SLIDE 89

Analysis Results

300 600 900 1200 1500 1800 400 800 1200 1600 2000 Time (hour) Hot-Point Temperatures (C) Hot-Point Temperature of the Core

Hot-Point Temperature of the Pressure Vessel

Hot-Point Temperature of the Concrete Wall

Figure 9: Hot-Point Temperatures

slide-90
SLIDE 90

Sensitivity Analysis - Emissivity

400 800 1200 1600

400 800 1200 1600 2000 Time (hr) Hot-Point Temperatures (C

Core Hot-Point Temperature (Benchmark E=0.73) Core Hot-Point Temperature(Emissivity=0.01) Core Hot-Point Temperature(Emissivity=1) Wall Hot-Point Temperature (Benchmark E=0.73) Wall Hot-Point Temperature (Emmisivity=0.01) Wall Hot-Point Temperature (Emmisivity=1)

Figure 11: Hot-Point Temperature Sensitivity to Emissivities

  • f Vessel and Concrete Wall in the LOCA Analysis
slide-91
SLIDE 91

Sensitivity Analysis-Conductivity

. 300 600 900 1200 1500 1800 300 600 900 1200 1500 1800 2100 Time (hr) Temperature (C)

Core Hot-Point Temperature When the Conductivity of the Soil and Concrete Wall is 0.54w/m.C (Benchmark Condition) Core Hot-Point Temperature When the Conductivity of the Soil and Concrete Wall is 5w/m.C Core Hot-Point Temperature When the Conductivity of the Soil and Concrete Wall is 10w/m.C" Concrete Wall Hot-Point Temperature When the Conductivity of the Soil and Concrete Wall is 0.54w/m.C (Benchmark Condition) Concrete Wall Hot-Point Temperature When the Conductivity of the Soil and Concrete Wall is 5w/m.C Concrete Wall Hot-Point Temperature When the Conductivity of the Soil and Concrete Wall is 10w/m.C

Figure 12: Hot-Point Temperature Sensitivity to the Conductivity

  • f Soil and Concrete Wall in the LOCA Analysis
slide-92
SLIDE 92

Conclusions for LOCA Analysis

  • No meltdown occurs
  • The temperatures of the concrete wall and the steel

pressure vessel are above their safety limit

  • The safety objectives can not been satisfied by the

improvement of the thermal properties

  • A convective term, natural or forced, is needed to

cool the concrete wall and the pressure vessel

Explain this somewhere

slide-93
SLIDE 93

Air Ingress Analysis Computational Fluid Dynamics

  • Benchmark to Japanese Diffusion, Thermal

and Multi-Component Tests

  • Benchmark to NACOK air ingress tests
  • Use FLUENT CFD code to develop

methodology

slide-94
SLIDE 94

Experimental Apparatus - Japanese

C4 2 7

Nitrogen Helium Valves

C3 C1 C2 H4 H3 H2 H1

Figure 16: Apparatus for Isothermal and Non-Isothermal experiments Figure 17: Structured mesh

slide-95
SLIDE 95

Isothermal Experiment

0.00 0.20 0.40 0.60 0.80 50 100 150 200 250 300 Time (min) Mole fraction

H-1 & C-1(Calculation) H-2 & C2 (Calculation) H-3 & C3 (Calculation) H-4 & C4 (Calculation) H-1 & C-1(Experiment) H-2 & C2 (Experiment) H-3 & C3 (Experiment) H-4 & C4 (Experiment)

Figure 18: Mole fraction of N2 for the isothermal experiment

slide-96
SLIDE 96

Thermal Experiment

Figure 19: The contour of the temperature bound4ary condition

Pure Helium in top pipe, pure Nitrogen in the bottom tank N2 Mole fractions are monitored in 8 points

  • Hot leg heated
  • Diffusion Coefficients as a

function of temperature

slide-97
SLIDE 97

Thermal Experiment

0.2 0.4 0.6 0.8 1 50 100 150 200 Time (min) Mole fraction of N2

H-1(FLUENT) C-1(FLUENT) H-1(Experiment) C-1(Experiment)

Figure 20: Comparison of mole fraction of N2 at Positions H-1 and C-1

0.2 0.4 0.6 0.8 1 50 100 150 200 Time(min) Mole Fraction

H2(Experiment) C2(Experiment) H-2(FLUENT) C-2(FLUENT)

Figure 21: Comparison of mole fraction

  • f N2 at Positions H-2 and C-2
slide-98
SLIDE 98

Thermal Experiment (Cont.)

0.2 0.4 0.6 0.8 1

50 100 150 200 250

Time(min) Mole Fraction of N2 H4(Exp) C4(Exp) H-4(Calc) C-4(Calc)

Figure 22: Comparison of mole fraction

  • f N2 at Positions H-1 and C-1
  • 0.15
  • 0.10
  • 0.05

0.00 0.05 0.10 0.15 0.20 0.25 2 4 6 Time (Second) Velocity (m/second)

Figure 23: The vibration after the

  • pening of the valves.
slide-99
SLIDE 99

Multi-Component Experiment(Cont.)

  • Chemical Reactions

– 1 surface reaction: C + O2 = x CO + y CO2 (+ Heat) – 2 volume Reactions: 2 CO + O2 = 2CO2 ( + Heat) 2 CO2 = 2 CO + O2 (- Heat)

n

  • c

p RT E K r

2

) exp( − =

Figure 35: The temperature boundary conditions for the multi-component experiment

slide-100
SLIDE 100

Multi-Component Experiment(Cont.)

0.00 0.03 0.06 0.09 0.12 0.15 0.18 0.21 20 40 60 80 100 120 140 Time(min) Mole Fraction O2(Experiment) O2(Calculation) CO(Experiment) CO(Calculation) CO2(Experiment) CO2(Calculation) Figure 36: Mole Fraction at Point-1 (80% Diffusion Coff.)

slide-101
SLIDE 101

Multi-Component Experiment(Cont.)

Figure 37: Mole Fraction at Point-3

0.00 0.04 0.08 0.12 0.16 0.20 0.24 20 40 60 80 100 120 140 Time(min) Mole Fraction

O2(Experiment) O2(Calculation) CO(Experiment) CO(Calculation) CO2(Experiment) CO2(Calculation)

slide-102
SLIDE 102

Multi-Component Experiment(Cont.)

Figure 38: Mole Fraction at Point-4

0.00 0.05 0.10 0.15 0.20 0.25 20 40 60 80 100 120 140 Time (min) Mole Fraction O2(Experiment) O2(Calculation) CO(Experiment) CO(Calculation) CO2(Experiment) CO2(Calculation)

slide-103
SLIDE 103

NACOK Natural Convection Experiments

no cont.

Figure 39: NACOK Experiment

slide-104
SLIDE 104

Boundary Conditions

Figure 41: Temperature Profile for one experiment

slide-105
SLIDE 105

The Mass Flow Rates

Figure 42: Mass Flow Rates for the NACOK Experiment 0.0E+00 1.0E-03 2.0E-03 3.0E-03 4.0E-03 100 300 500 700 900 1100 Temperature of the Pebble Bed (C) Mass Flow Rate (kg/s 5.0E-03 )

T_R=200 DC(Exp.) T_R=400 DC(Exp.) T_R=600 DC(Exp.) T_R=800 DC(Exp.) T_R=200 DC(FLUENT) T_R=400 DC(FLUENT) T_R=600 DC(FLUENT) T_R=800 DC(FLUENT)

slide-106
SLIDE 106

Verify the Chemical Model (FLUENT 6.0)

slide-107
SLIDE 107

The Detailed Model in Progress

slide-108
SLIDE 108

Detailed Bottom Reflector

slide-109
SLIDE 109

Summary

  • Air Ingress is a potentially serious event for high

temperature graphite reflected and moderated reactors (prismatic and pebble).

  • Realistic analyses are necessary to understand actual

behavior

  • Based on realistic analyses, mitigation strategies are

required.

  • Good news is that long time frames are involved at allow

for corrective actions (70 to 200 hours).

  • MIT working on detailed analysis of the event with

baseline modeling and testing with German Julich NACOK upcoming tests on air ingress.

slide-110
SLIDE 110

Extrinsic Safeguards Protection System for Pebble Bed Reactors

Proposed Concept

slide-111
SLIDE 111

Extrinsic Safeguards System for Pebble Bed Reactors

Waste Package Fresh Fuel Room Scrap Waste Can

Typical Waste Storage Room

slide-112
SLIDE 112

Waste Disposal Conclusions

  • Per kilowatt hour generated, the space taken in a

repository is less than spent fuel from light water reactors.

  • Number of shipments to waste disposal site 10

times higher using standard containers.

  • Graphite spent fuel waste form ideal for direct

disposal without costly overpack to prevent dissolution or corrosion.

  • Silicon Carbide may be an reffective retardant to

migration of fission products and actinides.

slide-113
SLIDE 113

Pebble Flow

  • Issue is the central graphite column and its

integrity

  • Don’t want fuel pebble in graphite or

graphite pebble in fuel

  • How to assess flow to assure high power

peaks do not occur that could lead to fuel failure

Conduct ed Experiment t o det ermine f low

slide-114
SLIDE 114

Radial Fuel Distribution Radial Fuel Distribution

  • A central core of pure

A central core of pure graphite reflector graphite reflector pebbles is surrounded pebbles is surrounded by an annulus of a by an annulus of a 50/50 fuel 50/50 fuel-

  • and

and-

  • reflector mix, and a

reflector mix, and a larger annulus of pure larger annulus of pure fuel pebbles. fuel pebbles.

slide-115
SLIDE 115

Half Model Data Collection

slide-116
SLIDE 116

Comparison to Design Profile

10 20 30 40 50 60 70 80 90 10 20 30 Width (cm) H eight (cm)

  • Velocity Profile very similar
  • Very flat until the funnel

region

30°, 4 cm exit

07.mpg 09.mpg

Movie Clips

slide-117
SLIDE 117

Trial with Central Column

slide-118
SLIDE 118

Video Demo

19.mpg 20.mpg 21.mpg 22.mpg 23.mpg
slide-119
SLIDE 119

Streamlines Confirmed by 3D Experiment

0 5 1015 20 40 60 80 100

  • 5

5 5 10 x (cm) y (cm)

slide-120
SLIDE 120

Slow Flow Results

  • Used drill to remove

pebbles at 120 /min.

  • Flow lines still linear
slide-121
SLIDE 121

Shaping Ring for Central Column Formation

Bot t om of Shaping ring

  • Shaping ring used to

form central column at top 3 inches

  • Rest open - no ring
  • Column maintained

during slow drain down.

slide-122
SLIDE 122

Core Monitoring System

Imaging of Core Tracer Ball Method

slide-123
SLIDE 123

Visually speaking… K N

Inverse Radon Transform

R I

Projection (line integrals)

Perfect Reconstruction!

Attenuation correction function

slide-124
SLIDE 124

Summary

  • Nitrogen tracer produces 10.8

MeV gamma ray

  • Gamma ray detected by detector

ring

  • Core is imaged by Tomography
slide-125
SLIDE 125

Image of Core

Core Boundary

  • Color intensity proportional to gamma

flux measured by detector

slide-126
SLIDE 126

Radial Neutron Flux (0-175cm) Profile of PBMR Core

10th slice (370 cm)

slide-127
SLIDE 127

Summary

Neutron flux is reconstructed Result of tomography

slide-128
SLIDE 128

License By Test

  • Build a research/demonstration plant
  • reactor research facility
  • Perform identified critical tests
  • If successful, certify design for

construction.

slide-129
SLIDE 129

Risk Informed Approach

  • Establish Public Health and Safety Goal
  • Demonstrate by a combination of deterministic

and probabilistic techniques that safety goal is met.

  • Using risk based techniques identify accident

scenarios, critical systems and components that need to be tested as a functional system.

slide-130
SLIDE 130

MI T’s Proj ect I nnovat ions

  • Advanced Fuels
  • Tot ally modular - build in a f act ory

and assemble at t he sit e

  • Replace component s inst ead of repair
  • I ndirect Cycle f or Hydrogen

Generat ion f or f uel cells & t ransport at ion

  • Advanced comput er aut omat ion
  • Demonst rat ion of saf et y t est s
slide-131
SLIDE 131

Future Research Activities

  • Build and Test Advanced Plate Fin IHX

Design

  • Benchmark new series of NACOK Air

Ingress Tests with CFD.

  • Perform Pebble Flow Experiments to

Reduce Central Column By-pass Flow

  • Expand Fuel Performance Model to handle

rapid transients (rod ejection)

  • Make and Test Advanced Fuel Particles

with Tsinghua University

slide-132
SLIDE 132

Summary

  • MI T Proj ect aimed at advanced pebble bed

react or development wit h f ocus on innovat ion in design, modularit y, license by t est , using a f ull scale react or research f acilit y t o explore dif f erent f uel cycles, process heat applicat ions, and advanced cont rol syst em design, helium gas t urbines and ot her component s.

  • Desire Collaborat ions t o develop int ernat ional

conf idence in t he t echnology, saf et y,economics and pract icalit y.

  • We have a unique opport unit y t o develop pebble

bed react ors but it is t ime crit ical