Recommendations on fine scale emissions derived from HERMESv3 M. - - PowerPoint PPT Presentation

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Recommendations on fine scale emissions derived from HERMESv3 M. - - PowerPoint PPT Presentation

Recommendations on fine scale emissions derived from HERMESv3 M. Guevara, Tena, C., Jorba, O., Prez Garca-Pando, C. FAIRMODE technical meeting 09/10/2019 October 07 - 09, 2019 Madrid, Spain Motivation Modelled emissions Gridded


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09/10/2019

Recommendations

  • n fine scale

emissions derived from HERMESv3

FAIRMODE technical meeting October 07 - 09, 2019 – Madrid, Spain

  • M. Guevara, Tena, C., Jorba, O., Pérez

García-Pando, C.

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SLIDE 2

Motivation

Gridded emission inventories Modelled emissions √ Gridded (fixed grid) X Not hourly (annual, monthly) X Not speciated √ Gridded (any grid or source level) √ Hourly √ Speciated

Emission processing systems Adapt the emission data to the air quality model’s requirement Emission models Implement detailed bottom-up emission estimation methodologies

(a) (b) (c) (d)

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HERMESv3

A python-based, parallel and multiscale emission modelling framework that processes and estimates gas and aerosol emissions for use in atmospheric chemistry models.

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HERMESv3

A python-based, parallel and multiscale emission modelling framework that processes and estimates gas and aerosol emissions for use in atmospheric chemistry models. global-regional module (HERMESv3_GR) bottom-up module (HERMESv3_BU)

A processing system that calculates emissions through an automatic combination of existing inventories and user defined vertical, temporal and speciation profiles An emission model that estimates emissions at the source level combining state-of-the-art bottom- up methods with local activity and emission factors

Guevara et al. (2019a, GMD) Guevara et al. (in preparation)

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HERMESv3_GR: global-regional module

  • Combination of multiple up-to-date gridded emission inventories
  • User defined destination working domain (multiple projections)
  • Application of country-specific scaling and masking factors
  • User defined vertical, temporal and speciation profiles per sector and pollutant
  • Outputs for multiple atmospheric chemistry models (CMAQ, WRF-Chem, MONARCH)
  • Available at the BSC git repository: https://earth.bsc.es/gitlab/es/hermesv3_gr

HERMESv3_GR output Emission data library

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HERMESv3_BU: Bottom-up module

Criteria pollutants: NOx, CO, SO2, NMVOC, NH3, PM10, PM2.5 Greenhouse gases: CO2, CH4

A_PublicPower B_Industry C_OtherStationary Comb F_Roadtransport K_AgriLivestock L_AgriOthers G_Shipping H_Aviation I_Offroad

user-dependent input data internal input data meteorology

Bottom-up and process-based estimation methodologies

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HERMESv3_GR: Temporal distribution

  • Specific monthly, weekly and diurnal profiles per sector and pollutant
  • Use of gridded profiles (variation not uniform across the space)

0.0 1.0 2.0 3.0 4.0 1 3 5 7 9 11 13 15 17 19 21 23

C_OtherStationaryCombution - Default C_OtherStationaryCombution - PM

0.0 0.5 1.0 1.5 2.0 2.5 3.0 3.5 4.0 4.5 5.0 5.5 1 20 39 58 77 96 115 134 153 172 191 210 229 248 267 286 305 324 343 362

Athens Barcelona Oslo

PM10 – EIONET Rural stations (December 2016)

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HERMESv3_BU: Road transport

𝐹𝑚,𝑗 ℎ = ෍

𝑤=1 𝑜

𝐵𝐵𝐸𝑈(ℎ)𝑤,𝑚 ∗ 𝐹𝐺(ℎ)𝑤,𝑚,𝑗

Estimation of link-level vehicle emissions

hot, cold-start, wear, evaporative, resuspension (speed and meteo dependent)

0.0 0.2 0.4 0.6 0.8 1.0

Euro 2 Euro 3 Euro 4 Euro 5 Euro 6 Diesel passenger cars @ 28km/h [g/km]

COPERT IV COPERT V COPERT V (with degradation factor) RSD

Amato et al. (2012)

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0.0 0.2 0.4 0.6 0.8 1.0

Euro 2 Euro 3 Euro 4 Euro 5 Euro 6 Petrol passenger cars @ 28km/h [g/km]

COPERT IV COPERT V COPERT V (with degradation factor) RSD

HERMESv3_BU: Road transport

𝐹𝑚,𝑗 ℎ = ෍

𝑤=1 𝑜

𝐵𝐵𝐸𝑈(ℎ)𝑤,𝑚 ∗ 𝐹𝐺(ℎ)𝑤,𝑚,𝑗

Estimation of link-level vehicle emissions

hot, cold-start, wear, evaporative, resuspension (speed and meteo dependent) Amato et al. (2012)

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HERMESv3_BU: Road transport

Low temperature NOx diesel emission penalty Grange et al. (2019)

𝐹𝑚,𝑗 ℎ = ෍

𝑤=1 𝑜

𝐵𝐵𝐸𝑈(ℎ)𝑤,𝑚 ∗ 𝐹𝐺(ℎ)𝑤,𝑚,𝑗

Estimation of link-level vehicle emissions

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HERMESv3_BU: Recreational boats

0.0E+00 5.0E+03 1.0E+04 1.5E+04 2.0E+04 2.5E+04 3.0E+04 3.5E+04

NOx SO2 CO NMVOC PM10 PM25 t/year

Total annual emissions

Port activities Small boats

  • Total Spanish boat park > 200.000
  • Large

contribution to CO and NMVOC emissions in coastal areas

  • Emissions mainly occurring during

summer season

  • How are these emissions currently

being treated in EMEP 0.1x01?

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HERMESv3_BU: LTO cycles

0% 20% 40% 60% 80% 100%

NOx CO PM10 PM2.5 NMVOC

apu taxi takeoff climbout approach landing

Main engines Brake and tyre wear Auxiliary Power Unit

  • Taxi out
  • Take off
  • Climb out
  • Approach
  • Landing
  • Taxi in
  • Landing
  • Pre-taxi out
  • Post-taxi in

Not included in the EMEP/EEA guidelines

Netcen (2004) Morris (2007)

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HERMESv3_BU: Fertilizers

Consideration of the spatial and temporal dynamical component of the emission processes.

𝐹 𝑦, 𝑒 = ෍

𝑑=1 𝑜

൯ ) 𝐵(𝑦 𝑑 ∗ ) Г(𝑦 𝑑 ∗ 𝐹𝐺(𝑦 𝑑 ∗ (𝑓0.022∗𝑈(𝑒)+0.042∗𝑋𝑇(𝑒)) ∗ ෍

𝑏=1 3

𝛾𝑏,𝑑 𝜏𝑑,𝑏 ∗ 2 ∗ 𝜌 ∗ 𝑓

(𝑒− 𝜐𝑑,𝑏)2 −2∗𝜏𝑑,𝑏

2

Local cultural techniques

  • N application rate
  • Type of fertilizers

Crop distribution

  • Crop hectares
  • Land uses

Soil properties

  • pH and Cation Exhange Capacity

NH3 volatilization

  • 2m temperature
  • Wind speed

Local cultural techniques

  • Crop calendars

Skjøth et al. (2011)

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HERMESv3_BU: Fertilizers

Consideration of the spatial and temporal dynamical component of the emission processes.

𝐹 𝑦, 𝑒 = ෍

𝑑=1 𝑜

൯ ) 𝐵(𝑦 𝑑 ∗ ) Г(𝑦 𝑑 ∗ 𝐹𝐺(𝑦 𝑑 ∗ (𝑓0.022∗𝑈(𝑒)+0.042∗𝑋𝑇(𝑒)) ∗ ෍

𝑏=1 3

𝛾𝑏,𝑑 𝜏𝑑,𝑏 ∗ 2 ∗ 𝜌 ∗ 𝑓

(𝑒− 𝜐𝑑,𝑏)2 −2∗𝜏𝑑,𝑏

2

20 40 60 80 100 120 1 18 35 52 69 86 103 120 137 154 171 188 205 222 239 256 273 290 307 324 341 358 t day-1

Lleida

20 40 60 80 100 120 1 18 35 52 69 86 103 120 137 154 171 188 205 222 239 256 273 290 307 324 341 358 t day-1

South of Castilla Leon Barley Maize Wheat Others HERMESv3 – NH3 L_AgriOthers (2015)

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HERMESv3_BU: Livestock

Use of the gridded Livestock of the World version 3 (GLWv3; Gilbert et al., 2018) GLWv3 versus location of farms HERMESv3 – NH3 G_Livestock (2015)

5 10 15 20 25 30 35 40 45 50 55 1 19 37 55 73 91 109 127 145 163 181 199 217 235 253 271 289 307 325 343 361 t day-1

Murcia Pigs Cattle Others

5 10 15 20 25 30 35 40 45 50 55 1 19 37 55 73 91 109 127 145 163 181 199 217 235 253 271 289 307 325 343 361 t day-1

Galicia Pigs Cattle Others

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HERMESv3_BU: Livestock

Van Damme et al. (2018, Nature) 0.0E+00 3.0E+04 6.0E+04 9.0E+04 1.2E+05

Aragon - Catalonia Murcia

Total NH3 [t/year] HERMESv3 IASI HERMESv3 – NH3 G_Livestock (2015) Use of the gridded Livestock of the World version 3 (GLWv3; Gilbert et al., 2018) IASI-derived total NH3

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Take home messages

  • Temporal variation of emissions:
  • It is important to consider differences across pollutants and regions
  • Road transport:
  • Measurements under real-world conditions are essential for the continuous

improvement/refinement of the emissions (e.g. temperatura effect)

  • Agriculture:
  • Consideration of the spatial and temporal dynamical component of the

emission processes is a key component.

  • Other mobile sources
  • LTO cycles: ensure that all the processes are considered (e.g. brake and tyre

wear)

  • Recreational boats: Large source of VOCs in summer and coastal areas. The

sector should be treated separately and not as part as the “OtherMobileSources”

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THANK YOU!

www.bsc.es marc.guevara@bsc.es