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Decay spectroscopy at RIBF: The EURICA project and its impact on - - PowerPoint PPT Presentation

Decay spectroscopy at RIBF: The EURICA project and its impact on nuclear structure and astrophysics ISOLDE Workshop and Users meeting 2015 2 nd 4 th , December, 2015 Department of Physics and Astronomy, KU Leuven RI Physics Lab., RIKEN


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SLIDE 1

Decay spectroscopy at RIBF: The EURICA project and its impact on nuclear structure and astrophysics

ISOLDE Workshop and Users meeting 2015 2nd – 4th, December, 2015 Department of Physics and Astronomy, KU Leuven RI Physics Lab., RIKEN Nishina Center Zhengyu Xu for the EURICA Collaboration

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SLIDE 2

Table of Content

What is EURICA? Motivation and experimental setup Highlights of experimental results Summary and perspective

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SLIDE 3

What is EURICA? Euroball Riken Cluster Array

High efficiency gamma-ray detector array + Highly segmented Si stopper / passive stopper + High beam intensity at RIBF (10 pnA 238U or 30 pnA 124Xe)

Isomer and b-decay spectroscopy!

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SLIDE 4
  • New magic number ?
  • Shell quenching?
  • Single particle levels?
  • Deformation?

Decay properties of exotic nuclei studied with EURICA

Beta-decay half lives, Beta- delayed neutron-emission probabilities of exotic nuclei.

Maandag - vrijdag: 10u00 - 12u30 en 13u30 - 17u00 Weekdagen na 17u00 op afspraak Zaterdag op afspraak

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SLIDE 5

General experimental setup of an EURICA campaign

Production Target

Separation

  • f RI

Identification

  • f RI

R R I I B B e e a a m m

EURICA 238U (124Xe) Beam RI Beam

Cluster Ge-detectors (gamma-ray detection) Cluster Ge-detectors (gamma-ray detection)

Beta-counting system inside EURICA

WAS3ABi : beta-ray detection WAS3ABi : beta-ray detection gamma-ray

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SLIDE 6

RISING@GSI 2006-2009 EURICA@RIKEN 2012-2015

Decay spectroscopy with the “old” cluster detectors

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SLIDE 7

Collaboration RIKEN / TUM / IBS

  • 8 DSSD 1-mm thick
  • 80 keV threshods
  • 20 keV energy resolution
  • 100 - 200 pps Maximum rate
  • Q value capability
  • About 20000 pixels

WAS3ABi (Wide-range Active Silicon Strip Stopper for beta and ions)

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SLIDE 8

Production Target

Separation

  • f RI

Identification

  • f RI

EURICA

Passive stopper LaBr3(Ce) (fast timing)

General experimental setup of an EURICA campaign

Different stopper/detectors can be employed to meet the requirements of specific experiments.

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SLIDE 9

International collaboration

  • J. Agramunt, P. Aguilera, T. Alharbi, A. Algora, G. Angelis, N. Aoi, P. Ascher, R. Avigo,

H.Baba, C. Borcea, A. Boso, A.M. Bruce, R.B. Cakirli, F.L.Bello Garrote, G. Benzoni, J.S.Berryman, R. Berta, B. Blank, N. Blasi, A. Blazhev, P. Boutachkov, S. Bonig, A. Bracco, F. Browne, F. Camera, R.J. Carroll, S. Ceruti, I. Celikovic, K.Y. Chae, J. Chiba,

  • L. Coraggio, A. Covello, F.C.L. Crespi, J.-M. Daugaus, R. Daido, P. Davis, M.C. Delattre,
  • F. Diel, F. Didiejean, Zs. Dombradi, P. Doornenbal, F. Drouet, H.J. Eberth, A. Estrade, Y.

Fang, T. Faestermann, G. France, S. Franchoo, Y. Fujita, N. Fukuda, A. Gadea, E. Ganioglu, A. Gargano, W. Gelletly, M. Gerbaux, R. Gernhauser, G. Gey, J. Giovninazzo,

  • S. Go, N. Goel, T. Goigoux, M. Gorska, A. Gottardo, H. Grawe, S. Grevy, C. Griffin, Vi.

Guadilla, T. Hashimoto, S. Hayakawa, J. Henderson, C. Hinke, N. Hinohara, E. Ideguchi,

  • S. Ilieva, N. Inabe, T. Ishigaki, T. Isobe, Y. Ito, D.G. Jenkins, P.R. John, H.S. Jung, A.

Jungclaus, T. Kajino, D. Kameda, H. Kanaoka, Y. Kanke, Y. Kawada, G.D. Kim, Y.-K. Kim, G. Kiss, Ka. Kobayashi, K. Kobayashi, M. Kobayashi, N. Kobayashi, K. Koehler, I. Kojouharov, T. Komatsubara, F.G. Kondev, Z. Korkulu, Y. Kondo, M. Kowalska, T. Kroll, R. Krucken, T. Kubo, S. Kubono, M. Kurata-Nishimura, T. Kurtukian Nieto, N. Kurz, I. Kuti, Y.K. Kwon, G.J. Lane, S. Lalkovski, G. Lane, E. Lee, J. Lee, P. Lee, S. Lenzi, M. Lewitowicz, Z. Li, J. Liu, T. Lokotko, G. Lorusso, G. Lotay, R. Lozeva, D. Lubos, C. Magron, F. Molina, I. Matea, K. Matsui, M. Matsushita, B. Melon, D. Mengoni, B. Meyer, S. Michimasa, T. Miyazaki, V. Modamio Hoybjor, S. Momiyama, C.-

  • B. Moon, A. Morales. A. Montaner-Piza, A.I. Morales, P. Morfouace, S. Morimoto, K.

Moschner, D. Mucher, E. Nacher, J. Nagumo, H. Naidja, T. Nakao, T. Nakatsukasa, D.R. Napoli, F, Naquvi, M. Niikura, H. Nishibata, S. Nishimura, I. Nishizuka, C. Nita, F. Nowacki, A. Odahara, K. Ogawa, H. Oikawa, R. Orlandi, S. Ota, T. Otsuka, H.J. Ong, S. Orrigo, M. Rajabali, J. Park, Z. Patel, A. Petrovici, F. Recchia, V. Phong, Zs. Podolyak, O.J. Roverts, L. Prochniak, P.H. Regan, S. Rice, E. Sahin, H. Sakurai, K. Sato, H. Schaffner, H.Scheit, P. Schury, C. Shand, Y. Shi, S. Shibagaki, T. Shimoda, Y. Shimizu, K. Sieja, L. Sinclair, G.S. Simpson, P.-A. Soderstrom, D. Sohler, I.G. Stefan, K. Steiger, D. Steppenbeck, K. Sugimoto, T. Sumikama, D. Suzuki, H. Suzuki, T. Tachibana, K. Tajiri,

  • S. Takano, A. Tashima, H. Takeda, Man. Tanaka, Mas. Tanaka, Y. Takei, R. Taniuchi, J.

Taprogge, K. Tajiri, T. Teranishi, S. Terashima, G. Thiamova, K. Tshoo, Zs. Vajta, J. Valiente Dobon, Y. Wakabayashi, P.M. Walker, H. Watanabe, A. Wendt, V. Werner, O. Wieland, K. Wimmer, J. Wu, Q. Wu, F.R. Xu, Z.Y. Xu, A. Yagi, S. Yagi, H. Yamaguchi,

  • K. Yamaguchi, T. Yamamoto, M. Yalcinkaya, R. Yokoyama, S. Yoshida, K. Yoshinaga, G.

Zhang

19 countries : 238 collaborators !

EURICA Collaboration

2012

124Xe

2013

238U

2012

238U

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SLIDE 10

EURICA Campaigns 2012-2015

Half-lives (T1/2) Isomer (T1/2) Beta-delayed gamma Beta-delayed n, p EC, Qb, New isotopes K.Möschner T.Sumikama F.Browne I.Nishizuka P.-A.Söderström A.Jungclaus G.Simpson G.Lorusso Y.Shimizu A.Yagi E.Ideguchi, M.Tanaka R.Yokoyama W.Jin L.Sinclair Z.Y.Xu D.Lubos H.S.Jung M.Lewitwicz H.Suzuki G.Lorusso M.Niikura E.Sahin R.Lozeva Z.Li Orsay Gr. V.Warner Z.Patel F.Bello D.Sohler, Z.Vajta J.Park I.Celikovic G.Zhang H.Watanabe P.A.Söderström P.A.Söderström G.Benzoni A.Odahara P.Boutachkov H.Watanabe F.Naqvi S.Nishimura R.Gernhäuser G.Simpson G.Gey P.Davies T.Sumikama J.Wu P.S.Lee, C.B.Moon G.Lorusso J.Jin B.Blank B.Rubio, T.Fujita, .. A.Algora, . .

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SLIDE 11

Experimental results in the region N=40 ~ 50

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SLIDE 12

Beta-decay half-lives beyond 78Ni

Shorter T1/2 beyond 78Ni: Pronounced in Z = 28, N=50 78Ni is a double magic nucleus !? Shorter T1/2 beyond 78Ni: Pronounced in Z = 28, N=50 78Ni is a double magic nucleus !? Decay curve of 79Ni

Z.Y.Xu, S.Nishimura, G.Lorusso et al., PRL 113, 032505 (2014)

77Co 78Ni 79Ni

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SLIDE 13

Studying the collectivity up to N=44 in the Fe chain

It is found that the experimental R4/2 ratio is properly reproduced for A>36 by the shell model

  • nly with the inclusion of the 1d5/2 neutron orbital in the valence space. This is interpreted, as

for Cr isotopes, in terms of the interplay between the quadrupole correlations of the ν1d5/2 and ν0g9/2 orbitals and the monopole component of the π0f7/2 - ν0f5/2 interaction, thus driving the deformation in the neutron-rich Cr-Fe region. G.Benzoni et al., PLB 751, 107 (2015)

68Fe 69Fe 70Fe

From 400 ions of 70Mn

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SLIDE 14

Experimental results in the region N=60 ~ 82

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SLIDE 15

Delayed coin. with 128Pd ions (Δt=0.15-25 μs) γ-γ coincidence with a gate on 1311 keV

B(E2;8+→6+) B(E2;8+→6+) Good ν=2 in the well isolated πg9/2 subshell Good ν=2 in the well isolated πg9/2 subshell Robust shell closure at N=82 Robust shell closure at N=82 Seniority (ν) scheme Seniority (ν) scheme

128Pd82 130Cd82

A.Jungclaus et al., PRL 99, 132501 (2007)

2 2

2 1 2 2 1 2 ) 2 ; 2 (

eff

e j n j J J E B                 

The seniority isomers in the N=82 isotones

  • H. Watanabe et al., PRL111, 152501 (2013)
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SLIDE 16

νf7/2

2 Jπ=6+ seniority isomers in 136, 138Sn

20 40 60 80 Counts

a)

216 391 688

100 200 300 400 500 600 700 800 900 Energy (keV) 2 4 6 8 10 12 14 16 Counts

b)

168 461 715 50 100 150 200 250 Time (ns) 20 40 C per 12.4 ns T1/2=46(7) ns 250 500 750 1000 Time (ns) 10 20 C per 100 ns T1/2=210(45) ns

136Sn 138Sn

875,000 ions 5,000 ions ~640 ns flight time BigRIPS T1/2=46(7) ns

T1/2=210(45) ns

The excited states up to 6+

  • f 136,138Sn were constructed

via the isomeric decay

  • spectra. The knowledge of

the excitation energies of the first 2+ states was extended to 138Sn.

The life time of the 136Sn isomer is very short!!

The experimental B(E2; 6+ → 4+) rate of 136Sn can be reproduced by reducing the neutron pairing strength by ~150 keV, with the result that the first 4+ state now has mixed seniority (46% ν = 2, 55% ν=4). G. S. Simpson et al., PRL 113, 132502 (2014)

136Sn 138Sn 134Sn

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SLIDE 17

N=50 N=82

20 40 60 Counts/2 keV 1000 2000 3000 4000 5000 6000 Energy (keV) 200 400 600 Counts/2 keV

988 keV

# # & @

132Cd 131Cd

x4

pg9/2

  • 1

pp1/2

  • 1

pp3/2

  • 1

New pp3/2 single-hole energy in 132Sn !

Identification of a proton single-hole state in 132Sn

empirical SM A.F. Lisetskiy realistic SM

  • H. Grawe, A. Gargano

No proton subshell structure !

  • J. Taprogge, A. Jungclaus et al.,

PRL 112, 132501 (2014)

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SLIDE 18

Two EURICA data sets: G.Simpson/A.Jungclaus & H.Watanabe/G.Lorusso

New Isotopes

144Te 140Sb 139,140Sn 136,137In 134,135Cd 131,132Ag 129,130Pd 127Rh 120,121Tc 118Mo

and more..

U-beam: 8 – 10 pnA ~ Two weeks Known T1/2

Beta-decay half-lives around A = 100~145

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SLIDE 19

Two EURICA data sets: G.Simpson/A.Jungclaus & H.Watanabe/G.Lorusso

New Isotopes

144Te 140Sb 139,140Sn 136,137In 134,135Cd 131,132Ag 129,130Pd 127Rh 120,121Tc 118Mo

and more..

U-beam: 8 – 10 pnA ~ Two weeks Known T1/2

Beta-decay half-lives around A = 100~145

G.Lorusso et al., PRL 114, 192501 (2015)

40 new half lives!!

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SLIDE 20

80 100 120 140 160 180 200 220 240 Mass number A Solar-system abundance pattern

Before After new RIBF data

Dip problem!

Rare earth elem.

1st Peak 2nd Peak 3rd Peak

238U 195Pt 130Xe 232Th 235U 128Te

The new data with an (n, γ) (γ, n) equilibrium. ⇄ The new data with an (n, γ) (γ, n) equilibrium. ⇄

G.Lorusso et al., PRL 114, 192501 (2015)

R-process abundance with new half lives from EURICA

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SLIDE 21

Lifetime measurements of the first 2+ states in 104,106Zr (N=64,66)

104Zr is the most deformed of the neutron-rich Zr isotopes. In addition,

comparison of the magnitude of the extracted deformation with the results of model calculations indicate that these nuclei are prolate

  • deformed. F.Browne, A.M. Bruce, T. Sumikama et al., PLB 750, 448 (2015)

Time-energy matrix from LaBr3.

104Zr 106Zr

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SLIDE 22

Experimental results in the region N~100

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SLIDE 23

Isomer decay spectroscopy of

164Sm and 166Gd

  • Z. Patel, P.-A. Söderström et al. PRL 113, 262502 (2014)

166Gd 166Gd 164Sm 164Sm

6- isomers have the

  • configuration. Also
  • berserved in

heavier N=102 isotones 170Er and

172Yb

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SLIDE 24

Energy systematics and a deformed shell gap at N=100

  • Most deformed N=102

nuclei to date

  • A local maximum at

N=100

  • Many models suggest a

deformed magic number N=100

  • These calculations also

show that a deformed shell closure would have an effect on the masses

  • f Z ≤ 62 nuclei
  • L. Satpathy & S. K. Patra

predict a deformed shell gap at N=100 from S2n

  • This will influence r-

process abundance calculations

  • L. Satpathy and S.K. Patra

NPA722, C24 (2003)

  • Z. Patel, P.-A. Söderström et al. PRL 113, 262502 (2014)
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SLIDE 25

Summary and perspective

  • Half-lives of many exotic nuclei around N=50 and N=82 were measured.

The new half-lives have great impact on both nuclear structure and nuclear astrophysics.

  • Isomeric and beta-delayed gamma-ray spectra have been investigated to

study nuclear shell/shape evolution in neutron-rich nuclei with N=40, 60, 82, and 100.

  • Data analysis is still ongoing and many new results are coming:
  • Proton-neutron correlation along N=Z nuclei (100Sn, 98In, 96Cd, 94Ag...).
  • New half-lives above Z=50.
  • Search for two-proton emitter in proton-rich Ge, Se, and Kr isotopes.
  • Many new isomeric and beta-delayed spectrum will be studied for

neutron-rich nuclei around 78Ni and 132Sn.

  • ...
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SLIDE 26

Thank you for your attention!

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SLIDE 27

Backup slides

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SLIDE 28

126Pd80 126Ag79

  • H. Watanabe et al.,

PRL 113, 042502 (2014)

7- : ν(h11/2

  • 1d3/2
  • 1)

10+ : ν(h11/2)-2

A long-lived isomer in 126Pd

Long-lived isomer Ex = 2406 keV T1/2 = 23. 3.0(8) ms Jπ = (10+) Rint = 26(8) % B(E3) = 0.07(2) W.u.

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SLIDE 29

A long-lived isomer in 129Cd

Gated on conversion electrons Gated on compton electrons

0.4 0.8 1.2 1.6 2 Ex (MeV)

1181 406 1587 353

E3 M1

(11/2-) (13/2-) (15/2-) (21/2+)

exp SM

nh11/2 x 2+(130Cd) nh11/2 x 5-(130Cd) 5-: g9/2

  • 1p1/2
  • 1 + g9/2
  • 1p3/2
  • 1 + g9/2
  • 1f5/2
  • 1

2+: g9/2

  • 2

=

E3

B(E3) is very sensitive to position of the pp3/2 and pf5/2 orbitals relative to the pg9/2 Position of pp3/2 orbital already fixed by the 988 keV g transition observed in 131In

Information on the missing fourth proton single-hole energy with respect to 132Sn ! T1/2 = 3.53(16) ms

Bexp(E3) = 505(23) e2fm6 = 0.51(2) W.u. BSM(E3) = 0.48 W.u. - for E(p3/2)-E(f5/2)=1.1 MeV and 0.5e

10 ms after 129Cd implantation Spectrum from Si

Spectrum from Ge Spectrum from Ge

  • J. Taprogge, A. Jungclaus et al.,

PLB 738, 223 (2014)