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TRIUMF Summer Institute, 2015 Precision Measurements of Nuclear Masses Klaus Blaum 113 th -25 th July 2015 Klaus.blaum@mpi-hd.mpg.de Content Motivation for precision mass data 1 Production of short-lived exotic ions 2 How to weigh an


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Klaus.blaum@mpi-hd.mpg.de

TRIUMF Summer Institute, 2015 “Precision Measurements of Nuclear Masses”

Klaus Blaum 113th-25th July 2015

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Content

1 3 4

Motivation for precision mass data How to weigh an atom Nuclear structure and astrophysics

5

Tests of fundamental symmetries

2

Production of short-lived exotic ions

6

Neutrino physics applications

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Some useful literature

Books and review articles:

L.S. Brown and G. Gabrielse: Physics of a single electron

  • r ion in a Penning trap; Rev. Mod. Phys. 58, 233 (1986)
  • G. Bollen: Traps for Rare Isotopes,

Lecture Notes in Physics, 651, 169-210 (2004) F.G. Major et al.; Charged Particle Traps, Volume I and II Springer, Vol. 37, Berlin (2005)

  • K. Blaum: High-accuracy mass spectrometry with stored ions,
  • Phys. Rep. 425, 1-78 (2006)
  • J. Äystö: Overview of recent highlights at ISOL facilities,
  • Nucl. Phys. A 805, 162c-171c (2008)
  • K. Blaum et al.: Precision atomic physics techniques for nuclear physics

with radioactive beams; Physica Scripta T152, 014017 (2013)

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1 Atomic masses: Motivation

E = mc2

mn,p ≈ 1 GeV/c2 = 1.000.000.000 eV/c2 ≈ 0,0000000000000000000000000017 kg

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H2 C60

(nuclear) astrophysics, astrochemistry, production of heavy elements, atomic and molecular binding energies

Fields of applications

nuclear structure, nuclear forces

T C P

fundamental interactions and their symmetries, fundamental constants

particle antiparticle

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Atomic and nuclear masses

MAtom = N•mneutron + Z•mproton + Z•melectron

  • (Batom + Bnucleus)/c2

= N · – binding energy + Z · + Z ·

Masses determine the atomic and nuclear binding energies reflecting all forces in the atom/nucleus.

δm/m < 10-10 δm/m = 10-6 – 10-8

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Why measuring atomic masses?

δm/m General physics & chemistry ≤ 10-5 Nuclear structure physics

  • separation of isobars

≤ 10-6 Astrophysics

  • separation of isomers

≤ 10-7 Weak interaction studies ≤ 10-8 Metrology - fundamental constants Neutrino physics ≤ 10-9 CPT tests ≤ 10-10 QED in highly-charged ions

  • separation of atomic states

≤ 10-11

N · – binding energy + Z · + Z ·

Sources: Accelerator or reactor based radioactive beam facilities and electron beam ion traps. CERN IMP/GSI MPIK TRIGA

KATRIN-TRAP TRIGA-TRAP THe-TRAP PENTA-TRAP Experimental setups CSRe/ESR ISOLTRAP/TITAN SHIPTRAP

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The liquid drop model

2 3 / 1 3 / 4 2 2 3 / 1 ,

) ( 5 3 / I A a a A Z r e A a a A E

OberfSymm Symm Oberf Vol Kern B − − −

+ + + + =

A = N + Z, neutron number N, proton number Z and elementary charge e Nuclear Radius: R ≈ r0A1/3 Symmetry: I2 = (N – Z)2/A2

Volume Surface Coulomb Symmetry Parity

  • C. F. v. Weizsäcker, Zeitschrift der Physik, 96, 431 (1935)
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Comparison Bnucl: Theory-experiment

Nuclear structure effects like shell closures become visible.

1949: The shell model and magic numbers (Göppert-Mayer + Jensen).

Nuclear structure effects like shell closures become visible.

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Test of nuclear mass models

Cs (Z=55)

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2 Production of short-lived exotic ions

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Radioactive ion beam production

nuclear reaction Primary beam Secondary beam

I0 IRIB

Reaction rate

C i 1 b 10 b

ion beam preparation, separation, acceleration/deceleration, ...

Principle

R = σreaction · φprimary · Ntarget

Cross sections 1 pb – > 10 b Beam flux 1011 – 1015 /cm2 /s Target thickness 0.1 – 100 g/cm2

RIB intensity

IRIB = ε · R ε = f ( )

Transmission, element, half-life, ionization, ...

0.1 / day - > 1012 / s

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Proton-induced reactions (ISOLDE, ISAC)

protons p n + Spallation + + Fragmentation + + Fission

201Fr 11Li

X

143Cs

Y

238U

1 GeV

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before

Protons 8 V 500 A 9 V 1000 A

http://isolde.web.cern.ch/isolde

  • E. Kugler, Hyp. Int. 129, 23-42 (2000).

after

ISOLDE target

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Target- station 1 GPS Target- station 2 HRS

ISOLDE target robots

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Ionization possibilities

H Li Na Be Mg Cs Rb K Fr Ba Sr Ca Ra La Y Sc Ac Hf Zr Ti Rf Ta Db W Sg Re Bh Os Hs Ir Mt Pt Ds Au Rg Hg

112

Al Tl Si Pb P Bi S Po Cl At Nb V

Mo

Cr

Tc

Mn

Ru

Fe

Rh

Co

Pd

Ni

Ag

Cu

Cd

Zn In Ga

Sn

Ge

Sb

As

Te

Se I Br

Xe

Kr Ar Rn B C N O F Ne He Th Ce

Pa

Pr U Nd

Np

Pm

Pu

Sm

Am

Eu

Cm

Gd

Bk

Tb

Cf

Dy

Es

Ho

Fm

Er

Md

Tm

No

Yb

Lr

Lu

+ SURFACE –

hot PLASMA cooled

LASER ION SOURCE:

113 114 115 ~80 elements ~1300 isotopes

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ISOL: Isotope Separation On-Line

ISOL principle

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3 How to weigh an atom

νc,2 νc,1 νc,1 νc,2

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How to weigh atoms/ions?

By capturing and storing of ions and comparing with other masses! Nobel Prize in Physics in 1989 to Hans Dehmelt und Wolfgang Paul „for the development of the ion trap technique“.

Wolfgang Paul (1913 - 1993) Hans Dehmelt (1922 - ... )

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SLIDE 20 Electron cooler Gas-target Quadrupole- triplet Septum- magnet Dipole magnet Fast kicker magnet RF-Accelerating cavity Hexapole- magnets From the FRS Extraction To the SIS Quadrupole- dublet Schottky pick-ups

Storage and cooling techniques

particles at nearly rest in space relativistic particles ∗ ion cooling ∗ long storage times ∗ single-ion sensitivity ∗ high accuracy

Storage ring

ESR

0 2.5 5 m

Penning trap

0 0.5 1 cm

z

r

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The Penning trap

  • Trapping of particle via motion in em field
  • Strong homog. magnetic field in z direction,

particle moves with cyclotron frequency → bound in radial direction

  • Weak, electrostatic quadrupole potential
  • Equations of motion in 3D:

z c

B m q = ω

) ( 2 ) , (

2 2 1 2 2

ρ ρ − = z d U z V

DC

F = −e0(∇φ(r) + v × B) + mr = 0

··

) 2 (

2 2 2 1 2

ρ + = z d

Geometry parameter
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Equation of motion in a Penning trap

F = −e0∇φ(r) + v × B

plus Lorentz force: equation of motion:

F = −e0(∇φ(r) + v × B) + mr = 0

··

axial oscillation

2

2

= + ⋅ z m z md U e  

m z = 0 ··

2

2 md U e

z =

ω z or axial frequency radial oscillation

2 4 2

2 2 z c c

ω ω ω ω − + =

+

2 4 2

2 2 z c c

ω ω ω ω − − =

modified cyclotron frequency magnetron frequency

iy x u + =

B m e

c

= ω

( )

t i

e u t u

ω −

= u u 2 u i

2 z c

= + ω − ω   

substitution:

·

u -

·

u =

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Storage of ions in a Penning trap

Ion q/m Charge q Mass m

U

B

The free cyclotron frequency is inverse proportional to the mass of the ions!

m qB

c

/ = ω

L.S. Brown, G. Gabrielse, Rev. Mod. Phys. 58, 233 (1986).

  • K. Blaum, Phys. Rep. 425, 1 (2006).

ωc

2 = ω+ 2+ω- 2+ωz 2

ωc = ω+

+ ω-

An invariance theorem saves the day:

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End of lecture 1

What did we learn? 1) Motivation for precision mass data 2) Liquid drop model and nuclear binding energy 3) Production of radioactive ions 4) Storage of charged particles 5) Penning trap technique What comes next? 1) Manipulation of stored ions 2) Frequency measurement techniques 3) Experimental setup 4) Applications of precision nuclear mass data * Nuclear physics and astrophysics