Quantum impurity systems and Luttinger-Friedel sum rule ~ Luttinger - - PowerPoint PPT Presentation

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Quantum impurity systems and Luttinger-Friedel sum rule ~ Luttinger - - PowerPoint PPT Presentation

Quantum criticality in Quantum impurity systems and Luttinger-Friedel sum rule ~ Luttinger integral as a topological invariant ~ Internat ationa onal Symp mpos osiu ium in H Honor of Profe fesso sor Nambu for the 10 10th A Annivers


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Quantum criticality in Quantum impurity systems and Luttinger-Friedel sum rule

~ Luttinger integral as a topological invariant ~

Internat ationa

  • nal Symp

mpos

  • siu

ium in H Honor of Profe fesso sor Nambu for the 10 10th A Annivers rsar ary y of hi his N Nobel Prize in P Physics

Yunori Nishikawa (Osaka City University)

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A.C.Hewson O.J.Curtin, D.J.G. Crow ( Imperial College London )

Collaborators

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Outline of Presentation

  • 1. Model and Systems

General Background Model and Some Quantum Critical Points

  • 2. Method and Some Results

Renormalized Perturbation Theory and Numerical Renormalization Group Application to Single Impurity Anderson Model Application to Two Impurity Anderson Model

  • 3. Results and Discussion

Luttinger –Friedel sum rule Violation of Luttinger-Friedel sum rule Discussion

  • 4. Summary and Conclusion
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Model and Systems

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Quantum dot High-Tc superconductor (Cuprate: YBa2Cu3O7-δ)

BaO BaO CuO2 CuO2 CuO CuO Y

General Background

Dilute magnetic alloys (Kondo effect) Au Mn Scanning tunneling microscopy (STM) Au Co Co

Single Impurity Anderson Model ( SIAM )

continuous energy levels (non-interacting system) hybridization discrete energy level + interaction

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Model

AM 1 AM 2

Two-Impurity Anderson Model (2IAM)

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QCP1: J QCP2:U12 QCP3:U12

AF J Kondo effect

Some Quantum Critical Points

Positive U12 > U Negative U12 < -|U|

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Method and Some Results

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Logarithmic discretization + Transformation to linear chains

Perturbation expansion in powers of the renormalized interaction parameters (overcounting are avoided) Exact expressions of some physical quantities in terms of the renormalized parameters Fermi liquid state : quasiparticles with residual renormalized interactions

NRG flow NRG flow Numerical Renormalization Group (NRG)

Renormalized Perturbation Theory and Numerical Renormalization Group

Renormalized Perturbation Theory (RPT) General assumption for low energy states (Fermi liquid) NRG flow and NRG fixed point

: A. C. Hewson, Phys. Rev. Lett. 70, 4007 (1993)

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Application to SIAM

  • A. C. Hewson, A. Oguri, and D. Meyer. Eur. Phys. J. B B40 177 2004

U/πΔ = 2 Wavefunction renomarization factor z = Δ~/Δ Renormalized U~ Wilson ratio R = χ/γ Exact (Bethe ansatz) 0.2392 0.2301 1.9620 NRG Λ=2.0 0.2389 0.2298 1.9620 NRG Λ=2.5 0.2390 0.2300 1.9621 NRG Λ=3.0 0.2390 0.2299 1.9619 NRG Λ=3.5 0.2390 0.2299 1.9620 Our method : all parameters (in principle) Parameter space Electron-hole symmetry, D→∞ Bethe ansatz (Exact) : special parameter

Quite good agreement

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Application to 2IAM

Exact expressions of some susceptibilities ( RPT )

Spin susceptibility Charge susceptibility Staggered spin susceptibility Staggered charge susceptibility

For 2IAM, no exact results such a Bethe ansatz solution (so far).

Dimensionless renormalized interaction parameters Quasiparticle density of states

( Nishikawa Y., Crow D. J. G., Hewson A. C., PHYSICAL REVIEW LETTERS 108 ( 056402 ) 2012, PHYSICAL REVIEW B 86 ( 125134 ) 2012 )

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(necessary condition for the assumption) ⇒ one η → 4 and the other η s → 0. At least, one susceptibility diverges because (assumption) At a particular QCP, only one susceptibility associated with the QCP diverges. It enables us to predict the values of the renormalized interaction parameters at the QCP using the following equations.

@QCP

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0.000160 1.999 0.9996 0.000279

  • 0.9995

0.9990

[ Predicted values ]

QCP1(Kondo-AF) QCP2(Kondo-CO)

[ Predicted values ]

AF CO Kondo effect

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  • 0.9999

Our method is reliable for 2IAM.

  • 0.9999

10^-9

[ Predicted values ]

QCP3(Kondo-AP) AP Kondo effect

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Results and Discussion

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Luttinger – Friedel sum rule

Luttinger’s theorem

The volume inside the Fermi surface is invariant by the interaction. (If the number of particles is held fixed.)

Friedel sum rule

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Violation of Luttinger –Fridel sum rule 1

local AF (electron-hole symmetry)

Magnetic field QCP1’

0.5

Unpublished result

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Violation of Luttinger –Fridel sum rule 2

Nishikawa Y., Curtin O. J., Hewson A. C., Crow D. J. G.,PHYSICAL REVIEW B 98 ( 104419 ) 2018

local AF (electron-hole asymmetry)

Magnetic field QCP1’’

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Violation of Luttinger –Fridel sum rule 3

Curtin O. J., Nishikawa Y., Hewson A. C., Crow D. J. G. JOURNAL OF PHYSICS COMMUNICATIONS 2 ( 031001 ) 2018

Kondo effect(electron-hole asymmetry) local AF(electron-hole asymmetry) QCP1 e-h asym

The local AF QCP (QCP1) is robust against parameter perturbations ( magnetic field, electron-hole asymmetry, ( geometric asymmetry ), and some of them )

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Violation of Luttinger –Fridel sum rule 4

QCP magnetic field magnetic field Unpublished result

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Discussion

1. Long-lived quasiparticle excitation at the Fermi level

  • 2. Adiabatic continuous

Constant in a phase Quantized [ Luttinger integral ] Luttinger integral as a Topological invariant ・ characterizing the two Fermi liquid phases ・ induced by electron correlations Robustness of the QCP against some perturbations

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For example, in the paper by M. Oshikawa ( PHYSICAL REVIEW LETTERS 84 (3370) 2000 ) ,

“ Luttinger’s theorem might be actually the first example of the topological quantization discovered in quantum many-body problem… ” “Luttinger's theorem perhaps does not look like a quantization, because the volume of the Fermi sea takes continuous values depending on the particle density. However, the insensitivity to the interaction resembles other quantization phenomena, …” “ In fact, it is not clear whether a Fermi liquid which violates Luttinger’s theorem can exist. ” “… the topological understanding has been missing for a long time. ”

⇒ ● (Local) Fermi liquid states violating Luttinger’s theorem ( Luttinger-Friedel sum rule).

  • Deviations from Luttinger-Friedel sum rule are quantized.

(Nishikawa Y., Curtin O. J., Hewson A. C., Crow D. J. G.,PHYSICAL REVIEW B 98 ( 104419 ) 2018, Curtin O. J., Nishikawa Y., Hewson

  • A. C., Crow D. J. G. JOURNAL OF PHYSICS COMMUNICATIONS 2 ( 031001 ) 2018)

⇒ Winding number for finite systems ( K. Seki, S. Yunoki, PHYSICAL REVIEW B 96 (085124)2017 ) → consistent with our results and proposal

(See also, G. G. Blesio, L. O. Manuel, P. Roura-Bas, A. A. Aligia, PHYSICAL REVIEW B 98 (195435) 2018)

Luttinger’s theorem…. something topological…

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Related experiment : heavy fermion system

Philipp Gegenwart, Qimiao Si, Frank Steglich, Nature Physics volume 4, 186–197 (2008)

http://www2.cpfs.mpg.de/~wirth/rec/stm4.html

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Summary and Conclusion

  • Quantum criticality in two impurity Anderson model
  • Method : RPT and NRG
  • Violation of Luttinger-Friedel sum rule in some Fermi liquid states
  • Luttinger integral as a topological invariant

Characterizing the two fermi liquid phases separated by the QCP Induced by electron correlations

  • Related experiment on a heavy fermion metal, YbRh2Si2

Thank you for your attention.