Subgroup 29
U-235 Capture Cross Section in the keV to MeV Energy Region
- O. Iwamoto (JAEA)
Progress report 2008
Subgroup 29 U-235 Capture Cross Section in the keV to MeV Energy - - PowerPoint PPT Presentation
Progress report 2008 Subgroup 29 U-235 Capture Cross Section in the keV to MeV Energy Region O. Iwamoto (JAEA) Introduction Fast-neuron critical experiments using U fuels BFS (IPPE): underestimation of sodium voided reactivity
U-235 Capture Cross Section in the keV to MeV Energy Region
Progress report 2008
MOX Sensitivity of 235U capture cross section sodium voided reactivity
criticality of FCA IX assemblies Neutron spectra
Horizontal Vertical
+
− = > <
+
1
) ( ) ( ) ( 1
1
i i
E E f c i i i
dE E E E E σ σ α i f i c i
Resonance Region JENDL-3.2 ENDF/B-VII.0 RRR 10-5 eV – 500 eV 10-5 eV – 2.25 keV URR 500 eV – 30 keV 2.25 keV – 25 keV Name Spectrum Handbook ID AVG (keV) ZEUS1 Intermediate HEU-MET-INTER-006, case1 5.05 ZEUS2 Intermediate HEU-MET-INTER-006, case2 10.33 ZEUS3 Intermediate HEU-MET-INTER-006, case3 24.02 ZEUS4 Intermediate HEU-MET-INTER-006, case4 FCA-IX-1 Intermediate 29.90 FCA-IX-2 Intermediate 116.52 FCA-IX-3 Intermediate 211.30
500 eV 2.25 kev 25 keV 30 keV RR( ENDF) RR (ENDF) (JENDL) (JENDL) 500 eV 2.25 kev 25 keV 30 keV RR( ENDF) (JENDL) (JENDL) (JENDL)
Case 1 Case 2
500 eV 2.25 kev 25 keV 30 keV RR( JENDL) (JENDL) (JENDL) ENDF FILE 3 500 eV 2.25 kev 25 keV 30 keV RR( JENDL) RR (ENDF) (ENDF) ENDF FILE 3
Case 3 Case 4 Case 5
500 eV 2.25 kev 25 keV 30 keV RR( ENDF) RR (JENDL) (ENDF) ENDF FILE 3
‐3 % ‐10 %
ZEUS1 ZEUS2 ZEUS3 ZEUS4
FCA‐IX‐1 FCA‐IX‐2 FCA‐IX‐3
Sensitivities of U‐235 capture to keff used in adjustment
Case 1: Uncertainties of experimental data are assumed to be 0.1%dk/kk’ correlation among the data of the same critical assembly is 0.8. Case 2: Uncertainties of experimental data are assumed to be 1.0%dk/kk’ correlation among the data of the same critical assembly is 0.95.
C/E values before and after adjustment Relative change in U‐235 capture
larger than JENDL-3.2 and statistical model calculations in the range of about 100eV to 3keV. Discrepancies are found also in the elastic scattering cross sections below 30 keV. The total and fission cross sections have no such noticeable discrepancies.
results.
2.25keV has a large impact on both the FCA-IX and Zeus calculations while difference below 500eV has an impact only on the Zeus calculations.
JENDL-3.2 for uranium-235 makes the C/E dependence on spectrum hardness smaller. However, this also results in unacceptable high C/E values. This can be an indication that there exists other energy region which also contributes to the multiplication factor. These cases need further investigation.
1 DEN/DER/SPRC WPEC meeting Tokai-mura, June 3-4-5, 2008
U-235 capture cross section around 1 keV – Is there a problem? (Ref. JEF/DOC-1250)
1. Introduction 2. Benchmark description and calculation 3. Analysis and discussion 4. Summary and conclusion
2 DEN/DER/SPRC WPEC meeting Tokai-mura, June 3-4-5, 2008
“Inconsistencies” reported by JAEA
cores: FCA IX-1, XI-2, XI-3 reactivity measurement BFS-62-3A sodium void measurement ZPPR-18A control rod measurement
JAEA proposed to investigate the problem under WPEC → SG29
Studied by CEA/KAERI as a contribution to SG29 Introduction
3 DEN/DER/SPRC WPEC meeting Tokai-mura, June 3-4-5, 2008
FCA IX-1, IX-2, XI-3 benchmark
Homogeneous core characteristics Benchmark description and calculations
7.77 12.5 26.8 Graphite/Uranium 0.20 0.39 1.00 (ref)
0.62 0.46 0.30 Spectral hardness r 0.87 0.93 1.00 (ref) Core C-12 rel. content 1.00 1.00 1.00 (ref) Core rel. steel content 3.00 2.00 1.00 (ref) Core rel. U-238 content 3.00 2.00 1.00 (ref) Core rel. U-235 content 35.56 40.64 60.96 Core height (cm) 17.89 23.10 30.35 Core outer radius (cm) IX-3 IX-2 IX-1
4 DEN/DER/SPRC WPEC meeting Tokai-mura, June 3-4-5, 2008
JAEA results using JENDL-3.2 and JENDL-3.3 + JAEA code system Benchmark description and calculations
5 DEN/DER/SPRC WPEC meeting Tokai-mura, June 3-4-5, 2008
KAERI/CEA results using JEF-2.2 and JEFF-3.1 + ERANOS code Benchmark description and calculations
0.99000 0.99500 1.00000 1.00500 1.01000 1.01500 FCA-IX-1 FCA-IX-2 FCA-IX-3
Experiment no. C/E of k-effective
JEFF-3.1 JEF-2.2
0.1 1 10 100 1000 10000 100000 1e+06 1e+07 1e+08
Relative sensitivity Energy [eV] FCA-IX-1 FCA-IX-2 FCA-IX-3
k-effective C/E Sensitivity of k-eff to the U-235 Capture XS
6 DEN/DER/SPRC WPEC meeting Tokai-mura, June 3-4-5, 2008
Breakdown of the calculated JEFF-3.1 – JEF-2.2 reactivity difference (in pcm) Analysis and discussion
Total
Fission spectrum
Other nuclides 871 759 577 U-238
U-235 IX-3 IX-2 IX-1
7 DEN/DER/SPRC WPEC meeting Tokai-mura, June 3-4-5, 2008
Breakdown of JEFF-3.1 – JEF-2.2 reactivity difference by nuclide and region Analysis and discussion
U235 U238 H1 C0 O16 CR50 CR52 CR53 CR54 MN55 FE54 FE56 FE57 FE58 NI58 NI60 NI61 NI62 NI64
2.60E-18 2.50E-03 5.00E-03 7.50E-03 1.00E-02
FCA-IX-1 FCA-IX-2 FCA-IX-3
Nuclide Contribution to reactivity change
Core Blanket
8 DEN/DER/SPRC WPEC meeting Tokai-mura, June 3-4-5, 2008
Breakdown of JEFF-3.1 – JEF-2.2 reactivity difference by nuclide and reaction Analysis and discussion
0.0E+00 5.0E-03 1.0E-02
U235 U238 H1 C0 O16 CR50 CR52 CR53 CR54 MN55 FE54 FE56 FE57 FE58 NI58 NI60 NI61 NI62 NI64 Contribution to reactivity change
TRANSPORT N,XN INELASTIC ELASTIC FISSION CAPTURE
FCA-IX-1
0.0E+00 2.0E-03 4.0E-03 6.0E-03 8.0E-03 1.0E-02
U235 U238 H1 C0 O16 CR50 CR52 CR53 CR54 MN55 FE54 FE56 FE57 FE58 NI58 NI60 NI61 NI62 NI64 Contribution to reactivity change
TRANSPORT N,XN INELASTIC ELASTIC FISSION CAPTURE
0.0E+00 2.0E-03 4.0E-03 6.0E-03 8.0E-03 1.0E-02 1.2E-02
U235 U238 H1 C0 O16 CR50 CR52 CR53 CR54 MN5 FE54 FE56 FE57 FE58 NI58 NI60 NI61 NI62 NI64 Contribution to reactivity change
TRANSPORT N,XN INELASTIC ELASTIC FISSION CAPTURE
FCA-IX-3 FCA-IX-2
9 DEN/DER/SPRC WPEC meeting Tokai-mura, June 3-4-5, 2008
U-235 contributions to the JEFF-3.1 – JEF-2.2 reactivity difference Analysis and discussion
0.00 50.00 1e-01 1e+00 1e+01 1e+02 1e+03 1e+04 1e+05 1e+06 1e+07 1e+08 Energy [eV] Capture Fission Elastic Inelastic n,xn Transport Sum Contribution to reactivity change [pcm]
0.00 50.00 1e-01 1e+00 1e+01 1e+02 1e+03 1e+04 1e+05 1e+06 1e+07 1e+08 Energy [eV] Capture Fission Elastic Inelastic n,xn Transport Sum Contribution to reactivity change [pcm]
FCA-IX-3 FCA-IX-2
0.00 50.00 1e-01 1e+00 1e+01 1e+02 1e+03 1e+04 1e+05 1e+06 1e+07 1e+08 Energy [eV] Capture Fission Elastic Inelastic n,xn Transport Sum Contribution to reactivity change [pcm]
FCA-IX-1
10 10 DEN/DER/SPRC WPEC meeting Tokai-mura, June 3-4-5, 2008
U-238 contributions to the JEFF-3.1 – JEF-2.2 reactivity difference Analysis and discussion
0.00 50.00 100.00 150.00 200.00 250.00 300.00 1e-01 1e+00 1e+01 1e+02 1e+03 1e+04 1e+05 1e+06 1e+07 1e+08 Energy [eV] Capture Fission Elastic Inelastic n,xn Transport Sum Contribution to reactivity change [pcm]
0.00 50.00 100.00 150.00 200.00 250.00 300.00 1e-01 1e+00 1e+01 1e+02 1e+03 1e+04 1e+05 1e+06 1e+07 1e+08 Energy [eV] Capture Fission Elastic Inelastic n,xn Transport Sum Contribution to reactivity change [pcm]
0.00 50.00 100.00 150.00 200.00 250.00 300.00 1e-01 1e+00 1e+01 1e+02 1e+03 1e+04 1e+05 1e+06 1e+07 1e+08 Energy [eV] Capture Fission Elastic Inelastic n,xn Transport Sum Contribution to reactivity change [pcm]
FCA-IX-1 FCA-IX-3 FCA-IX-2
11 11 DEN/DER/SPRC WPEC meeting Tokai-mura, June 3-4-5, 2008
Summary
by CEA/KAERI using JEFF files
depleted U blanket provided by JAEA under WPEC/SG29
between the JEF-2.2 and JEFF-3.1 U-235 capture & fission cross sections in the core → net <0 term U-238 transport cross section (l > 0) in the blanket → net >0 term
235 capture in the keV range, a fairly good C/E agreement appears to be
Summary and conclusion
12 12 DEN/DER/SPRC WPEC meeting Tokai-mura, June 3-4-5, 2008
Conclusion
alone, but from positive and negative contributions of various magnitude mainly caused by U-235 capture: negative, keV range U-235 fission: negative 100 keV range, positive MeV range U-238 transport: positive, MeV range
and one cannot immediately conclude that there is a problem with the latest evaluated U-235 capture cross section around 1 keV
(and JENDL-3.3) U-235 capture cross section in the keV region, but the FCA IX-1, IX-2, IX3 benchmarks alone do not provide enough evidence to motivate changes
Summary and conclusion
P1 elastic scattering cross section of U-238 JEFF-2.2, JENDL-3.3 >> JEFF-3.1, JENDL/AC
Sensitivity of P1 elastic scattering cross section of U-238 to keff
C/E of criticality of small fast systems `Reflector bias’ observed in the JENDL-3.3 results disappears in JENDL/AC due to the revision of P1 elastic of U-238.
C/E for criticality of small fast systems
C/E of criticality of uranium-fueled fast systems
0.990 0.995 1.000 1.005 1.010 1.015 1.020 B F S
2
Z e u s
H M F 3 Z P P R
1 F F C A
X
Z P R
/ 2 3 B i g T e n F l a t t
5 G
i v a C/E ENDF/B-VII.0 JENDL/AC
Sensitivity of U5 capture to keff
04/June/2008 WPEC SG29 Meeting 1
Reactor Physics Group, JAEA
04/June/2008 WPEC SG29 Meeting 2
To evaluate U-235 capture cross section, a new experimental core was considered. From view point of effectiveness of U-235 capture cross section evaluation in kev energy range, the previous results were taken into account;
To check the effectiveness, the following sensitivity was considered;
Σ ΔΣ ⋅ = Σ ΔΣ ⋅ Σ ΔΣ Δ ⇒ − = → Δ S J J J J J J ρ ρ ρ ρ ρ ρ ρ ) 33 ( ) 33 ( ) 32 ( ) 33 ( ) 32 33 (
04/June/2008 WPEC SG29 Meeting 3
C(1/4") C(1/4") C(1/16") C(1/16") HEU(1/16") HEU(1/16") C(1/4") C(1/4") C(1/4") C(1/4") C(1/4") C(1/4") C(1/4") C(1/4") C(1/4") EU(1/8") EU(1/16") C(1/4") HEU(1/16") EU(1/16") EU(1/8") C(1/4") EU(1/16")
Reference fuel cell (FCA-IX-1 core) Fuel cell for New Core (Averaged Enrichment=32wt%)
04/June/2008 WPEC SG29 Meeting 4
Na cell Void cell
NA NA SUS NA NA HEU(1/16") HEU(1/16") NA NA NA SUS SSV SSV SUS SSV HEU(1/16") SSV SSV HEU(1/16") SSV SUS SSV
FCA-IX-1 core
04/June/2008 WPEC SG29 Meeting 5
Na cell Void cell
NA EU(1/8") NA NA NA NA HEU(1/16") EU(1/16") EU(1/16") EU(1/8") EU(1/16") NA EU(1/8") SSV HEU(1/16") EU(1/16") SSV EU(1/16") SSV SSV EU(1/8") SSV EU(1/16") SSV
New Core (Case6)
04/June/2008 WPEC SG29 Meeting 6
X X X X
Test zone Radial blanket(DUB) Core Test zone Test zone
Core Radial blanket(DUB) Radial blanket(DUB) Axial blanket (DUB) Axial blanket (DUB)
Test zone
r~30cm H~60cm
04/June/2008 WPEC SG29 Meeting 7
X X X X
Radial blanket(SB) Radial blanket(DUB) Core Test zone
Core Radial blanket(SB) Radial blanket(SB) Axial blanket (SB) Radial blanket(DUB) Radial blanket(DUB) Axial blanket (SB)
Test zone
r~30cm H~60cm
04/June/2008 WPEC SG29 Meeting 8
Isotope and Reaction Breakdown of Sensitivity ( )
0.0 0.1 0.2 0.3 0.4 U235 Cap. U235 Fiss. U238 Cap. C Elas. C Mu Na Cap. Na Elas. Na Inelas. Cr Elas. Fe Cap. Fe Elas. Total All Ref(L=20.3cm) Ref(L=40.6cm)
Δρ(J33->J32)/ ρ(J33)
0.0 0.1 0.2 0.3 0.4 U235 Cap. U235 Fiss. U238 Cap. C Elas. C Mu Na Cap. Na Elas. Na Inelas. Cr Elas. Fe Cap. Fe Elas. Total All SB(L=20.3cm)J33 SB(L=40.6cm)J33
Δρ(J33->J32)/ ρ(J33)
Ref core (FCA-IX-1)
ρ(J33)=-34pcm(L=20.3cm) =-83pcm(L=40.3cm)
New core(with SB regions)
ρ(J33)=- 67pcm(L=20.3cm) =-180pcm(L=40.3cm)
(L : Axial length of perturbed region)
) 33 ( ) 32 33 ( J J J ρ ρ → Δ
04/June/2008 WPEC SG29 Meeting 9
Energy Breakdown of Sensitivity of Na Void Reactivity Worth ( ) for U-235 Capture Cross Sections
(注:Lは摂動領域長を表す。)
0.00 0.02 0.04 0.06 0.08 0.10 0.12 0.14 101 102 103 104 105 106 107
Ref(L=20.3cm) Case6(L=20.3cm) Case6SB(L=20.3cm) SB(L=20.3cm)
Δρ
(J33->J32)/ρ (J33)
En(eV)
(void region:-2Z to +2Z)
) 33 ( ) 32 33 ( J J J ρ ρ → Δ
04/June/2008 WPEC SG29 Meeting 10
Energy Breakdown of Sensitivity of Na Void Reactivity Worth ( ) for U-235 Capture Cross Sections
(注:Lは摂動領域長を表す。)
0.00 0.02 0.04 0.06 0.08 0.10 0.12 0.14 101 102 103 104 105 106 107
Ref(L=40.6cm) Case6(L=40.6cm) Case6SB(L=40.6cm) SB(L=40.6cm)
Δρ
(J33->J32)/ρ (J33)
En(eV)
(void region:-4Z to +4Z)
) 33 ( ) 32 33 ( J J J ρ ρ → Δ
04/June/2008 WPEC SG29 Meeting 11
A new experimental core was selected to evaluate U-235 capture cross section in kev energy range. Na void reactivity worth measurement is effective in the evaluation of U-235 capture cross section. The experiment was delay since FCA operation stopped in July, 2007. The experimental core will be constructed in the end of this FY and measurements will carried out in the beginning of the next FY. (FCA operation will restart in November, 2008.)