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Measurement of ambient neutrons in an underground laboratory at Kamioka Observatory Keita Mizukoshi Kobe University TAUP2019 at Toyama International Conference Center 9 Sep. 2019 Introduction Neutron is the one of the most serious


  1. Measurement of ambient neutrons in an underground laboratory at Kamioka Observatory Keita Mizukoshi Kobe University TAUP2019 at Toyama International Conference Center 9 Sep. 2019

  2. Introduction • Neutron is the one of the most serious backgrounds (BG) for experiments in underground. • Direct Dark matter search • Neutrino-less double beta decay search • To evaluate and shield neutron BG, 
 it is very important to evaluate ambient neutron flux • Such neutron BG has not measured systematically. • Low rate in underground i → Required high efficiency • Unknown generated points → Energy unknown • Our goal is quantitative neutron flux in the underground � 2 Keita Mizukoshi Kobe Univ.

  3. Detector (He-3 proportional counter) K. Mizukoshi et al., PTEP 123C01 3 He proportional counter • We used a 3 He proportional counter. 3 He + n → 3 H + p + 0 . 76 MeV • The energy of the exothermal reaction in the neutron capture can be obtained. ~5 k barn at thermal DAQ PC • This detector is thermal fast sensitive to thermal SUS φ 52mm neutrons (~0.025 eV), 3 He - 10 atm and cannot measure an initial neutron energy. 380mm “Setup A” � 3 Keita Mizukoshi Kobe Univ.

  4. 4 Setup for fast neutron K. Mizukoshi et al., PTEP 123C01 • To measure high energy neutron, 
 fast we used a moderator (polyethylene). thermal • Boron sheet captured thermal neutrons and reduce its effect. 3 He Thermal neutron “Setup A” ~0.025eV 160 ) 2 Counts/(neutron/cm Setup A 140 Setup B thermal 120 fast Setup B w/o B-sheet 100 80 Boron sheet 60 t5mm Polyethylene 40 3 He 20 0 510mm 9 8 6 5 3 − − − 7 − − − 4 − − 2 − 1 2 10 10 10 10 10 10 10 10 10 1 10 10 Generated neutron energy (MeV) Efficiency estimated by Geant4 “Setup B” Keita Mizukoshi Kobe Univ.

  5. noise peak Wall effect Electric 
 Counts/bins Results 100 80 60 40 3 He + n → 3 H + p + 0 . 76 MeV 20 • Full energy peak is 0.76 MeV. 
 0 0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 1 Measured energy (MeV) If 3H or p escapes, continuum region Measured spectrum in setup B will be made in a low energy (Wall Counts/bins effect). 1200 • Low energy region below 0.3 MeV is 1000 dominated by electric noise for 800 ambient neutron measurement. 600 • We counted events up to 0.85 MeV 400 200 and down to 0.5 MeV, then the number 0 of total events was estimated by a 0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 1 Measured energy (MeV) clear spectrum observed using 252Cf. Spectrum of Source ( 252 Cf) Count rate in each setup • The count rate of Setup A A B Setup (R A ) and B (R B ) involves a 1.295 ± 0.034 0.446 ± 0.018 Count rate ( × 10 -3 cps) detection of thermal and 
 14.03 19.27 Live time (day) fast neutron, respectively. K. Mizukoshi et al., PTEP 123C01 � 5 Keita Mizukoshi Kobe Univ.

  6. Simulation K. Mizukoshi et al., PTEP 123C01 Main components in each samples (wt. %) sample1 sample2 sample3 • To convert from the count rates (RA, RB) to O 40.5 37.9 35.6 ambient neutron flux, the spectral shape was Ca 28.0 24.3 29.7 required. The shape cannot measured by He-3 Si 16.6 15.6 12.0 detector thus estimated by simulation. Fe 7.6 16.6 13.5 Al 5.2 0.3 0.1 • We considered the source of the neutrons Mn 0.8 3.5 2.9 made from ( α ,n) reaction of U/Th series decay. − 6 × 10 Number of nentrons /chain decay/0.1 MeV • Neutron induced by cosmic muon is negligible. 2.2 Bin width 0.1 MeV JR-1 ( α , n) 2 JA-3 ( α , n) Sample 1 ( α , n) 1.8 Sample 1 + 3% of hydrogen • We picked three types of rocks as samples, 1.6 Sample 2 ( α , n) Sample 3 ( α , n) 1.4 238 Sample 1 ( U fission) they had much different abundance of 1.2 Sample 1 (Th series) 1 chemical compositions. 0.8 Much 
 0.6 difference! 0.4 • The difference affects much the yield of 0.2 0 0 1 2 3 4 5 6 7 neutrons. Neutron energy (MeV) Generated neutron in vary rocks JR-1 and JA-3 are geometrical reference database � 6 Keita Mizukoshi Kobe Univ.

  7. K. Mizukoshi et al., PTEP 123C01 Data driven analysis Thermalization parameter 
 obtained by measurement • We cannot investigate the all wall rock B /R 4 components in details. A Ratio of count rates R 3.5 • Especially amount of water contents in the 3 rock and chemical composition including 2.5 Hydrogen will much affect thermalization of 2 Experimental ratio Error band fast neutrons. 1.5 Sample 1 Sample 2 1 Sample 3 • Thus, thermalization in the rock was JR-1 JA-3 0.5 unknown. 0 1 2 3 4 5 6 7 • We regarded the percentage of hydrogen % of h. e. Experimental ratio v.s. parameter (%of h. e.) in simulation as a thermalization parameter. /s 2 10 2 Counts /MeV /cm 10 Sample 1 with 3% of h.e. • %of h.e. was derived by the experimental JR-1 with 1% of h.e. 1 JA-3 with 1% of h.e. 1/E result (the ratio between setups A and B) 1 − 10 2 − 10 in each rock component. 3 − 10 4 − 10 • The most likely spectra (made from 5 − 10 experimental data) in each sample are 6 − 10 − 7 10 almost same. − 8 10 • This is not affected by uncertainty of 9 8 6 5 3 − − 7 − − 4 − 2 1 2 − − − − 10 10 10 10 10 10 10 10 10 1 10 10 Neutron energy (MeV) Simulation. The most likely spectrum � 7 Keita Mizukoshi Kobe Univ.

  8. Obtained spectrum K. Mizukoshi et al., PTEP 123C01 • We obtained the most likely /s 2 10 2 Counts /MeV /cm The most likely spectrum 10 2% of hydrogen spectrum of the ambient neutron. 1 4% of hydrogen 1/E − 1 10 • We compared the fluxes 
 2 − 10 − 3 10 (the previous study fluxes in other 4 − 10 − 5 10 − 6 10 underground laboratories). Thermal neutron 7 ~0.025eV − 10 − 8 10 • They are the same order of 9 8 6 5 3 − − 7 − − 4 − 2 1 2 − − − − 10 10 10 10 10 10 10 10 10 1 10 10 magnitude. 
 Neutron energy (MeV) The most likely spectrum Neutron fluxes in previous researches It is difficult to compare 
 • Flux ( × 10 -6 cm -2 s -1) Thermal Non-thermal the result simply because 
 there are many difference 
 Kamioka +0.7 +1.2 7.9 ± 0.23 15.6 ± 0.5 (This result, Mizukoshi) -0.7 -1.4 in these measurement 
 Kamioka 8.26 ± 0.58 11.5 ± 1.2 (e.g., detector, assumption 
 (Minamino 2004) Gran Sasso of spectral shape, and 
 13.3 ± 1.5 10.2 ± 1.1 (A. Lindi 1988) ※ definition of flux) LSM 14.3 ± 1.3 4.2 ± 2.8 (K. Eitel 2012) ※ ※ They used the different definition of flux. 
 � 8 We adjusted the same definition of us. Keita Mizukoshi Kobe Univ.

  9. New interest /s 2 10 2 Counts /MeV /cm The most likely spectrum 10 2% of hydrogen 1 4% of hydrogen 1/E 1 − 10 2 − 10 Excess − 3 10 In the previous research, rough • 4 − 10 spectral shape was assumed 
 − 5 10 6 − 10 (e.g., Boltzmann distribution and 1/E). 7 − 10 8 − 10 • The most likely spectrum 
 9 8 6 5 3 − − − 7 − − − 4 − − 2 − 1 2 10 10 10 10 10 10 10 10 10 1 10 10 Neutron energy (MeV) suggests the excess in a The most likely spectrum few MeV. • Since the cross section of • The excess is interesting 
 high energy neutrons is for direct dark matter search. small, it continues to be a • The excess should be high energy neutron. • Once it lose energy, the confirmed by a liquid cross section increases. it scintillator which has a continues to lose energy. sensitivity for the neutron. • Therefore, the excess will • Even such basic information remain at several MeV. has not confirmed… K. Mizukoshi et al., PTEP 123C01 � 9 Keita Mizukoshi Kobe Univ.

  10. Summary • We evaluated an ambient neutron spectrum and + 1.9 obtained the flux (23.5 ± 0.7 stat. sys. × 10 -6 cm -2 s -1 ) - 2.1 at the Kamioka Observatory. using 3 He proportional counter and moderator effectively • with data-driven analysis and simulation • considering systematic errors • • Spectral excess around a few MeV was suggested. It should be confirmed by a sensitive detector for non-thermal neutron. • We are preparing a low BG liquid scintillator. � 10 Keita Mizukoshi Kobe Univ.

  11. Backup slides

  12. Main backgrounds of our experiment cosmic muon • Rate events search experiments are Muon Veto counter placed in underground to reduce BGs ~ Cosmic muon • For Others Shield Detector • Remaining high-energy muon 
 (Pb) ← active veto by scintillator neutron Fiducial 
 • Ambient gamma 
 External 
 Volume (FV) for events ← shield / self-shielding / PSD gamma • Alpha from U/Th chain 
 ← very careful washing • Neutron 
 ← It’s difficult to reduce • Shield with materials which have large cross-section for General ways to reduce BGs neutron in underground experiment • Sometimes neutron makes other BGs (gamma in detector) (Conceptional fig) � 12 Keita Mizukoshi Kobe Univ.

  13. How much neutron is in underground Photo CANDLES Collaboration • I worked for a neutrino-less double beta decay experiment (CANDLES 3+ Experiment) at Kamioka Observatory. • This experiment reduces ambient neutron with Boron shield (~5000 barn for thermal neutron). • Ambient neutron (flux, spectrum) was not understood well. CANDLES Experiment • I would like to show how to for neutrinoless double beta decay measure ambient neutron to using 48 CaF 2 Scintillator demonstrate how difficult to handle neutron as a rare BG. � 13 Keita Mizukoshi Kobe Univ.

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