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Measurement of ambient neutrons in an underground laboratory at Kamioka Observatory Keita Mizukoshi Kobe University TAUP2019 at Toyama International Conference Center 9 Sep. 2019 Introduction Neutron is the one of the most serious


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SLIDE 1

Measurement of ambient neutrons in an underground laboratory at Kamioka Observatory

Keita Mizukoshi Kobe University TAUP2019 at Toyama International Conference Center 9 Sep. 2019

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SLIDE 2

Keita Mizukoshi Kobe Univ.

Introduction

  • Neutron is the one of the most serious backgrounds

(BG) for experiments in underground.

  • Direct Dark matter search
  • Neutrino-less double beta decay search
  • To evaluate and shield neutron BG, 


it is very important to evaluate ambient neutron flux

  • Such neutron BG has not measured systematically.
  • Low rate in underground i→ Required high efficiency
  • Unknown generated points → Energy unknown
  • Our goal is quantitative neutron flux in the underground

2

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SLIDE 3

Keita Mizukoshi Kobe Univ.

Detector (He-3 proportional counter)

  • We used a 3He

proportional counter.

  • The energy of the

exothermal reaction in the neutron capture can be obtained.

  • This detector is

sensitive to thermal neutrons (~0.025 eV), and cannot measure an initial neutron energy.

3

3He proportional counter

DAQ PC

3He + n → 3H + p + 0.76 MeV

3He - 10 atm

SUS

thermal fast

“Setup A”

380mm φ52mm

  • K. Mizukoshi et al., PTEP 123C01

~5 k barn at thermal

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SLIDE 4

Keita Mizukoshi Kobe Univ.

Setup for fast neutron

thermal fast “Setup A”

Polyethylene

3He

Boron sheet

thermal fast “Setup B”

510mm

t5mm

3He

Efficiency estimated by Geant4

9 −

10

8 −

10

7 −

10

6 −

10

5 −

10

4 −

10

3 −

10

2 −

10

1 −

10 1 10

2

10 Generated neutron energy (MeV) 20 40 60 80 100 120 140 160 )

2

Counts/(neutron/cm

Setup A Setup B Setup B w/o B-sheet

Thermal neutron ~0.025eV

  • To measure high energy neutron, 


we used a moderator (polyethylene).

  • Boron sheet captured thermal

neutrons and reduce its effect.

4

  • K. Mizukoshi et al., PTEP 123C01
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SLIDE 5

Keita Mizukoshi Kobe Univ.

Results

  • Full energy peak is 0.76 MeV. 


If 3H or p escapes, continuum region will be made in a low energy (Wall effect).

  • Low energy region below 0.3 MeV is

dominated by electric noise for ambient neutron measurement.

  • We counted events up to 0.85 MeV

and down to 0.5 MeV, then the number

  • f total events was estimated by a

clear spectrum observed using 252Cf.

5

Setup

A B

Count rate (×10-3cps)

1.295 ± 0.034 0.446 ± 0.018

Live time (day)

14.03 19.27

0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 1 Measured energy (MeV) 200 400 600 800 1000 1200 Counts/bins 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 1 Measured energy (MeV) 20 40 60 80 100 Counts/bins

Spectrum of Source (252Cf) Measured spectrum in setup B

3He + n → 3H + p + 0.76 MeV

Count rate in each setup

  • The count rate of Setup A

(RA) and B (RB) involves a detection of thermal and
 fast neutron, respectively.

Electric
 noise peak Wall effect

  • K. Mizukoshi et al., PTEP 123C01
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SLIDE 6

Keita Mizukoshi Kobe Univ.

Simulation

  • To convert from the count rates (RA, RB) to

ambient neutron flux, the spectral shape was

  • required. The shape cannot measured by He-3

detector thus estimated by simulation.

  • We considered the source of the neutrons

made from (α,n) reaction of U/Th series decay.

  • Neutron induced by cosmic muon is negligible.
  • We picked three types of rocks as samples,

they had much different abundance of chemical compositions.

  • The difference affects much the yield of

neutrons.

6

1 2 3 4 5 6 7 Neutron energy (MeV) 0.2 0.4 0.6 0.8 1 1.2 1.4 1.6 1.8 2 2.2

6 −

10 × Number of nentrons /chain decay/0.1 MeV

, n) α JR-1 ( , n) α JA-3 ( , n) α Sample 1 ( Sample 1 + 3% of hydrogen , n) α Sample 2 ( , n) α Sample 3 ( U fission)

238

Sample 1 ( Sample 1 (Th series)

Bin width 0.1 MeV

Generated neutron in vary rocks

(wt. %) sample1 sample2 sample3

O 40.5 37.9 35.6 Ca 28.0 24.3 29.7 Si 16.6 15.6 12.0 Fe 7.6 16.6 13.5 Al 5.2 0.3 0.1 Mn 0.8 3.5 2.9

Main components in each samples

JR-1 and JA-3 are geometrical reference database

Much
 difference!

  • K. Mizukoshi et al., PTEP 123C01
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SLIDE 7

Keita Mizukoshi Kobe Univ.

Data driven analysis

  • We cannot investigate the all wall rock

components in details.

  • Especially amount of water contents in the

rock and chemical composition including Hydrogen will much affect thermalization of fast neutrons.

  • Thus, thermalization in the rock was

unknown.

  • We regarded the percentage of hydrogen

(%of h. e.) in simulation as a thermalization parameter.

  • %of h.e. was derived by the experimental

result (the ratio between setups A and B) in each rock component.

  • The most likely spectra (made from

experimental data) in each sample are almost same.

  • This is not affected by uncertainty of

Simulation. 7

1 2 3 4 5 6 7 % of h. e. 0.5 1 1.5 2 2.5 3 3.5 4

B

/R

A

Ratio of count rates R

Experimental ratio Error band Sample 1 Sample 2 Sample 3 JR-1 JA-3 9 −

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8 −

10

7 −

10

6 −

10

5 −

10

4 −

10

3 −

10

2 −

10

1 −

10 1 10

2

10 Neutron energy (MeV)

8 −

10

7 −

10

6 −

10

5 −

10

4 −

10

3 −

10

2 −

10

1 −

10 1 10

2

10 /s

2

Counts /MeV /cm

Sample 1 with 3% of h.e. JR-1 with 1% of h.e. JA-3 with 1% of h.e. 1/E

The most likely spectrum

Experimental ratio v.s. parameter

Thermalization parameter


  • btained by measurement
  • K. Mizukoshi et al., PTEP 123C01
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SLIDE 8

Keita Mizukoshi Kobe Univ.

Obtained spectrum

  • We obtained the most likely

spectrum of the ambient neutron.

  • We compared the fluxes 


(the previous study fluxes in other underground laboratories).

  • They are the same order of

magnitude.


  • It is difficult to compare 


the result simply because 
 there are many difference
 in these measurement 
 (e.g., detector, assumption 


  • f spectral shape, and 


definition of flux) 8

9 −

10

8 −

10

7 −

10

6 −

10

5 −

10

4 −

10

3 −

10

2 −

10

1 −

10 1 10

2

10 Neutron energy (MeV)

8 −

10

7 −

10

6 −

10

5 −

10

4 −

10

3 −

10

2 −

10

1 −

10 1 10

2

10 /s

2

Counts /MeV /cm

The most likely spectrum 2% of hydrogen 4% of hydrogen 1/E

Flux (×10-6 cm-2 s-1) Thermal Non-thermal

Kamioka (This result, Mizukoshi) 7.9 ± 0.23 +0.7

  • 0.7

15.6 ± 0.5 +1.2

  • 1.4

Kamioka (Minamino 2004) 8.26 ± 0.58 11.5 ± 1.2 Gran Sasso (A. Lindi 1988)※ 13.3 ± 1.5 10.2 ± 1.1 LSM (K. Eitel 2012)※ 14.3 ± 1.3 4.2 ± 2.8

The most likely spectrum Neutron fluxes in previous researches

※They used the different definition of flux. 
 We adjusted the same definition of us.

Thermal neutron ~0.025eV

  • K. Mizukoshi et al., PTEP 123C01
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SLIDE 9

Keita Mizukoshi Kobe Univ.

New interest

  • In the previous research, rough

spectral shape was assumed 
 (e.g., Boltzmann distribution and 1/E).

  • The most likely spectrum 


suggests the excess in a few MeV.

  • The excess is interesting 


for direct dark matter search.

  • The excess should be

confirmed by a liquid scintillator which has a sensitivity for the neutron.

  • Even such basic information

has not confirmed…

9

9 −

10

8 −

10

7 −

10

6 −

10

5 −

10

4 −

10

3 −

10

2 −

10

1 −

10 1 10

2

10 Neutron energy (MeV)

8 −

10

7 −

10

6 −

10

5 −

10

4 −

10

3 −

10

2 −

10

1 −

10 1 10

2

10 /s

2

Counts /MeV /cm

The most likely spectrum 2% of hydrogen 4% of hydrogen 1/E

The most likely spectrum

Excess

  • Since the cross section of

high energy neutrons is small, it continues to be a high energy neutron.

  • Once it lose energy, the

cross section increases. it continues to lose energy.

  • Therefore, the excess will

remain at several MeV.

  • K. Mizukoshi et al., PTEP 123C01
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SLIDE 10

Keita Mizukoshi Kobe Univ.

Summary

  • We evaluated an ambient neutron spectrum and
  • btained the flux (23.5 ± 0.7stat. sys.×10-6 cm-2 s-1)

at the Kamioka Observatory.

  • using 3He proportional counter and moderator effectively
  • with data-driven analysis and simulation
  • considering systematic errors
  • Spectral excess around a few MeV was
  • suggested. It should be confirmed by a sensitive

detector for non-thermal neutron.

  • We are preparing a low BG liquid scintillator.

10

+1.9

  • 2.1
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SLIDE 11

Backup slides

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SLIDE 12

Keita Mizukoshi Kobe Univ.

Main backgrounds of our experiment

  • Rate events search experiments are

placed in underground to reduce BGs ~ Cosmic muon

  • For Others
  • Remaining high-energy muon 


← active veto by scintillator

  • Ambient gamma 


← shield / self-shielding / PSD

  • Alpha from U/Th chain 


← very careful washing

  • Neutron 


← It’s difficult to reduce

  • Shield with materials which

have large cross-section for neutron

  • Sometimes neutron makes
  • ther BGs (gamma in detector)

12

Fiducial
 Volume (FV) for events

cosmic muon External
 gamma

General ways to reduce BGs in underground experiment

Muon Veto counter Shield (Pb)

(Conceptional fig)

Detector neutron

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SLIDE 13

Keita Mizukoshi Kobe Univ.

How much neutron is in underground

  • I worked for a neutrino-less

double beta decay experiment (CANDLES 3+ Experiment) at Kamioka Observatory.

  • This experiment reduces

ambient neutron with Boron shield (~5000 barn for thermal neutron).

  • Ambient neutron (flux,

spectrum) was not understood well.

  • I would like to show how to

measure ambient neutron to demonstrate how difficult to handle neutron as a rare BG.

13

CANDLES Experiment

for neutrinoless double beta decay using 48CaF2 Scintillator

Photo CANDLES Collaboration

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SLIDE 14

Keita Mizukoshi Kobe Univ.

Main neutron detectors for underground

14

He-3 Counter Liquid Scintillator Gd-Water Čerenkov

Čerenko

Emulsion Thermal Neutron Very good No Very good No Fast Neutron No sensitivity† Good Good Good Energy Sensitivity No Possible No Possible n/γ rejection Good Sometime Good No Good Internal background Low Sometime bad Low Low Handling Analysis Easy Difficult Difficult Very difficult Detection
 Efficiency Very good so-so so-so Very good

†Generally.

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SLIDE 15

Keita Mizukoshi Kobe Univ.

Neutron source (Not U/Th)

  • We can consider the ambient

neutron made from cosmic muon.

  • It can make high energy

neutron (>10 MeV), the number of neutrons by muon is 100 times less than the

  • nes by U/Th series.
  • In this research, we ignored

the contribution of muon.

15

Generated neutrons from cosmic muon Spectrum of each source for sample1

100 200 300 400 500 600 700 800 900 1000 Neutron energy(MeV)

16 −

10

15 −

10

14 −

10

13 −

10

12 −

10

11 −

10 /s

3

Number of produced neutrons /MeV /cm

Sample 1 Sample 2 Sample 3

Bin width 10 MeV 9 −

10

8 −

10

7 −

10

6 −

10

5 −

10

4 −

10

3 −

10

2 −

10

1 −

10 1 10

2

10 Neutron energy (MeV)

14 −

10

13 −

10

12 −

10

11 −

10

10 −

10

9 −

10

8 −

10

7 −

10

6 −

10

5 −

10

4 −

10

3 −

10

2 −

10

1 −

10 1 10 /s

2

Counts /MeV /cm

Summed spectrum w/o muon , n) α U ( , n) α Th ( U fission

238

Muon

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SLIDE 16

Keita Mizukoshi Kobe Univ.

Simulation uncertainty for neutron

  • Geant4 - Monte-Carlo toolkit

widely used in Particle Physics

  • PHITs - Boltzmann equation

solver used in Nuclear Physics

  • These simulation tools produce

huge uncertainty.

  • These spectrum simulate

neutrons made in rocks around underground

  • laboratory. These neutron

source is Uranium and Thorium chain nuclei.

16

0.05 0.1 0.15 0.2 0.25 0.3

6 −

10 × Energy(MeV) 0.2 0.4 0.6 0.8 1 1.2 1.4 1.6 current /cm^2 /MeV /s 0.05 0.1 0.15 0.2 0.25 0.3 0.35 0.4 0.45 Neutron energy (MeV) 0.2 0.4 0.6 0.8 1 1.2 1.4 1.6 1.8

6 −

10 × Counts /s /cm^2 /MeV

Example: Differences of simulation tools for transported neutron energy spectrum
 PHITs Geant4 Thermal neutron Fast neutron PHITs Geant4

  • K. Mizukoshi et al., PTEP 123C01
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SLIDE 17

Keita Mizukoshi Kobe Univ.

All components of the rocks

17

(wt. %) sample1 sample2 sample3

sampleA sampleC

KamRock Si

16.6 15.6 12.0 29.1 27.8 18.5

Ti

0.2 0.0 0.0 0.5 0.5 0.1

Al

5.2 0.3 0.1 7.1 8.3 10.6

Fe

7.6 16.6 13.5 4.6 4.5 1

Mn

0.8 3.5 2.9 0.1 0.1

Mg

0.6 1.1 0.7 2.2 1.3 0.3

Ca

28.0 24.3 29.7 4.5 5.2 1.8

Na

0.0 0.2 0.0 2.4 2.6 3.9

K

0.0 0.1 0.0 1.2 1.5 2.1

P

0.2 0.0 0.0 0.1 0.1 0.1

S

0.0 0.1 1.2 0.0 0.0

Zn

0.0 0.1 4.3 0.0 0.0

Sr

0.1 0.0 0.0 0.0 0.0

Nb

0.0 0.0 0.0 0.0 0.0

Sn

0.1 0.0 0.0 0.0 0.0

Pb

0.0 0.0 0.0 0.0 0.0

O

40.5 37.9 35.6 48.3 48.1 60.7

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SLIDE 18

Keita Mizukoshi Kobe Univ.

He-3 Cross section for neutron

  • He cross section is much

large for thermal neutrons.

  • Cross sections of the rock

components have the same trend.

  • Since the cross section of

high energy neutrons is small, it continues to be a high energy neutron.

  • Once it lose energy, the

cross section increases. it continues to lose energy.

  • Therefore, the dip will

remain at several MeV.

18

10-7 10-6 10-5 10-4 10-3 10-2 10-1 100 101 102 103 104 105 10-2 10-1 100 101 102 103 104 105 106 107

Cross Section (barns) Neutron Energy (eV)

He-3

total elastic capture (n,p)

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SLIDE 19

Keita Mizukoshi Kobe Univ.

Definition of Flux

  • Two types of definition are

used.

  • (1)Number of particle through

the sphere (radius r)/
 the area of grate circle(πr2)

  • Widely used in Nuclear physics
  • We use that.
  • (2)Number of particle through

the circle (radius r)/ the area (πr2)

  • Widely used in Particle physics
  • LSM and Gran Sasso would

use this definition.

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R r

  • Def. 1
  • Def. 2

Count No count