A biochemical way to oxidize alcohols: Alcohol dehydrogenase H H H - - PowerPoint PPT Presentation

a biochemical way to oxidize alcohols alcohol
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A biochemical way to oxidize alcohols: Alcohol dehydrogenase H H H - - PowerPoint PPT Presentation

A biochemical way to oxidize alcohols: Alcohol dehydrogenase H H H + ENZ :B ENZ H NAD + NAD + + + + H B H 3 C O H 3 C O H R + N H 2 N O H H H 3 C O H : B Enzyme The enzyme, :BENZ, has a basic functional group in


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SLIDE 1

A biochemical way to oxidize alcohols: Alcohol dehydrogenase

N

+

R N H2 O C H3 O H H H B Enzyme : C H3 O H H H :B ENZ C H3 O H B

+ ENZ

H H NAD + NAD+ + + +

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SLIDE 2

The enzyme, :B–ENZ, has a basic functional group in proximity to where ethanol will bind

B Enzyme :

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SLIDE 3

There also is a binding site for NAD+

N

+

R N H2 O B Enzyme :

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SLIDE 4

When the alcohol binds in the acitve site of the enzyme, an elimination reaction can proceed

N

+

R N H2 O C H3 O H H H B Enzyme :

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SLIDE 5

Deprtonation by the base

N

+

R N H2 O C H3 O H H H B Enzyme :

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SLIDE 6

allows for C=O double bond formation

N

+

R N H2 O C H3 O H H H B Enzyme :

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SLIDE 7

the formal leaving group is H-, a hydride, which can be added to NAD+

N

+

R N H2 O C H3 O H H H B Enzyme :

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SLIDE 8

with allylic rearrangement of the pi electon system

N

+

R N H2 O C H3 O H H H B Enzyme :

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SLIDE 9

to quench the formal positive change of nitrogen . . .It’s an E2-type elimination reaction!

N

+

R N H2 O C H3 O H H H B Enzyme :

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SLIDE 10

N R N H2 O H C H3 O H B

+ Enzyme

H .. C H3 O H H H :B ENZ C H3 O H B

+ ENZ

H H NAD + NAD+ + + +