Synthesis and electrochemical redox properties of arylated p - - PowerPoint PPT Presentation

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Synthesis and electrochemical redox properties of arylated p - - PowerPoint PPT Presentation

Synthesis and electrochemical redox properties of arylated p benzoquinones, naphthoquinones and alkylamidoalkyl p benzoquinones naphthoquinones and alkylamidoalkyl p benzoquinones Mariam al Azani, Mazen al Sulaibi, Thies Thiemann, Miguel


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Synthesis and electrochemical redox properties of arylated p‐benzoquinones, naphthoquinones and alkylamidoalkyl p benzoquinones naphthoquinones and alkylamidoalkyl‐p‐benzoquinones Mariam al Azani, Mazen al Sulaibi, Thies Thiemann, Miguel Ángel Montiel, Carlos Sánche Sánchez and Jesus Iniesta Sánche Sánchez and Jesus Iniesta Corresponding authors: thiesthiemann@yahoo.de and jesus.iniesta@ua.es

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SLIDE 4

20

O O O C H3 CH3

10 20 I (nA)

O O O CH3 C H3 CH3 C H3

  • 1.8 -1.6 -1.4 -1.2 -1.0 -0.8 -0.6 -0.4 -0.2

0.0

  • 20
  • 10

E vs Fc

+/Fc

  • 1.8 -1.6 -1.4 -1.2 -1.0 -0.8 -0.6 -0.4 -0.2

0.0

E vs Fc

+/Fc

  • 1.8 -1.6 -1.4 -1.2 -1.0 -0.8 -0.6 -0.4 -0.2

0.0

E vs Fc

+/Fc

E vs Fc /Fc

O

E vs Fc /Fc E vs Fc /Fc

5 10

O N

+

O

  • O

O Cl O

  • 10
  • 5

I (nA)

O O

  • 1.8 -1.6 -1.4 -1.2 -1.0 -0.8 -0.6 -0.4 -0.2

0.0

E vs Fc

+/Fc

  • 1.8 -1.6 -1.4 -1.2 -1.0 -0.8 -0.6 -0.4 -0.2

0.0

E vs Fc

+/Fc

  • 1.8 -1.6 -1.4 -1.2 -1.0 -0.8 -0.6 -0.4 -0.2

0.0

  • 15

E vs Fc

+/Fc

Figure 1. Cyclic voltammetry of 5 mM of benzoquinone (A), phenylbenzoquinone (B), 3‐chlorophenylbenzoquinone (C), 3‐nitrophenylbenzoquinone (D), 2,5‐tert‐Butyl‐p‐ benzoquinone (E) and phenylnaphthoquinone (F) in the ionic liquid [bmim][BF4] 100 benzoquinone (E) and phenylnaphthoquinone (F) in the ionic liquid [bmim][BF4]. 100 µm diameter Au microelectrode. Neat [bmim][BF4] (red dashed line). Scan rate 100 mV/s. Third scan recorded.

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SLIDE 5

O O

O O

O N

O NH O

4

O

O

2

  • 4
  • 2

I (nA)

  • 8
  • 6
  • 1

.8 -1 .6 -1 .4 -1 .2 -1 .0 -0 .8 -0 .6 -0 .4 -0 .2 0 .0

E v s F c

+/F

c

  • 1

.8 -1 .6 -1 .4 -1 .2 -1 .0 -0 .8 -0 .6 -0 .4 -0 .2 0 .0

E v s F c

+/F

c

Figure 2. Cyclic voltammetry of 5 mM of N‐Benzyl 3‐(1,4‐dimethoxyphen‐2‐ yl)propionamide (16a) (A), and N‐Benzyl carboxamidoethyl‐p‐benzoquinone (16b) (B) in the ionic liquid [bmim][BF4]. 100 µm diameter Au microelectrode. Scan rate 100 mV/s. Third scan recorded.