Thesis defense Excitations in topological superfluids and - - PowerPoint PPT Presentation

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Thesis defense Excitations in topological superfluids and - - PowerPoint PPT Presentation

Thesis defense Excitations in topological superfluids and superconductors Hao Wu Supervisor: James A. Sauls Northwestern University December 3, 2016 DMR-1106315 Introduction superconductivity and superfluidity Heike Onnes: superconductor


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SLIDE 1

Thesis defense

Excitations in topological superfluids and superconductors

Hao Wu Supervisor: James A. Sauls

Northwestern University

December 3, 2016 DMR-1106315

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SLIDE 2

Introduction – superconductivity and superfluidity

Heike Onnes: superconductor & liquid helium

”Mercury has passed into a new state, which on account of its extraordinary electrical properties may be called the superconductive state” – Onnes 1911 ”his investigations on the properties of matter at low temperatures which led, inter alia, to the production of liquid helium” – Nobel prize committee 1913

Superconductivity – zero conductivity, Meissener effect Ginzburg-Landau

Complex order parameter Ψ Gauge symmetry breaking U(1)

Bardeen-Cooper-Schrieffer (BCS) theory

Electron-phonon interaction Cooper pair – Bound state of electrons |p,"i,|p,#i

I Fermi statistics I attractive interaction

Bogoliubov quasiparticles (u(p),v(p))T

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SLIDE 3

Introduction – superconductivity and superfluidity

Superfluid 4He – frictionless flow, quantized vortices

Bose-Einstein condensation: macroscopically occupied ground state Gauge symmetry breaking

Superfluid 3He

Anisotropic Cooper pair of 3He atoms

I Repulsive interaction non-swave I Spin susceptibility spin-triplet pairing

Attractive interaction – spin exchange Unconventional superfluid

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SLIDE 4

Spin-Triplet, P-wave Pairing - Superfluid Phases of 3He Symmetry Group of Normal 3He : G = SO(3)S ⇥SO(3)L ⇥U(1)N ⇥P⇥T Phase Diagram of Bulk 3He

0.0 0.5 1.0 1.5 2.0 2.5 T [mK] 5 10 15 20 25 30 P [bar]

A B

PCP

3He

Superfluid

Spin-Triplet, P-wave Order Parameter : ∆αβ (p) =~ d(p)· (i~ σσy)αβ dµ(p) = Aµi pi Chiral ABM State ~ l = ˆ m⇥ ˆ n Aµi = ∆ ˆ dµ ( ˆ m+iˆ n)i Lz = 1 , Sz = 0 “Isotropic” BW State Aµi = ∆δµi J = 0 , Jz = 0

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SLIDE 5

Symmetry and topology of superfluid phases Nambu-Bogoliubov Hamiltonian for 3He-A : b H = ✓ ξ(p) c(px ±ipy) c(px ⌥ipy) ξ(p) ◆ = ~ m(p)·b ~ τ I Symmetry: C⇥U(1)N + L I Topological Invariant G.E. Volovik, JETP 67(9), 1804-1811 (1988): N2D = π

Z

d2p (2π)2 ˆ m(p)· ✓ ∂ ˆ m ∂ px ⇥ ∂ ˆ m ∂ py ◆ = ±1 Nambu-Bogoliubov Hamiltonian for 3He-B : b H = ξ(p)b τ3 +cp· ˆ σb τ1 I Symmetry: C⇥T⇥SO(3)L+S I Topological Invariant G.E. Volovik, JETP Lett. 90: 398 (2009): N3D =

Z

d3p 24π2 εi jk Tr n Γ( b H1∂pi b H)⇥( b H1∂pj b H)( b H1∂pk b H)

  • = 2,

Γ = CT Bulk-edge correspondence I Nontrivial bulk topology gapless boundary states I Bogoliubov quasiparticle, particle-hole mixing Majorana Fermion

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SLIDE 6

Superfluid in confined geometry

Porous medium – aerogels Phase diagram

  • J. Pollanen et al., Nature Physics 8, 317-320 (2012)

Polar phase

  • V. Dmitriev et al., PRL 115, 165304 (2015)

Slab geometry

  • L. Levitin et al., Science 340, 841-844 (2013)
  • A. Vorontsov and J. A. Sauls, PRL 98, 045301 (2007)
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SLIDE 7

Confinement induced inhomogeneous superfluid phase

Missing Stripe phase

L. Levitin et al., Science 340, 841-844 (2013)

Exist in slab geometry

  • A. Vorontsov and J. A. Sauls, PRL 98, 045301 (2007)

Exist with diffusive surface

  • K. Aoyama, arXiv:1605.07302 (2016)

Generic phenomena, in cylinders

  • K. Aoyama, PRB 89, 140502 (2014)
  • J. Wiman and J. A. Sauls, to be published (2016)

Strong-coupling effect

  • J. Wiman and J. A. Sauls, JLTP 184, 10541070 (2016)

Chiral stripe phase

  • H. Wu and J. A. Sauls, to be published (2016)

I Periodic chiral domain walls (PDW) I Competing phases – Polar, PDW, ABM

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SLIDE 8

Chiral superconductivity

Chiral superconductors Complex order parameter: ∆(p) = |∆(p)|eiφ(p) Phase winding:

I

Cp

dφ(p) = n⇥2π Time reversal symmetry breaking Nontrivial bulk topology – b H = ~ m(p)·b ~ τ ∆(p) = ∆(px +ipy) Majorana Fermions Chiral Weyl Fermion Spontaneous charge current Half quantum vortex Phase vortex + d-vector rotation Non-abelian statistics quantum computing

ϕ=0 ϕ=π ϕ=3π/4 ϕ=π/2 ϕ=π/4

  • D. Ivanov, PRL 86, 268 (2001)
  • J. Jang et al., Science 331, 186-188 (2011)
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SLIDE 9

Is Sr2RuO4 a chiral superconductor? Sr2RuO4 Tc = 1.15K Evidence for chiral superconductivity I Spin triplet pairing S = 1 NMR I Broken time reversal symmetry I Two dimensional E1u representation, px ±ipy Evidence against chiral superconductivity I Missing edge current I No second transition Kerr rotation

cooled in -43 Oe! warmup in ZF

  • J. Xia et al. - PRL 97, 167002 (2006)

Uniaxial strain

  • C. Hicks et al., Science 344, 283-285 (2014)
  • J. Xia et al., PRL 97, 167002 (2006)
  • R. Cava, Chem. Commun. (2005)
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SLIDE 10

Outline Goal : Search for Majorana Fermions Novel superfluid phases under confinement Indentification of chiral superconductor Content :

1

Introduction of quasiclassical theory (Ch 2)

2

Majorana states and currents on superfluid 3He-B (Ch 3-4)

  • H. Wu and J. Sauls, PRB 88, 184506 (2013)

3

Edge spectrum, currents and phase transitions in 3He-A film (Ch 5-6)

  • H. Wu and J. Sauls, to be published (2016)

4

Collective modes and power absoptions in chiral superconductor (Ch 7-8)

  • H. Wu and J. Sauls, to be published (2016)

5

Conclusion (Ch 9)

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SLIDE 11

Elements of quasi-classical theory

Quasiclassical Green’s function: b G(R,p;ε) = ˆ g ˆ f ˜ ˆ f ˜ ˆ g ! , ∆ ⌧ Ef , ¯ h/pf ⌧ ξ0 ... gαβ(R,p) =

Z ϖ

ϖ dξ(p)

Z

dreip·r ⌦ TrΨ(R+r/2)Ψ†(Rr/2) ↵ fαβ(R,p) =

Z ϖ

ϖ dξ(p)

Z

dreip·r hTrΨ(R+r/2)Ψ(Rr/2)i Equilibrium Eilenberger’s transport equation h ε ˆ τ3 b ∆(R,p), b G(R,p;ε) i +i¯ hv(p)·∇R b G(R,p;ε) = 0 Self-consistent equation ˆ ∆(R,p) =

Z

dp0V(p,p0)

Z ϖ

ϖ dε ˆ

f(R,p0;ε) Linear response theory b G(R,p;ε,t) = b G(R,p;ε)eq +δ b G(R,p;ε,t), b ∆(R,p;t) = b ∆(R,p)eq +δ b ∆(R,p;t) p = pf ˆ p

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SLIDE 12

Superfluid 3He-B in a film with width D

D

x y z

3He-B

Bulk 3He-B I Fully gapped E(p) = q ξ 2(p)+∆2 I Helicity eigenstate Surface 3He-B I Gapless Fermions E(p) = ±cpk I Ising spin state

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SLIDE 13

Quasi-classical theory for confined 3He-B

B Phase Order parameter ˆ ∆ = ~ d ·(i~ σσy) dx = ∆k(z)px, dy = ∆k(z)py, dz = ∆?(z)pz, Nambu Green’s function b G(p,z;ε) = g+~ g·~ σ ~ f·(i~ σσy) ˜ ~ f·(iσy~ σ) ˜ g+ ˜ ~ g·~ σ tr ! Eilenberger’s equation h b HA , b G i +i¯ hvp ·∇b G = 0 Andreev Hamiltonian b HA = εb τ3 b ∆ Integrate along trajectories p, p

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SLIDE 14

Green’s function for specular 3He-B surface – Quasiparticle propagator

Quasiparticle Green’s function (Scalar) g = πε p ∆2 ε2 " 1+ ∆2

? cos2 θ

∆2

k sin2 θ ε2 e2 p ∆2ε2z/vz

# Local density of states N (p,z;ε) = 1 π Img(p,z;ε) Quasiparticle Green’s function (Spin vector) ~ g = π∆?∆k sinθ cosθ ∆2

k sin2 θ ε2

e2

p ∆2ε2z/vz~

e2 Local spin density of states ~ S (p,z;ε) = 1 π Im~ g(p,z;ε)

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SLIDE 15

Green’s function for specular 3He-B surface – Cooper pair propagator Anomalous Green’s function fz = π∆? cosθ p ∆2 ε2 " 1e2

p ∆2ε2 z/vz + iε

p ∆2 ε2 ∆2

k sin2 θ ε2 e2 p ∆2ε2 z/vz

# fk = π∆k sinθ p ∆2 ε2 " 1+ ∆? cos2 θ ∆2

k sin2 θ ε2 e2 p ∆2ε2 z/vz

#

1 2 3 4 5 6 z/ξ∆ 0.0 0.2 0.4 0.6 0.8 1.0 1.2

∆k/∆ ∆?/∆ I ξ∆ = vf /2∆ I Supression of pz orbital I Enhancement of pk orbital I Change in length scale ξ∆

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SLIDE 16

Local density of states

ε/∆

2 1 1 2

pk / pf

1.0 0.5 0.0 0.5 1.0 2 4 6

N(p||, ε)

Surface bound states Bound state energy εb = ±cpk, c = (∆k/p f ) Spectral weight π∆? cosθ 2 e2∆?z/vf Continuous spectrum |ε| > ∆ lim

z!∞Nc(p,z;ε) = Nbulk

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SLIDE 17

Spontaneous spin current

Spin spectral function: ~ S = π∆? cosθ 2 [δ(ε +c pk)δ(ε c pk)]e2∆?z/vf ~ e2 Confining length: ξ∆ = vf /2∆? Spin polarized along~ e2 = z⇥p Spectral Spin current: ~ Jα(p,z;ε) = 2Nf vp ⇥ Sα(p,z;ε)Sα(p0,z;ε) ⇤ Time reversal p ! p0: Sα(p,z;ε) = Sα(p0,z;ε), ~ Jα(p,z;ε) = ~ Jα(p0,z;ε) spin current tensor J (p,z;ε)⇥ @ 1 +1 1 A

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SLIDE 18

Surface spin current

−1.0 −0.5 0.0 0.5 1.0

x

−1.0 −0.5 0.0 0.5 1.0

Spin current structure on the surface

Flow direction Spin polarization

y

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SLIDE 19

Spectral spin current density pk = 0.5p f

−2 −1 1 2 1 2 3 4 5 −2 −1 1 2

Fermi Distribution

ε / ∆

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SLIDE 20

Finite temperature spin current

Sheet current – current per unit area K(T) ⌘

Z

dz

Z

dp

Z

dε J (p,z;ε) ' ✓ 1 27πζ(3) 4 T 3 ∆3 ◆ K(0)

0.0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 1.0

T/TC

0.0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 1.0

∆(T)/∆(0) K(T)/K(0) 1 − 27πζ(3)

4 T 3 ∆3

Ground state current: K(0) = 1 6n2Dv f ¯ h/2 Temperature dependence: power law T 3 No static fields couple to spin current

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SLIDE 21

Mass current in a channel

D

ϕ1

ϕ2

~ ps = ~ 2 ~ r'

x y z

Constant phase gradient ˆ

∆(p,r) = ˆ ∆0(p,r)eiϕ(r)

~ ps = ¯ h 2∇ϕ( ~ r) – DC superflow Local Gauge transform ε ! ε ps ·v(p)

1

Solve transport equation, gauge transform back: b g0 g

2

Current response: j(z,T) = Nf

Z

dpπT ∑

εn

g(p,z;εn)

3

Landau molecular field: vMF(p,z) =

Z

dp0 As(p,p0)πT ∑

εn

g(p0,z;εn)

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SLIDE 22

Surface mass current reduction

1.0 0.8 0.6 0.4 0.2 0.0 0.2 0.4 0.6 0.8 1.0

pk/pf

1.0 0.5 0.0 0.5 1.0

εb(p||)/∆|| Dispersion of 3He-B Surface Bound State

εb(p||) = (±∆||/pf vs) ⇥ p|| εb(p||) = ±∆||/pf ⇥ p||

No bound state contribution to zero temperature mass current j(z,0) = nps

D ξ∆

Thermal excitation of gapless states larger reduction at surface Low temperature power law dependence: J(T) = nps(1aT 3) I Surface to bulk ratio D I Fermi-liquid effect – pressure P

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SLIDE 23

Mass flow with Fermi liquid effect

Mass flow at various pressure

0.2 0.4 0.6 0.8 1.0 1.2 1.4 1.6 1.8 2.0 2.2 2.4 2.6

T [mK]

0.0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 1.0

ρs/ρ

Total Mass Current at P = 34 bar Bulk Mass Current at P = 34 bar leading order correction ∼ T 3

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SLIDE 24

Two dimensional superfluid A phase Topological superfluid b H = ~ m·b ~ τ ~ m = (∆px,∆py,ξ(p)) Detection of edge current – transverse mobility

  • H. Ikegami et al., Science 341(6141), 59-62 (2013)
  • O. Shevtsov and J. Sauls, PRB 94, 064511 (2016)

Edge state: gapless Weyl fermion

1.0 0.5 0.0 0.5 1.0 pk/pf 1.0 0.5 0.0 0.5 1.0 ε(pk)∆

  • ccupied

empty

ε(pk) = c pk

continuum

Spontaneous ground state current j(x) = Nf vf ∆ex/ξ∆

J1 J2 D 3He-A

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SLIDE 25

Confined geometry D ! 10ξ0

Main focus: Hybridization of bound fermions at opposing edges New ground states in confinement superfluid film

Chiral A-Phase order Parameter ∆(p) = ∆?(x)px +i∆k(x)py Specular reflection at both edges px = px, py = py Spatial dependent gap amplitudes ∆?(0) = ∆?(D) = 0

∆ ˆ p ˆ p

1 2 3 4 5 6 7 8 9 10 11 12

x/ξ0

0.0 0.1 0.2 0.3 0.4

∆bulk ∆k(x) ∆?(x)

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SLIDE 26

Quasiclassical wave function – Andreev’s Equation

Andreev’s Equation b HA |Ψ(r;p)i+i¯ hvp ·∇|Ψ(r;p)i = 0 |Ψi = (u,v)T b HA = εb τ3 b ∆ Boundary condition

Ψ(0,y;p) = Ψ(0,y;p) Ψ(D,y;p) = Ψ(D,y;p)

Bloch wave solution

Ψ(x,p) = eikx ¯ Ψ(x,p)

Bound state dispersion

ε(p,k)2 = ∆2p2

y +∆2p2 x(1cos(2kD))/(cosh(2λD)cos(2kD))

with

λ = p ∆2 ε2 x = 0 x = 2D ∆?px +i∆kpy x = −2D x = 4D ∆?px +i∆kpy 2D

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SLIDE 27

Bound state under confinement – local spectrum at x = D

1.0 0.5 0.0 0.5 1.0 pk/pf 1.0 0.5 0.0 0.5 1.0 ε/∆ 4 8 12 16 20 24 28 32 36 40

∆?px +i∆kpy x = D x = 0

ε(pk) = c pk

continuum

ε(pk) = cpk

continuum

I Energy band at each pk I Van Hove singularities

−1.0 −0.5 0.0 0.5 1.0

ε/∆

2 4 6 8 10

N(ε)/N0

Van Hove Singularity normal incidence py = px(45o)

ε2 = ∆2p2

y +∆2p2 x/cosh(λD)2

ε2 = ∆2p2

y

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SLIDE 28

Continuum spectrum under confinement – band structure at x = D

1.0 0.5 0.0 0.5 1.0 pk/pf 4 2 2 4 ε/∆ 4 8 12 16 20 24 28 32 36 40 Band gap in continuum Band gap: largest pk = 0 smallest pk = pf Van Hove sigularities

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SLIDE 29

0.0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 1.0 T[Tc] 0.0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 1.0 J[n¯

h 4 ]

D = ∞ D = 15ξ0 D = 12ξ0 D = 11ξ0 D = 10.4ξ0 D = 10ξ0 D = 9.75ξ0 D = 9.6ξ0

Edge currents

∆?px +i∆kpy x = D x = 0

D/2

J(T) =

Z D/2

dx jy(x;T)

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SLIDE 30

Edge currents

0.0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 1.0 T[Tc] 0.0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 1.0 J[n¯

h 4 ]

D = ∞ D = 15ξ0 D = 12ξ0 D = 11ξ0 D = 10.4ξ0 D = 10ξ0 D = 9.75ξ0 D = 9.6ξ0

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SLIDE 31

Phase Diagram I – Polar to A phase transition

6 8 10 12 14 16 18 20 D/ξ0 0.0 0.2 0.4 0.6 0.8 1.0 T/Tc

Polar Chiral

D = 9.75ξ0

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SLIDE 32

Linear instability analysis Instability in polar phase ∆(p,x,y) = i∆kpy + A31(x,y)px +A32(x,y)py

I Pertubative term ∆1(p,r) in orbital basis

Eigenvalue equations for fourier component ∆1(p,Q)

greens function:

ωm = q ∆2

k +ε2 m

f1(p,Qx,Qy) = ∆1(p,Qx,Qy)πωm/ ⇣ ω2

m +

  • vp ·Q

2 /4 ⌘ self-consistency: ∆1(p,Qx,Qy) =

Z

dp0V(p,p0)T

εm<ωc

εm

f1(p0,Qx,Qy;εm)

The smallest D for nonvanishing ∆1 Qy(T) ⇠ π/15ξ0 – single mode instability

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SLIDE 33

Phase diagram II – polar to periodic domain wall(PDW) phase transition

6 8 10 12 14 16 18 20

D/ξ0

0.0 0.2 0.4 0.6 0.8 1.0

T/Tc

Polar Chiral PDW

Dc2 Dc1

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SLIDE 34

Phase diagram II – polar to periodic domain wall(PDW) phase transition

6 8 10 12 14 16 18 20

D/ξ0

0.0 0.2 0.4 0.6 0.8 1.0

T/Tc

(10.5, 0.7) Polar Chiral PDW

Dc2 Dc1

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SLIDE 35

Self-consistent PDW order parameter T = 0.7Tc,D = 10.5ξ0, ∆ = ∆?px +∆kpy Base state pure polar ∆0 = i∆py Small (104) random fluctuations |∆?|

0.4 0.8 1.2 ⇥104

|∆k|

0.02 0.10 0.20 30 15 15 30

x[ξ0]

5 10

y[ξ0] cos(φ?)

1.0 0.5 0.0 0.5 1.0

cos(φk)

3 3 ⇥104

Self-Consistent calculation ∆?(r),∆k(r) ∆(r,p) = ∆?(r)px + ∆k(r)py h d HA , b G(r,p;εm) i + i¯ hvp · ∇b G(r,p;εm) = 0

∆(r,p) = T ∑

m Z

dp0 v(p,p0)f(r,p0;εm)

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SLIDE 36

Self-consistent PDW order parameter T = 0.7Tc,D = 10.5ξ0, ∆ = ∆?px +∆kpy

|∆?|

0.02 0.04 0.06 0.08

|∆k|

0.269 0.271 0.273 30 15 15 30

x[ξ0]

5 10

y[ξ0] cos(φ?)

1.0 0.5 0.0 0.5 1.0

cos(φk)

0.15 0.05 0.05 0.15

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SLIDE 37

Self-consistent PDW order parameter T = 0.7Tc, ∆ = ∆?px +∆kpy D = 10.5ξ0

−0.08 0.00 0.08

∆1,R 2πTc

−0.05 0.00 0.05

∆2,R

−0.0003 0.0000 0.0003

∆1,I

center edge

−30 −20 −10 10 20 30

y/ξ0

0.267 0.270 0.273

∆2,I

px + ipy px + ipy −px + ipy

D = 11.5ξ0

−0.1 0.0 0.1

∆1,R 2πTc

−0.10 −0.05 0.00

∆2,R

center edge

−0.001 0.000 0.001

∆1,I

−30 −20 −10 10 20 30

y/ξ0

0.26 0.27

∆2,I

px + ipy −px + ipy

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SLIDE 38

Dc1 comparing free energy

Competing phases:

I Homogeneous A-phase I Chiral domain wall

Free energy functional – Luttinger-Ward ∆Ω[b G,b ∆] = 1 2

Z 1

0 dλSp0 n

b ∆(b Gλ b G)

  • +∆Φ[b

G]

Self-consistent order parameter b ∆(D,T) auxiliary propagator b Gλ Integration over space, momentum, energy and λ

Find the critical D(T) at which ∆ΩDW < ∆ΩA

6 8 10 12 14 16 18 20 D/ξ0 0.0 0.2 0.4 0.6 0.8 1.0 T/Tc Polar Chiral PDW

Dc2 Dc1

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SLIDE 39

Difference in free energy density D = 15ξ0,T = 0.5Tc y/ξ0

−20 −15 −10 −5 5 10 15 20

x/ξ0

2 4 6 8 10 12 14 −1.0 −0.5 0.0 0.5 1.0

∆ΩDW − ∆ΩA

×10−3

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SLIDE 40

Phase diagram III – PDW to chiral phase transition, comparing free energy

6 8 10 12 14 16 18 20 D/ξ0 0.0 0.2 0.4 0.6 0.8 1.0 T/Tc

Polar Chiral PDW

Dc2 Dc1

slide-41
SLIDE 41

Phase piagram III

6 8 10 12 14 16 18 20 D/ξ0 0.0 0.2 0.4 0.6 0.8 1.0 T/Tc

Polar Chiral PDW

Dc2 Dc1 Broken symmetry I time reversal I translational

slide-42
SLIDE 42

Phase diagram III

6 8 10 12 14 16 18 20 D/ξ0 0.0 0.2 0.4 0.6 0.8 1.0 T/Tc

Polar Chiral PDW

time reversal ⇥ half lattice translation Dc2 Dc1

slide-43
SLIDE 43

Phase diagram III

6 8 10 12 14 16 18 20 D/ξ0 0.0 0.2 0.4 0.6 0.8 1.0 T/Tc

Polar Chiral PDW

D PDW D 3He-A

Dc2 Dc1

slide-44
SLIDE 44

Superconducting Bosonic modes – eigenmodes for order parameter fluctuation

Conventional superconductor ∆ = |∆|eiφ I Higgs mode – amplitude fluctuation ω = 2|∆|

  • R. Sooryakumar and M. Klein, PRL 45, 660 (1980)

I Bogoliubov mode – phase fluctuation ω = 0 Unconventional pairing, e.g. 3He ˆ ∆ = ~ d(p)·(i~ σσy)

VOLUME 45, NUMBER 4

PHYSICAL REVIEW LETTERS

28 JUx,v 1980 two 20-MHz fundamental

transducers separated

by 0.318 cm." This combination allowed meas-

urements at 10, 20, 30, 50, and 60 MHz. Both

cells were in good thermal contact with a lantha-

num-diluted cerium-magnesium-nitrate ther mom-

eter whose susceptibility

was monitored

by a SQUID detection

system. The thermometer

was

calibrated against 7, as a function

  • f pressure

with the Pt Helsinki scale." The detection

scheme used in the experiment is described

in detail else-

  • where. " Briefly,

we used a phase-sensitive

sys-

tem capable of resolving both the in- and out-of- phase components

  • f the received

sound signal,

relative to a stable reference signal operating

in a phase-locked loop fixed at the drive frequen-

  • cy. The gain of the system was independent
  • f

phase to within 3-4P& The sound attenuation

and

phase velocity shift,

bc, were obtained

from the changes

  • f the signal amplitude

and phase,

re-

spectively.

As an overall check on all of our measurements, we have selectively compared the data obtained using the phase-sensitive

sys-

tem to that obtained from a non-phase-sensitive detector and a boxcar integrator. The attenua- tion data showed

no dependence upon the detec-

tion scheme used,

as long as the variation

in c was less than -1%. With larger changes in c, the

phase-sensitive

method becomes less reliable

because of changes

in the resonant frequency

  • f

the transducers, and for these cases, the data were obtained by our second method. In Fig. 1, we show the attenuation

  • f 60-MHz

zero sound versus reduced temperature, at a pressure

  • f 5.3 bars.

The peak location of the main attenuation feature near T, cannot be deter- mined because of loss of the signal in this region, but we have marked the expected position

  • f the

collective-mode peak as predicted

by Eq. (1), as well as the pair-breaking

cutoff temperature, using the Ginzburg-Landau expression for the en- ergy gap:

  • 2 ~g

Z (T) =mt

Tc

C

where 6C/C„ is the specific heat jump at T„ which was taken from the recent measurements by the Alvesalo et al." The main attenuation peak is observed to split into two parts, in agree- ment with earlier observations by Paulson and W'heatley. The new feature, marked

y, is completely un-

expected and, to our knowledge, not previously

  • bserved.

This extraordinarily narrow attenua- tion peak was observed at 30, 50, and 60 MHz,

l5-

.

/12/5h .. 2b, . E

l0-

5-

I-

CI

20jd&

I

0.6

I I

0.8 0.9

~ ~ ~ ~

l.o

  • FIG. 1. Relative

attenuation

  • f 60-MHz sound at 5.3

bars.

Arrows

show the predicted

location of the collec- tive-mode

and pair-breaking attenuation

peaks.

The height of the p peak is not known because of loss of the signal for relative attenuation &16 cm '.

h(u =Ass(T «),

(3) where

A is a constant and 6~(T) is given by Eq.

(2). In Table I, we give the values

  • f the y peak

location relative to T„as well as the values"

  • f AC/C„used

to calculate

A from the data. The

depending

  • n pressure.

At each pressure,

there

is a characteristic

frequency above which this fea- ture can be resolved. This presumably

results from the combined effect of the variation

with frequency

  • f the location in temperature
  • f the

y feature and the broadening

near T, of the main attenuation peak, whose width depends

  • n the

ratio h~/r,

where

7 is the quasiparticle

lifetime

at the Fermi surface (-10-' sec).' Thus, at too

low frequencies

the expected position in tempera-

ture of the y feature falls within

the region of high attenuation, where it cannot be resolved. As the pressure

is lowered,

the height

  • f this peak

(for a constant frequency) increases

and its width in temperature

decreases.

This decrease of

width is expected if the broadening

is due to quasi- particle

lifetime effects. Using the phase-sensi- tive detection scheme,

we also observe a sound-

velocity change at the y peak. In Fig. 2, we show both the sound attenuation and the velocity shift in the vicinity

  • f this feature.

The velocity change

is superimposed

  • n a smooth variation
  • f c which

is observed'

at temperatures

below the main attenuation

peak.

In the absence of any prediction

for this fea- ture,

we have tried to characterize

it in the most

  • bvious

way, which is to assume 263

Sound attenuation, J = 2+

  • R. Giannetta et al., PRL 45, 262 (1980)

Acoustic Faraday effect, J = 2+

  • Y. Lee et. al., Nature 400, 431-433 (1999)
slide-45
SLIDE 45

Fermi surfaces and pairing models for Sr2RuO4 ARPES Fermi Surface

ARPES

  • A. Damascelli et al., PRL 85, 5194 (2000)

0.0 0.5 1.0

φ/π

0.0 0.5 1.0 1.5

|∆(p)|/∆

κ = 0.00 κ = 0.20 κ = 0.40 κ = 0.60 κ = 0.80 κ = 1.00

S = 1, p-wave Cooper Pairs (E1u) ⇡ 2D Fermi surface (γ-band)

  • T. M. Rice and M. Sigrist, J. Phys. Cond. Mat. 7(47) (1995)

~ d(p) = ˆ d

  • Ax ˆ

px +Ay ˆ py

  • Anisotropic E1u Cooper Pairs:
  • Q. H. Wang et. al., EPL 104(1) (2013)
  • T. Scaffidi et al., PRB 89, 220510 (2014)

ˆ px ! Yx(p) = ˆ px I(p) ˆ py ! Yy(p) = ˆ py I(p) I( ˆ px, ˆ py) invariant under D4h I(p) = 1+κ

  • |2 ˆ

px ˆ py|1

  • 1+4κ(1κ)/π 2κ(13κ/4)

1 2

0  ε  1 I Multi-component order + Anisotropy Spectroscopy of Pairing Symmetry

slide-46
SLIDE 46

Linear responses in chiral superconductors Order parameter (Nambu): b ∆(p) = ✓ ˆ d ·(i~ σσy)∆(p) ˆ d ·(iσy~ σ)˜ ∆(p) ◆ Chiral basis: Y± = Yx ±iYy, equilibrium state ∆(p) ⇠ ∆Y+ Coupling to vector field: b vext = vp ·A(~ q,ω) b τ3 Dynamic gap in chiral basis: d(p) ! ∆(p,~ q,ω) = ∆(p)+d(p,~ q,ω) ∆(p,~ q,ω) = ∆Y+ + D(~ q,ω)Y+ + E(~ q,ω)Y ˜ ∆(p,~ q,ω) = ∆Y + D⇤(~ q,ω)Y + E⇤(~ q,ω)Y+ Current response: d± ⌘ d ± ˜ d δ~ j = Nf

Z

dpf v f (pf ) ⇢ 1+ η2 ω2 η2 (1λ)

  • vext +η ¯

λ

  • ∆Rd i∆Id+

I Fermionic quasiparticle contribution I Bosonic mode contribution

slide-47
SLIDE 47

Dynamical equation for order parameter fluctuation Self-consistent equation for order parameter fluctuations: d(p,~ q,ω) =

Z

dp0V(p,p0)

Z

dε 4πi δfK(p0,~ q;ε,ω) Coupled equations for: d(p) = DY+ + EY , ˜ d(p) = D⇤Y + E⇤Y+

d(p) = 1 2

Z

dp0V(p,p0) ⇢ 1 2 η ¯ λ∆(p0)vext +  γ(p0)+ 1 2(ω2 η02 2|∆(p0)|2)¯ λ

  • d(p0)¯

λ∆2(p0) ˜ d(p0)

  • ˜

d(p) = 1 2

Z

dp0V(p,p0) ⇢ +1 2 η ¯ λ∆⇤(p0)vext +  γ(p0)+ 1 2(ω2 η02 2|∆(p0)|2)¯ λ

  • ˜

d(p0)¯ λ∆⇤(p0)2d(p0)

  • Energy integrals:

η(p) = v(p)·~ q, γ(p0) ' 2/V Tsuneto function: λ(p,ω) ⌘ |∆|2 ¯ λ = |∆(p)|2

Z ∞

|∆(p)|

dε q ε2 |∆(p)|2 tanh ✓ βε 2 ◆ 1 ε2 (ω/2)2

I S.K. Yip and JAS, J. Low Temp. Phys. 86 (1992)

Normal Modes: D± = D±D⇤ E± = i(E ±E⇤)

slide-48
SLIDE 48

Eigen Mode Frequency and Lifetime

Anderson-Bogoliubov (Goldstone) Mode ω2D = 0 Anderson-Higgs Mode (ˆ Y+) ✓ ω2 4λ10∆(T)2 λ00 ◆ D+ = 0 λmn =

I dφ

2π λ(p)Im(p)cosn(2φ)

slide-49
SLIDE 49

Eigen Mode Frequency and Lifetime

Anderson-Bogoliubov (Goldstone) Mode ω2D = 0 Anderson-Higgs Mode (ˆ Y+) ✓ ω2 4λ10∆(T)2 λ00 ◆ D+ = 0 Anderson-Higgs Mode (ˆ Y) ✓ ω2 4∆(T)2λ11 λ00 ◆ E+ = 0 ✓ ω2 4∆(T)2(λ10 λ11) λ00 ◆ E = 0 λmn =

I dφ

2π λ(p)Im(p)cosn(2φ)

slide-50
SLIDE 50

Eigenmode Frequencies and Lifetimes

0.0 0.2 0.4 0.6 0.8 κ 0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4

E+ E− Γ+ Γ− 2∆max 2∆min

slide-51
SLIDE 51

Mode coupling to a transverse EM field

x y

A Λ

EM field parallel to the surface Transverse field in suprconductor

  • q
  • A
  • q
  • A

Polarization [100] direction – gap minimum h (ω +iΓ)2 ω2

E+

i E+ = ie c Λ100 (ω)qv2

f ∆A(q,ω)

Polarization [110] direction – gap maximum h (ω +iΓ)2 ω2

E-

i E = e c Λ110 (ω)qv2

f ∆A(q,ω)

slide-52
SLIDE 52

Superconducting power absorption

Current response δ~ j(q,ω) = K(q,ω)~ A(q,ω), K(q,ω) = Kex(q,ω)+Kmode(q,ω) Joule’s law P(ω) =

Z ∞

0 dxRe

h ~ E⇤(x,ω)·~ j(x,ω) i Power absorption P

S(ω) = 2ω|B0(ω)|2

c

Z dq

2π ImK(q,ω)

  • q2 + 4π

c K(q,ω)

  • 2

P . J. Hirschfeld et al., PRB 40, 10 (1989)

slide-53
SLIDE 53

Power absorption for isotropic κ = 0 chiral superconductor

0.0 0.5 1.0 1.5 2.0 2.5

ω[2∆]

0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4

P[P0]

×10−2

PS Pex I P

S = P ex +P mode ,

P

0 = |B0(ω)|2vf

π I Quasiparticle absorption ω = 2∆ I Collective Mode ω = p 2∆ I Mode dispersion ω2(q) = ω2

E +

v2

f q2

2 narrow peak width

slide-54
SLIDE 54

Power absorption for anisotropic κ 6= 0 chiral superconductor Polarization [100]

0.0 0.5 1.0 1.5 2.0 2.5

[2∆]

0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4

P[P0]

×10−2

2∆min 2∆max

  • A
  • q

0.0 0.5 1.0 1.5 2.0 2.5 [2∆] 0.0 0.2 0.4 0.6 0.8 P[P0] ×10−2

= ME+

2∆min 2∆max

  • A
  • q

Polarization [110]

0.0 0.5 1.0 1.5 2.0 2.5

[2∆]

0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4

P[P0]

×10−2

2∆min 2∆max

  • q
  • A

0.0 0.5 1.0 1.5 2.0 2.5 [2∆] 0.0 0.4 0.8 1.2 1.6 2.0 P[P0] ×10−3

= ME−

2∆min 2∆max

  • q
  • A
slide-55
SLIDE 55

Impurity effect – order parameter and quasiparticle spectrum

Impurity Model – s-wave: nimp, u0 lifetime Γ = ¯ h τ , cross section ¯ s I ¯ s ! 0 weak scattering Born limit I ¯ s ! 1 strong scattering unitary limit

0.1 0.2 0.3 0.4 0.5 0.6 0.7 0.8 0.9 1.0 T/Tc0 0.00 0.05 0.10 0.15 0.20 0.25 0.30 0.35 Γ = 0.00 Γ = 0.05 Γ = 0.10 Γ = 0.15 Γ = 0.20 Γ = 0.25

0.0 0.1 0.2 0.3 0.4 0.5 ε/2πTc0 0.0 0.6 1.2 1.8 2.4 3.0 3.6 4.2 4.8 Γ = 0.02 Born Γ = 0.02 Unitary Γ = 0.1 Born Γ = 0.1 Unitary clean

Isotropic gap κ = 0

0.0 0.1 0.2 0.3 0.4 0.5 0.6 ε/2πTc0 0.0 0.6 1.2 1.8 2.4 3.0 Γ = 0.02 Born Γ = 0.02 Unitary Γ = 0.1 Born Γ = 0.1 Unitary clean

Anisotropic gap κ = 1

slide-56
SLIDE 56

Impurity effect – collective mode spectrum

Γ = 0.02, ¯ s = 0

0.0 0.2 0.4 0.6 0.8 κ 0.0 0.2 0.4 0.6 E+ E− Γ+ Γ− 2∆max 2∆min

Γ = 0.1, ¯ s = 0

0.0 0.2 0.4 0.6 0.8 κ 0.0 0.2 0.4 0.6 E+ E− Γ+ Γ− 2∆max 2∆min

Γ = 0.02, ¯ s = 0

0.0 0.2 0.4 0.6 0.8 κ 0.0 0.2 0.4 0.6 E+ E− Γ+ Γ− 2∆max 2∆min

Γ = 0.1, ¯ s = 0

0.0 0.2 0.4 0.6 0.8 κ 0.0 0.2 0.4 0.6 E+ E− Γ+ Γ− 2∆max 2∆min

slide-57
SLIDE 57

Impurity effect – power absorption

0.0 0.5 1.0 1.5 0.0 0.2 0.4 0.6 0.8 1.0

P[P0]

×10−1

PS Pex

0.0 0.5 1.0 1.5 2.0

ω[2∆]

Isotropic case κ = 0 Γ = 0.02, Left ¯ s = 0, Right ¯ s = 0.9 Born: absorption peak ω = p 2∆ Unitary: large absorption ω ⇠ ∆

0.0 0.5 1.0 1.5 2.0

ω[2∆]

1 2 3 4

P[P0]

×10−2 2∆min 2∆max

PS Pex

Polarization [100]

0.0 0.5 1.0 1.5 2.0

ω[2∆]

1 2 3 4

P[P0]

×10−2 2∆min 2∆max

PS Pex

Polarization [110]

slide-58
SLIDE 58

Summary

Topological superfluid 3He-B Surface Majorana spectrum E(p) = ±cpk Helical spin current Mass current and temperature dependence j(T) = nps(1aT 3) Confined chiral superfluid 3He-A film Fermionic quasiparticle bands under lateral confinement Prediction of new ground state – periodic chiral domain walls Chiral superconductor with anisotropic gap Bosonic modes with opposite chirality to ground state Anisotropic transverse wave power absorption Impurity effects on mode spectrum and power absorption

slide-59
SLIDE 59

Acknowledgement

Supervisor: Prof. James A. Sauls NU Condensed matter group: ... Domestic and international collaborators:

  • Prof. Takeshi Mizushima, Prof. Suk Bum Chung, Prof. Erhai Zhao, Prof.

Anton Vorontsov, Prof. Bill Halperin, Prof. John Saunders, Prof. Jeevak Parpia, Prof. John Davis

slide-60
SLIDE 60

Majorana and Bogoliubov eigenspinor

1

Define projection operator b P± = 1 2 h b 1± b G(p,z;ε) i b P+(): Project a spinor into particle(hole) sector

2

Act on a particular state i.e. Ψ = b P+ 1 T

3

Projected state at energy εb Ψ = u(θ,z) 2π h Ψ(+)δ(ε cpk)+Ψ()δ(ε +cpk) i

slide-61
SLIDE 61

Majorana and Bogoliubov eigenspinor

4

Spinor with bound state energy εb = ±cpk Ψ(+) = Φ+ eiφΦ, Ψ() = Φ+ +eiφΦ Amplitude u(θ,z) = π2∆? cosθ 2 e2∆?z/vf

5

Sz eigenstates Φ± respectively Φ+ =

  • 1

i T , Φ =

  • i

1 T

6

Ψ(±): Eigenstates of spin operator ⌥~ e2 ·~ S

slide-62
SLIDE 62

Majorana and Bogoliubov eigenspinor

4

Spinor with bound state energy εb = ±cpk Ψ(+) = Φ+ eiφΦ, Ψ() = Φ+ +eiφΦ Amplitude u(θ,z) = π2∆? cosθ 2 e2∆?z/vf

5

Sz eigenstates Φ± respectively Φ+ =

  • 1

i T , Φ =

  • i

1 T

6

Ψ(±): Eigenstates of spin operator ⌥~ e2 ·~ S Same spinor as obtained from solving Andreev Equation (K.Nagai et al 2008 , T.Mizushima 2012)

slide-63
SLIDE 63

Selfconsistent spectrum

2 4 6 8

ε and ∆ are in units of Tc N in units of N0 ∆px + i∆py

2 4 6 8 −6 −5 −4 −3 −2 −1 1 2 3 4 2 4 6 8

py = 0 (normal) py = px (45o) px = 0 (grazing)

1 2

∆ = ∆

1 2

∆ = 0.5∆

6 12 1 2

Self-consistent gap

slide-64
SLIDE 64

Confined chiral domain wall

∆?px + i∆kpy

−∆?px + i∆kpy

Lower energy per unit length

  • Y. Tsutsumi, JLTP

, 2014

PDW domain wall

slide-65
SLIDE 65

Confined chiral domain wall

x = D x = 0 ∆?px + i∆kpy

−∆?px + i∆kpy

Lower energy per unit length

  • Y. Tsutsumi, JLTP

, 2014

PDW domain wall Apparent violation of current conservation

slide-66
SLIDE 66

Confined chiral domain wall

x = D x = 0 ∆?px + i∆kpy

−∆?px + i∆kpy

Lower energy per unit length

  • Y. Tsutsumi, JLTP

, 2014

PDW domain wall Apparent violation of current conservation

∆(r,p) = ∆+(r)y+(p)+∆(r)y(p) with y±(p) = px ±ipy

slide-67
SLIDE 67

Local current density

−30 −20 −10 10 20 30

y/ξ0

5 10 15 20

x/ξ0 j(x, y)

slide-68
SLIDE 68

Local current density

−0.2 0.0 0.2 0.4 0.6

jx [Nf(2πTc)m3vf]

x = 10ξ0 x = 5.5ξ0 x = 1.9ξ0 x = 0.0ξ0

−30 −20 −10 10 20 30

y/ξ0

−0.6 −0.4 −0.2 0.0 0.2 0.4 0.6

jy

slide-69
SLIDE 69

Normal state power absorption

1 2 3 4 5 6 ω[vf/Λ] 0.0 0.2 0.4 0.6 0.8 1.0 1.2 PN[P0] ×10−2

Normal state power absorption

2 4 6 ω[vf/Λ] 0.0 0.2 0.4 0.6 0.8 1.0 1.2 1.4 PN[P0] ×10−2 Λ/vfτ = 0.01 Λ/vfτ = 0.03 Λ/vfτ = 0.05 2 4 6 ω[vf/Λ] 0.0 0.2 0.4 0.6 0.8 1.0 ×10−1 Λ/vfτ = 0.1 Λ/vfτ = 0.5 Λ/vfτ = 0.9

Power absorption with impurities