Synthesis of linalool and limonene sensitizing hydroperoxides ! E - - PowerPoint PPT Presentation

synthesis of linalool and limonene
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Synthesis of linalool and limonene sensitizing hydroperoxides ! E - - PowerPoint PPT Presentation

Synthesis of linalool and limonene sensitizing hydroperoxides ! E Gimnez-Arnau Laboratoire de Dermatochimie Institut de Chimie de Strasbourg Universit de Strasbourg (CNRS-UMR 7177) Strasbourg, France Methods to prepare hydroperoxides


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Synthesis of linalool and limonene sensitizing hydroperoxides !

E Giménez-Arnau

Laboratoire de Dermatochimie Institut de Chimie de Strasbourg Université de Strasbourg (CNRS-UMR 7177) Strasbourg, France

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Methods to prepare hydroperoxides

Autoxidation of unsaturated compounds!

Initiation! Propagation! Termination! fast! slow! non-radical products!

General mechanism! For unsaturated compounds!

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Non-selective, multitude of oxidation products … !

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Methods to prepare hydroperoxides

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Methods to prepare hydroperoxides

Singlet oxygen ene reaction – Schenck reaction!

production of singlet oxygen! f i Photochemical methods : mostly employed!

Bengal Rose! Methylene Blue!

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Methods to prepare hydroperoxides

Singlet oxygen ene reaction – Schenck reaction!

Chemical methods: peroxomolybdates intermediates!

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Methods to prepare hydroperoxides

Schenck reaction on trisubstituted olefins!

regioselectivity and stereoselectivity

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Methods to prepare hydroperoxides

Nucleophilic substitution on allylic alcohols !

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Hydroperoxides of our concern

Lin-7-OOH! Lim-2-OOH!

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Synthesis of Lin-7-OOH

Experimental conditions : obtention of 1O2

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Schenck reaction on trisubstituted olefin!

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Synthesis of Lin-7-OOH

Experimental conditions : microemulsion

Schenck reaction on trisubstituted olefin!

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Synthesis of Lin-7-OOH

Mixture of hydroperoxides TBDPSCl Imidazole DMF 391 mg 1,2 éq. 2 éq. 8,5 mL Two isomers protected 200 mg 1,2 éq. 2 éq. 8,5 mL One single isomer protected

Chemical derivatization (silylization) of the hydroperoxides!

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Synthesis of Lin-7-OOH

Deprotection of the peroxysilane!

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Synthesis of Lin-7-OOH

Derivatization/Deprotection optimization!

Weight mixture hydroperoxides Concentration mixture hydroperoxides Reaction time Yield on the last two steps 200 mg 0,13 mol.L-1 2 days 13% 200 mg 0,11 mol.L-1 10 days 61% 200 mg 0,14 mol.L-1 10 days 59% 200 mg 0,21 mol.L-1 10 days 96% 1 g 0,21 mol.L-1 10 days 9%

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Synthesis of Lin-7-OOH

Summary!

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Synthesis of Lim-2-OOH

First tests! Schenck reaction SN2 nucleophilic substitution

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Synthesis of Lim-2-OOH

SN1 nucleophilic substitution!

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