Environmental Environmental Acid rain Acid rain Chemistry - - PDF document

environmental environmental acid rain acid rain chemistry
SMART_READER_LITE
LIVE PREVIEW

Environmental Environmental Acid rain Acid rain Chemistry - - PDF document

Environmental Environmental Acid rain Acid rain Chemistry Chemistry APCH211 APCH211 Dr PG Ndungu Dr PG Ndungu Acid Rain Acid Rain Acidic Deposition Acidic Deposition Dry deposition Acid cid rai rain" "


slide-1
SLIDE 1

1

Environmental Environmental Chemistry Chemistry

APCH211 APCH211 Dr PG Ndungu Dr PG Ndungu

Acid rain Acid rain

Acid Rain Acid Rain

“Acid

cid rai rain" – " – General eral term appl rm applied ied t to an any f form o rm of wet prec precipitation, usua usually in in the the tr trop

  • posphere, w

with a acid idic ic spec species str stronger tha than CO CO2

Includes r

es rain, s sleet, s , snow

  • w,

, fog, o

  • r dew

Na

Natu tural ral pH pH of ra rain in water r ~ ~ 5.6 5.6 (f (from d m dissolved CO CO2)

Can ha

n have deposi deposition

  • n of
  • f dr

dry y gases and gases and com compou

  • unds –

– so

  • calle

called dr dry y dep deposition

Aqueo

eous us and and dr dry dep deposi sition ar are e col collectively t termed aci med acid dep deposi sition

The

e precur ursors rs or chemical f al forerunne rerunners o rs of ac acid r rain f formation rmation res result fr from

  • m both

th na natur tural sour sources, such such a as volc lcanoes a and deca caying vege getation a and ma man- n-made sour sources, prim primarily emi emissions of sulf

  • f sulfur

di dioxide (S e (SO2) an and d nitrog

  • gen

en ox

  • xid

ides (N es (NOx) r ) resulti sulting f ng from fossil ssil fuel comb mbust ustio ion. n.

Acid

id ra rain is in is pa partic icularly d dama magi ging t to la lakes, str streams, a and fore rests an and t d the pl e plan ants ts an and d an animals t that l at live i in these ese e ecosys

  • systems

ms. .

Acidic Deposition Acidic Deposition

Wet deposition

refers to acidic rain, fog and snow. If the acidic chemicals in the air are

blown into areas where the weather is wet, the acids can fall to the ground in the form of rain, snow, fog, or mist. Dry deposition

In areas where the weather is dry, the

acid chemicals may become incorporated into dust or smoke and fall to the ground through dry deposition sticking to the ground, buildings, homes, cars, and trees. Later, when moisture content i id l ti i d d g increases, acid solution is produced.

Main Culprits in Acidic Precipitation Main Culprits in Acidic Precipitation

Nit Nitrogen spec species:

NOx

NOx

Sou

Sources incl include b burn rning of

  • f

fo fossil f fuels, s, b biomas ass, s, e etc

Natural S

tural Sour urce ces; s; A Anorexic ic t i t il t Sul Sulfur Spec Species

SO

SO2

Foss

ssil f il fuels & els & sulfur o fur ore s e smeltin elting

H2S,

S, & & CS CS2:

Wetlands a

and sub submerged soi soils wa waters, ers, so soil ils, s, etc

NH

NH3

Animal exc

excret eta, a, fertiliz izer ers a and micr crobio

  • biolo

logical r gical release ase

Wetlands a

and sub submerged soi soils

Dim

Dimethylsulfide, ( (CH3)2S, c S, carbon

  • nyl

yl sul sulfi fide, COS, COS, me methyl mer mercaptan, CH CH3SH a and Dime Dimethyl disu isulfide, CH CH3SS SSCH CH3. .

Ocean an

Ocean and d soils. ils.

Atmosph mospheric c Pr Production

  • duction Of Nitric A

Of Nitric Acid id Atmosph mospheric c Pr Production

  • duction Of Nitric A

Of Nitric Acid id

The principle reaction sequence contributing to production of nitric acid starts with nitric

  • xide,

NO from combustion processes. Nitric tric oxide ide Chemis hemistry: Dayti time me

NO is oxidized by O2, O3 or ROO – e.g.

NO + O3 NO2 + O2

3 This NO2 radical can then contribute to

  • zone and OH radical production i.e.

plays a role in smog formation

  • Short lifetime, thus smog events don’t last,

& not that frequent

  • Main removal sequence for NO is via

catalyst (M), OH rxns

NO2 + OH + M HNO3 + M

slide-2
SLIDE 2

2

Nitric Nitric acid acid Product Production at

  • n at Night

Night Nitric Nitric acid acid Product Production at

  • n at Night

Night

  • Key species is the nitrate radical

(NO3).

  • Formed via O3 & NO2
  • Atmospheric

production

  • f

dinitrogen pentoxide (N2O5) occurs when NO3 reacts with NO2 is the

  • nly way to form in the atmosphere
  • nly way to form in the atmosphere.
  • N2O5 is a store of NO3.
  • Can decompose back to NO3

and NO2

  • Can react with water to form

nitric acid

Easily zapped by the rising sun! (λ ~ 600 -700nm)

Reactions of actions of NO NO Reactions of actions of NO NO3 with h with hydroca drocarbo bons ns with h with hydroca drocarbo bons ns

  • Easily removes an H from alkanes

NO3 + RH R + HNO3

  • The R radical can then react with O2 to form peroxyl radicals
  • With alkenes the NO3 radical reacts via an addition mechanism producing nitro-oxy

substituted organic radicals which can regenerate NO2, or relatively stable organic nitrate compounds (see - Paul S. Monks. Gas-phase radical chemistry in the troposphere. Ch Chem. Soc.

  • Soc. Rev., 2005, 34, 376-395, for e.g. with propene)

NO3 + CnH2n CnH2nNO3

  • With aldehydes, typically form nitric acid and the corresponding radical

NO3 + RCHO RCO + HNO3

  • Overall nighttime chemistry of NO3 can recycle NOx, or form HNO3, depending on the mix
  • f hydrocarbons
  • Can be a nighttime source of OH radicals

Remo moval of l of Nitric Nitric Acid Acid Remo moval of l of Nitric Nitric Acid Acid

Removal is accomplished by either wet or dry

deposition

One of the main contributors to acid precipitation. Nitric acid can react with ammonia:

NH3 + HNO3 NH4NO3

The ammonium nitrate, NH4NO3 can act as a

condensation nucleus for the formation of a water droplet or it can be deposited as part of the solid aerosol

Atmos mospheric Pr Produ

  • ducti

tion of

  • f Sulfuri

Sulfuric A Acid id Atmos mospheric Pr Produ

  • ducti

tion of

  • f Sulfuri

Sulfuric A Acid id

Ox Oxida idation of reduc educed ed sulf sulfur ur spec specie ies

  • Production of sulfuric acid is

more complex than that of nitric acid as the starting materials cover a wide range of reduced sulfur and partially

  • xidized

sulfur compounds.

  • These include hydrogen sulfide,

carbon disulfide, carbonyl sulfide, methyl mercaptan, di th l di lfid d di th l dimethyl disulfide, and dimethyl sulfide. All these compounds contain sulfur in its oxidation state (-2).

  • Mostly from natural sources

S S S C C O S H H

Se Sequence o ence of Reaction tions o s of Sul Sulfur ur Se Sequence o ence of Reaction tions o s of Sul Sulfur ur Cmpds Cmpds Cmpds Cmpds

  • Once sulfur compounds are

in the air, a sequence of reaction begin as follows:

H2S + OH H2O + SH CS2 + OH COS + SH COS + OH CO2 + SH

Further

  • xidation
  • f

thionyl radical eventually produces sulfur dioxide:

SH + O2 SO + OH SH + O3 SHO + O2 SHO + O2 SO + HOO

The SO radical can then react

NB NB:

  • The

above reactions release thionyl radical, SH as the initial product.

  • Importance of OH!
  • Hydrogen

sulfide and carbon disulfide unlike carbonyl sulfide, are very reactive and therefore are quickly consumed

with either O2, O3 or NO2 to give SO2 and other products.

2SO + O2 2SO2 SO + O3 SO2 + O2 SO + NO2 SO2 + NO NB NB. SO2 is ultimately converted to sulfuric acid, H2SO4.

Where is the OH coming from?

More About More About SO SOx…

  • Dimethyl

sulfide is produced by phytoplankton living in surface waters of the

  • cean. It is oxidized by hydroxyl radical (OH)

with a final product being sulfuric acid.

  • Sulfur dioxide SO2 is also released in large

quantities directly into the atmosphere from sulfide ore smelting and fossil-fuel combustion.

slide-3
SLIDE 3

3

Peer to Peer Assignment: Mount Peer to Peer Assignment: Mount Pinatubo Pinatubo

Re Reducing Re Reducing Acid Rain Acid Rain Acid Rain Acid Rain

There are several ways to reduce acid rain (i.e. acid deposition). These range from government policy to societal changes and individual action. e.g. given by epa (http://www.epa.gov/acidrain/reducing/):

Understand acid deposition’s causes and

  • Understand acid deposition s causes and

effects

  • Clean up smokestacks and exhaust pipes
  • Use alternative energy sources
  • Restore a damaged environment
  • Look to the future
  • Take action as individuals

The steps involved in reduction of acid deposition are:

Recycle, Reuse, Reduce or the 3 R’s of waste management has evolved from the initial concepts championed in the 1970’s & now includes, amongst other things, prevention & minimization

Reducing Ac ducing Acid ra id rain in Reducing Ac ducing Acid ra id rain in

Unde derstand a rstand acid de depo positio tion’s c causes a and d effects

  • understand acid deposition’s causes and effects, and to track changes in the environment.
  • Scientist collect air, water & soil samples and measure them for various characteristics such as pH

and chemical composition, and investigate the effects of acid deposition on human-made materials.

  • Scientists understand the effects of sulfur dioxide (SO2) and nitrogen oxides (NOx), and any other

acid causing species

  • People to understand the process of how acid rain damages the environment (Need to educate Policy

Makers!).

  • People to find out what changes could be made to the air pollution sources that cause the problem
  • People to find out what changes could be made to the air pollution sources that cause the problem

(Need to educate Policy Makers!).

Steps t eps to solv solve e acid acid depositi deposition Steps t eps to solv solve e acid acid depositi deposition problem problem problem problem

a) a)

Cl Clean n up sm smokestac estacks a and e exhaus ust t pipes pipes WH WHY? Almost all of the electricity that powers modern life comes from burning fossil fuels such as coal (Over 80% in RSA) fuels such as coal (Over 80% in RSA), natural gas, and oil. Sulfur dioxide (SO2) and nitrogen oxides (NOx) are the main acid chemicals.

  • Options for reducing SO2 emissions,

include: using coal containing less sulfur, washing the coal, and using devices called “scrubbers” to chemically remove the SO2 from the gases leaving the smokestack.

  • Power plants to change type of fuels

e.g, burning natural gas creates much less SO2 than burning coal.

St Steps eps to solv solve acid depos e acid depositi tion

  • n…

St Steps eps to solv solve acid depos e acid depositi tion

  • n…

b) b)

Us Use alterna ernativ tive energy ergy sources ces

  • Other sources of electricity besides

fossil fuels. They include nuclear power, hydropower, wind energy, tidal, geothermal energy, and solar energy.

  • Alternatives to internal combustion

engines

  • batteries, solar cells, and fuel

cells NB NB: All sources

  • f

energy have environmental costs as well as benefits.

Steps t eps to sol solve e aci acid deposi deposition… Steps t eps to sol solve e aci acid deposi deposition…

c) c)

Restor

  • re a damaged env

nviron

  • nme

ment NB! It takes many years for ecosystems to recover from acid deposition, even after emissions are reduced and the rain pH is restored to normal. There are some things that people can do to bring back lakes and streams i kl more quickly.

  • Limestone or lime (a naturally occurring basic compound) can be added

to acidic lakes to “cancel out” the acidity. Li Liming, has been used extensively in Norway and Sweden.

slide-4
SLIDE 4

4

St Steps t eps to solve solve acid acid deposition… deposition… St Steps t eps to solve solve acid acid deposition… deposition…

d) d)

Evaluation of the

  • f the pr

progr

  • gress ma

made on a

  • n acid

id ra rain in red reduction pr proc

  • cess
  • Monitoring Very Important!

If the depositions are reduced environmental

  • If the depositions are reduced, environmental

protection agency (EPA) scientists must assess the reductions to make sure they are achieving the anticipated results.

  • If no changes, to consider additional ways to reduce

emissions that cause acid deposition. Example: focus on energy efficiency and alternative energy.

St Steps eps to solv solve acid depos e acid depositi tion

  • n…

St Steps eps to solv solve acid depos e acid depositi tion

  • n…

e) e)

Take ac actio tion as as indivi individuals Yes! You too can make a difference!

  • Turn off lights, computers, and other appliances when you're not using them

(Unplug chargers when not in use!).

  • Use energy-efficient appliances for lighting, air conditioners, heaters, refrigerators,

washing machines, etc.

  • Use public transportation or better yet walk or bicycle whenever possible
  • Use public transportation, or better yet, walk or bicycle whenever possible
  • Buy vehicles with low NOx emissions, and properly maintain your vehicle (In the

News, Mercedes, VW, etc, complaining RSA fuel quality has too much sulfur for latest technologies).

  • 6. Be well informed.

WHAT ABOUT TALKING TO GOVERNMENT What Policies, Programs, or commitment in general has RSA made (PEER TO PEER ASSIGNMENT)?

THE CHEMISTRY OF THE CHEMISTRY OF URBAN AND URBAN AND INDOOR INDOOR ATMOSPHERES ATMOSPHERES

The Chemistry of Urban & Indoor Atmospheres The Chemistry of Urban & Indoor Atmospheres

The chemical composition of air in places where people

live & work (urban areas, homes, offices, etc) vary with modernization or industrialization of the locality.

Urban areas are likely to be affected by atmospheric

pollution due to the following major factors:

Combustion of fossil fuels (mostly cars) In-space heating and cooling Power generation and industrialization Incineration of waste materials

Urban & Indoor Atmospheres… Urban & Indoor Atmospheres…

  • Use of petroleum products especially

in motor vehicles result in ground- level emissions of carbon monoxides, volatile hydrocarbons, nitrogen oxides and sometimes, lead compounds. These emissions are accompanied by aldehydes and other secondary pollutants.

  • The combustion of biomass and coal

produces substantial concentrations p

  • f solid particulate matter along with

nitrogen oxides, polyaromatic hydrocarbon (PAHs) compounds as well as sulphur dioxide.

  • Open burning refuse or garbage

cause air pollution is a source of volatile organic carbon compounds and solid particulate matter (SPM).

  • Hurricanes and wind are the source
  • f particulate matter such as dust

especially in dry areas.

Pollutants In The Urban Atmosphere Pollutants In The Urban Atmosphere

World Health Organization (WHO) Standards for Air Quality

The WHO guidelines for air quality take into account time period over

which measurements is done. This is known as human exposure.

Potential toxicity depend on both atmospheric concentration and

duration of contact with the atmosphere. That is; Exposure = Concentration x time

slide-5
SLIDE 5

5

Quality guidelines Quality guidelines

The quality guidelines must specify the acceptable

concentration to be exposed to humans over a specified period.

Example: carbon monoxide at 20mg.m-3 (20ppbv) may

be acceptable if exposure time is 1 hour but not t bl f l i d ti acceptable for longer period times.

For longer exposure such as 8hrs, the allowed

concentration of carbon dioxide should not exceed 10mg.m-3, that is, 0.01ppmv or 10ppbv.

WHO works closely with United Nations Environmental

Program (UNEP) to carry out air quality monitoring.

Table 1 is a summary of WHO guideline values for air quality-values in µg.m-3 or parts per trillion in volume (pptv). SPM=Suspended particulate matter TSP=Total suspended particulate

Pollutant Max. time weighted (µg/. m-3) Average time SO2 CO NO2 500 30,000 400 10 min 1 hr 1 hr

particulate RSP = Respirable suspended particulate, PM10 with particle size

< 10µm

O3 SPM (black smoke) TSP RSP; PM10 Pb 150-200 100-150 150-230 70 0.5-1 1 hr 24hr 24hr 24hr 1yr Updated values (2005) can be found at: http://www.who.int/mediacentre/factsheets/fs313/en/index.html You Need it!

Suspended Particles Matter (SPM) Suspended Particles Matter (SPM)

  • Concentration of atmospheric particulates is

severe in some megacities (cities > 10million population) and average levels may range from 200 to 600 µg.m-3 or pptv.

  • Human health associated with high values depend on the nature of

particulates particulates. Examples: those derived from coal and those in the PM10 or PM2.5 categories, have been shown to be hazardous. NB: PM10 is particulate matter size < 10µm ; PM2.5 < 2.5µm.

Air quality Air quality param parameters Air quality Air quality param parameters

Carbon Monoxide (CO): depend on high traffic density – vary from city

to city.

Sulphur dioxide (SO2): Usually produced by coal. Sulfur dioxide conc. Is

low in cities that use low coal fuels

Nitrogen dioxide (NO2): Higher levels expected indoors with poor

ventilation where kerosene or natural gas used for heating and cooking.

Ozone (O3): from reaction of gases in the troposphere; trace amounts may

result from mass transfer from stratosphere.

Lead (Pb): Airborne lead depends on the population of cars, the

concentration of lead additives in the fuel and availability of unleaded fuel. Concentrations in leaded gasoline vary between 0.1 and 2.0 g.L-1.

  • NB. Use of tetraethyl lead to augment the octane number (?) is becoming less.

More info from: http://www.bbc.co.uk/dna/h2g2/A16407173 You Need it!

INDOOR AIR QUALITY INDOOR AIR QUALITY

  • Many people spend most of their

time indoors (home, office, etc.). The atmospheres encountered indoor vary a great deal.

  • The materials of house construction

may vary from clay-rich soils or

  • ther fresh or baked earth materials.
  • In some cases the homes are open
  • In some cases, the homes are open

and air exchange is rapid while in

  • thers heating may be done over an
  • pen fire in a room without a

chimney and also a variety of fuels may be used.

  • The building materials may range

from bricks, stones, wood, various plastics and metals.

  • Activities in the homes include:

cleaning, cooking, heating over

  • pen or closed fires with varying

smoke conditions.

Major fac jor factor

  • rs that

s that de determine rmine the the quality quality of

  • f indoor

indoor air air Major fac jor factor

  • rs that

s that de determine rmine the the quality quality of

  • f indoor

indoor air air

  • The nature of the ambient air, outdoor around the building plays a
  • role. In this case, the outdoor atmosphere is influenced by air
  • utside.
  • Design and site of the building is important. This will dictate the

quality of exchange of indoor atmosphere.

  • Nature of materials present in the building such as polymers. The

latter could be a source of formaldehydes or other partially

  • xidized organic compounds.
  • Building materials from clays concrete etc may contain traces of
  • Building materials from clays, concrete, etc., may contain traces of

radioactive elements such as uranium.

  • Activities that take place inside the house. These may include

combustion of wood for heating, cooking gas, electric cookers, etc. Cleaning of the house may involve mechanical devices such as vacuum cleaner, that create dust.

  • Use of cleaning solvents and detergents, insecticide sprays, toilet

sprays and air fresheners.

Another reference you will need: Indoor Air Quality Guidelines: selected pollutants(PDF) http://www.who.int/indoorair/publications/en/index.html

slide-6
SLIDE 6

6

COMMON INDOOR AIR CONTAMINANTS COMMON INDOOR AIR CONTAMINANTS

Air contaminants refer to levels above the outdoor background level.

  • 1. Radioactive compounds:
  • Radioactivity is usually associated with Radon noble gas, Rn released by

Uranium isotope 238 and also by Thorium isotope 232 with half-lifes of 4.5 and 14 billion years, respectively. These elements are found in geological materials such as rocks and fossils

Radioactiv Radioactivity ity Radioactiv Radioactivity ity

The spontaneous emission of particles and/or

energy from atomic nuclei.

The spontaneous emission of radiation from the

nucleus of an atom. Radion Radionuclides lose particles and energy through this process of radioactive decay.

Ra Radioacti dioactive e e elements ents Ra Radioacti dioactive e e elements ents

Radioa

Radioactiv ctive e e elem ement ents, such as ura uraniu ium ( (239

239U)

U) thor

  • rium (

m (234

234Th

Th) and pota tassium ssium ( (40

40K)

K) break down (decay) fairly readily to form lighter atoms e.g Be, B.

  • The energy that is released in the process is made up of small, fast-moving

particles and high-energy waves.

  • These particles and waves are, of course, invisible. (The level of radioactivity of an

element varies according to how stable its atoms are).

  • Other elements with naturally occurring radioactive forms, (isotopes) are carbon

(C13

13), bismuth (210 210Bi

Bi), radon (223

223R) and strontium (88 88Sr

Sr).

Conti… Radioactivity process Conti… Radioactivity process

Radioactivity is a random process that happens

naturally as the isotopes in particular elements decay. The isotopes continue to break down over time.

The length of time that is taken for half of the nuclei in

an element to decay is called its 'half-life'.

A half

half-lif life can be very short (milliseconds to hours) or A half half lif life can be very short (milliseconds to hours) or very long (hundreds of thousands of years).

Radiation also arises from nuclea

nuclear f r fissio ssion.

Fiss

Fission can be spontaneous but is usually initiated in a nuclear reactor. Fission is a radioactive process; it releases energy as the heavy nucleus is split into two.

Ex Exam ample: Calcul Calculation of

  • f Half

Half Ex Exam ample: Calcul Calculation of

  • f Half

Half-

  • Lif

Life of

  • f

Lif Life of

  • f

Ra Radioacti dioactive El e Elelemnts emnts Ra Radioacti dioactive El e Elelemnts emnts

Consider strontium -9 0 which has a half-life of

approximately 28 years.

  • Initially, at time t= 0, the sample is 100% strontium-90
  • After 28 years, only half the original amount of

strontium will remain: ½ x 100% = 50%

  • After another 28 years, only half of this amount of

strontium-90 will remain: ½ x 50% = 25% strontium-90 will remain: ½ x 50% = 25%

  • After another 28 years, only half of this amount of

strontium will remain: ½ x 25% = 12.5%

  • and so on.
  • At any given time, the amount of strontium-90 that has

undergone decay can be calculated: amount of strontium-90 decayed = the original amount - the amount remaining.

Calculat ions Calculat ions

The amount of radioactive isotope remaining

can be calculated: Nt = No x (0 .5 ) num ber of half- lives Nt = amount of radioisotope remaining No = original amount of radioisotope number of half-lives = time ÷ half-life

Exam ple

p Calculate the percentage of strontium-90 remaining after 280 years. Nt = No x (0 .5 ) num ber of half- lives Nt = ? % No = 100% number of half-lives = time ÷ half-life = 280 ÷ 28 = 10 Nt = 100 x (0.5) 10 = 0.098%

slide-7
SLIDE 7

7

Num ber

  • f Half-

lives Tim e ( years) % Strontium - 9 0 rem aining % Strontium - 9 0 that has decayed 100

Strontiu ntium-9 m-90 h half-lif ifes es

1 28 50 50 2 56 25 75 3 84 12.5 87.5 4 112 6.25 93.75 5 140 3.125 96.875 6 168 1.5625 98.4375

Stront ntium-90 ium-90 half-

half-lifes

  • 2. Volatile Organic Compounds
  • 2. Volatile Organic Compounds (VOCs)

(VOCs)

Sources are:

  • Paints: toluene, ethylbenzene, 2-isopropanol and butanone.
  • Cleaning agents: households solvents, detergents.
  • Wood-building materials such as plywood produce formaldehyde.
  • 3. Polybrominated diphenyl ether
  • 3. Polybrominated diphenyl ether

Polybrominated diphenyl ether (PBDE) is toxic. General structure is shown below. PBDE is used in commercial household products such as plastics casings for appliances, in fabrics used for clothing, carpets, etc.

Chem Chemica ical struct structur ure of e of PBDEs DEs Conti…air contaminants Conti…air contaminants

  • 4. Emissions from indoor combustion.

This is combustion of fuel that contains VOCs;

burning of coal, wood and biomass.

Tobacco smoking is a source of many VOCs

i l di ld h d k t i b h including aldehydes, ketones, organic bases such as nicotine, organic acids.

  • 5. Indoor particulates
  • 5. Indoor particulates

These include: solid aerosols from dust; combustion of coal & biomass material.

  • Particle size is usually in the range PM10

(<10µm). Particle size <2µm, can easily enter respiratory track. p y

  • Smoking contributes to respirable particulate

matter inside a building.

  • Polyaromatic

hydrocarbons (PAHs) are emitted from coal & biomass.

slide-8
SLIDE 8

8

Particles in the atmosphere Particles in the atmosphere

  • Particulate is a term that has come to stand for particles in the

atmosphere.

  • Particulate matter makes up the most visible and obvious form of

air pollution.

  • Particles in the atmosphere range from 0.5 mm (size of sand)

down to molecular size level (nanometer).

  • Particles may consist of either solids or liquid droplets.
  • Atmospheric aerosols are solid or liquid particles smaller than 100

µm in diameter.

  • Pollutant particles in the 1 nm to 10 µm range are commonly

suspended in the air near sources of pollution such as the urban atmosphere, industrial plants, highways and power plants. DESCRIPTION OF ATMOSPHERIC PARTICLES Terms Meaning 1. Aerosol Colloidal-sized atmospheric particle 2. Condensation aerosol Formed by condensation of vapors or reactions of gases. 3. Dispersion l Formed by grinding of solids, t i ti f li id aerosol atomization

  • f

liquids

  • r

dispersion of dusts. 4. Fog Denotes high level of water droplets 5. Haze Denotes decreased visibility due to presence of particles 6. Mists Liquid particles 7. Smoke Particles formed by incomplete combustion of fuel

Nature of particles Nature of particles

  • Very small solid particles include (1 nm-10 µm ): carbon

black, silver iodide, combustion nuclei, sea-salt nuclei- tend to be acidic.

  • Larger particles include (100 µm -500 µm ) : cement dust,

wind blown soil dust, foundry dust and pulverized coal- tend to be basic. Li id i l i i l d i d f d lf i id

  • Liquid particles-mist, include raindrops, fog and sulfuric acid

mixture

  • Particles of biological origin: viruses, bacteria, bacterial

spores, fungal spores and pollen.

  • Important atmospheric contaminants- mainly inorganic and
  • rganic particles.

Effects of atmospheric particles Effects of atmospheric particles

  • Effects on climate
  • Damage buildings
  • Impact on human health (people with asthma)
  • Reduced visibility & causes undesirable aesthetic effects

NB: Aerosols, natural and anthropogenic, can affect the climate by changing the a radiation is transmitted thro gh the atmosphere the way radiation is transmitted through the atmosphere.

Effects of atmospheric particles… Effects of atmospheric particles…

All aerosols both absorb and scatter solar and terrestrial radiation. If a substance absorbs a significant amount of radiation, as well as

scattering, it is called absorbing.

This is quantified as the ratio of scattering alone to scattering plus

absorption (extinction) of radiation by a particle.

Physical behaviour of particles Physical behaviour of particles

  • Small colloidal particles undergo diffusion processes and coagulate

together to form larger particles.

  • Mechanism for removal of particles from the atmosphere is mainly through

sedimentation & scavenging by rain drops and then precipitation.

  • Particle size refers to diameter of the particle but in some cases radius may

b d be used.

slide-9
SLIDE 9

9

Process for particle formation Process for particle formation

  • Physical Process: particle formation is mainly through disintegration of

larger particles > 1 µm

  • Many dispersion aerosols originate from natural sources: sea-spray,

windblown dust, volcanic dust.

  • Chemical process: Inorganic particles are mainly metal oxides formed by
  • xidation of the metal by oxygen.
  • Organic particles are produced mainly through internal combustion

engines. N.B. Recall: PHOTOCHEMICAL SMOG

Composition of Inorganic Particles Composition of Inorganic Particles

  • Aluminium oxide, iron oxide, calcium oxide and silicon dioxide are due to soil

erosion, rock dust, coal combustion.

  • Carbon particles- due to incomplete combustion
  • Sodium and chlorine compounds- due to marine aerosols
  • Antimony and selenium- due to combustion of oil, coal or refuse.
  • Lead from combustion of leaded fuels & wastes

Composition of Organic Particles Composition of Organic Particles A wide variety of organic compounds most of which are toxic: polycyclic aromatic hydrocarbons (PAHs) such as benzo(a)pyrene, chrysene, benzo-fluoranthene, acridine. Radioactive particles

  • Main source of radionuclides in atmosphere is randon: it is
  • Main source of radionuclides in atmosphere is randon: it is

a noble gas produced from radium decay.

  • Cosmic rays in the atmosphere produce radionuclides

which are isotopes of: 7Be , 10Be, 14C, 39Cl, 3H, 22Na, 32P and 33P

Control of Particulate Emissions Control of Particulate Emissions

  • Removal of particulate matter from gas streams is the most practiced means
  • f air pollution control.
  • Techniques for removal depends on particle size, loading, nature of

particles and type of scrubbing system.

Methods of particle removal Methods of particle removal

These include:

  • Sedimentation and inertia, i.e gravitational settling as a continuous process.
  • Particle filtration using fabric filters that allow gas molecules to pass

through but retain the particulate matter.

  • Scrubbers- this involves use of scrubbing liquid which forms small droplets

for scavenging particles from the gas stream. g g p g

Air P r Pollut llution

  • n Cont

Control rol for Par r Partic iculat ulate e Emissions issions Air P r Pollut llution

  • n Cont

Control rol for Par r Partic iculat ulate e Emissions issions

It is possible to minimize emissions of aerosol particles

from point of source such as thermal electrical generating stations or industrial smelting units.

Containment of particulate matter is achieved using

devises that remove the aerosols from fast moving devises that remove the aerosols from fast moving stack gas stream. Common collection methods include: settling chambers, cyclones, fabric filter, scrubbers, and electrostatic precipitators as shown in the slides that follow.

slide-10
SLIDE 10

10

Settling Chambers Settling Chambers

Are the simplest and commonly used. Ad

Advantages ages

Sim

Simple le t to build build, lo low w cost, lo cost, low w main maintenance, lo low w pressur pressure dr drop,

  • p,

simple to to dispose of collected m mate teri rial als

Di

Disad sadvantages

Limit

mited d to to removal o l of partic icles les l larger t than40-60 40-60 μm d m diameter

Construction includes variety of baffles and open space designed

to allow the particles sufficient time to settle under the force of gravity.

Settling rates are limited by gravity therefore method effective for

large particle size >10µm.

They come in different design. The mechanism include adsorption

and absorption.

Types of Settling Chambers Types of Settling Chambers

Simple expansion chamber Multiple-tray settling chamber.

Supp Slide 1

Momentum Separators Momentum Separators

Thes

ese e di differ s er slightly from yo your t ur typica cal s l settling ttling cham ambers vi via a the additio addition o

  • f simp

mple le ch chamb amber f r feature atures t that at al allow f for di r directi rectiona nal l ch change anges i s in ai air r flow that add at add a a down downward inerti tial f al force e to supple plement ent t the g e gravit itatio ional nal force. e.

Supp Slide 2

Combustion Combustion Fabric Filters: Filtration Fabric Filters: Filtration

Fabric filter or bags operate in a similar principle as

vacuum cleaner.

The air stream is made to pass thro a porous fabric

material and is effective for particulates size in the range 0.01 - 10µm range.

Bags or fabric filters are sensitive to temperature and

  • humidity. The fine particles clog the filters and there4

must be periodically cleaned. Advantag ntages es Disadv dvant antages

  • High Collection Efficiency (>99%)
  • Effective for a Wide Range of Dust Types
  • Modules Can be Factory Assembled
  • Operates Over Wide Range of Gas Flow

Rates

  • Reasonably Low Pressure Drop
  • Good Efficiency for Small Particles
  • Dry Collection and Disposal
  • Large Footprint
  • Temperature Limitations
  • Requires Dry Environment
  • Fire or Explosion Potential
  • High Maintenance Cost

Filtration Filtration

slide-11
SLIDE 11

11

Electrostatic Precipitator Electrostatic Precipitator

Electrostatic precipitator causes the particles in a gas stream to become

charged by electrons produced thro an electrical discharge between two electrodes.

The negatively charged particles then migrate to the positive electrode and

are collected and removed from the emission stream. Positively charged particles move to negative electrode.

Advantag ntages es Disadv dvant antages

  • High Collection Efficiency
  • Dry Collection and Disposal
  • Small Pressure Drop
  • Capable of Handling Large Gas Flow

Rates

  • Low Electrical Power Requirements
  • Low Maintenance
  • Disadvantages
  • High Capital Cost
  • Particle Resistivity Limitations
  • May Require Injection of SO3 or

NH3 to Control Resistivity

  • Relatively Large Footprint
  • Special Precautions for Safe

Operating at High Voltage

Electrostatic Precipitator Electrostatic Precipitator Scrubbers Scrubbers

Scrubbers allow gas stream to be in contact with a

fine mist or spray of water.

The water droplets capture many small particles and

these settle more rapidly into a collector container.

Scrubbers come in different designs as shown below.

Advantag ntages es Disadv dvant antages

  • High Collection Efficiency
  • Capable of Handling Flammable and

Explosive Dusts

  • Can Handle Mists
  • Low Maintenance
  • Simple Design and Easy to Install
  • Provides Cooling for Hot Gases
  • Neutralizes Corrosive Gases and Dusts
  • Waste Water Must be Treated
  • Collected Particulates are in

Sludge Form

  • High Corrosion Potential
  • High Pressure Drop
  • May Require Protection Against

Freezing

  • Final Exhaust Must be

Reheated

  • Sludge Disposal May be

Expensive

Absorption Method Absorption Method Adsorption Adsorption Liquid Scrubber Liquid Scrubber

slide-12
SLIDE 12

12

Cy Cyclon clones es Cy Cyclon clones es

Cyclones are cone-shaped devices that cause the waste

gas stream to swirl rapidly in spiral fashion causing larger particles to move towards the wall of the cone by centrifugal force.

Once in contact with the wall, the particles slide down

the inner surface of the cone to a collection container the inner surface of the cone to a collection container below it.

Stoke’s law determines the extent of removal of

particles but the settling rates can be greatly enhanced by the increased force due to cyclone action. In this case removal of particles <10µm can be achieved.

Stokes Law Stokes Law

Where vt = terminal velocity of particles in m.s-1; d it f ti l i

3

η ρ ρ ν 18 d g C )

  • (

2 p p a t = pp = density of particle in g.cm-3 Pa = density of air = 1.2 x 103 g.m-3 at Po and 25° C; C = Stokes correction factor for assuming spherical shape and discontinous of fluid interactions when the particle size is small compared with the molecular mean path in air. g = acceleration due to gravity = 9.8 m.s-2 dp = particle diameter in meters and = viscosity of air = 1.9 x 10-2 g.m-1.s-1 at P° and 25° C

Cyclone Cyclone Combustion Combustion

Minimize Emission from point Minimize Emission from point Source: example SO Source: example SO2

Minimize emissions of aerosol particles from point

  • f source such as thermal electrical generating

stations or industrial smelting units.

EXAMPLE: EXAMPLE: Sulfur Dioxide Control Sulfur Dioxide Control

http://www.apt.lanl.gov/projects/cctc/factsheets/puair/adflugasdemo.html

slide-13
SLIDE 13

13

Clean Coal Technologies Clean Coal Technologies

Advanced Flue Gas Desulfurization

Demonstration Project - e.g. of a series of initiatives

Others Include

Carbon Capture and storage Underground coal gasification

Why Clean Coal? Why Clean Coal?

Coal Usage

In RSA Coal used to

generate over 85% of th l t i it

Impact of Coal

Mining

Water scarcity

the electricity

Globally Coal accounts

for more than 40% of Electricity produced

Only realistic

technology for next 20 – 50 years

Water scarcity Water Pollution

Burning

SOx, NOx,

particulates, CO2, fly ash

CO CO2 Sequestration Sequestration

  • Cle

Clean a and trea treat the the CO CO2 the then st stor

  • re it

it

  • Curr

Currently used used in in enh enhanced oil reco

  • il recovery
  • Opt

Options t to use use sa salin line (v (ver ery sa salt lty) a aquif uifers

  • Aban

andone ned c coal al mines, ot

  • the

her g r geolog

  • logic c

ic caverns et rns etc

Underground Coal Gasification (UCG) Underground Coal Gasification (UCG)

Hist Histori rically a lo lot of t of the w the work rk was d s done ne in in the f the former rmer US USSR Resurge rgence in in int interest rest (Ch (China, na, A Austral ralia, a, Europe, pe, America Americas & & RSA

SA SASOL Maj Majuba

http://www.eskom.co.za/live/content.php?Item_ID=14077